IP Library Granted Patent US 10,633,400
Granted Patent B2
US 10,633,400 · App. 15/593,165 · Granted Apr 28, 2020

Nanocomposite silicon oxygen carbon materials and uses

Inventors: Andrew R. Hopkins (Sylvania, OH); Douglas M. Dukes (Troy, NY); Brian L. Benac (Hadley, NY); Ashish P. Diwanji (New Albany, OH); Charles C. Rinzler (Cambridge, MA); Mark S. Land (Houston, TX)
Assignee: Melior Innovations, Inc.
C07F7/0803B82Y30/00C04B35/56C04B35/5603C04B35/571C04B35/806C07F7/0838C07F7/1804C08G77/12C08K3/14C08K5/56C08L83/00C08L83/04C08L83/06C09K8/80C01P2002/60C04B2235/3418C04B2235/3826C04B2235/44C04B2235/48C04B2235/483C04B2235/528C04B2235/5427C04B2235/5436C04B2235/6581C04B2235/77C04B2235/96C08G77/20C08G77/80C08L83/14Y10T428/131
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Quick Facts
Patent No.
US 10,633,400
App. No.
15/593,165
Granted
Apr 28, 2020
Kind
B2
Abstract

Nanocomposite silicon and carbon compositions. These compositions can be made from polymer derived ceramics, and in particular, polysilocarb precursors. The nanocomposite can have non-voids or be nano-void free and can form larger macro-structures and macro-composite structures. The nanocomposite can contain free carbon domains in an amorphous SiOC matrix.

Claims (30)

1. A nanocomposite material comprising: a first composition comprising silicon, free carbon and a first moiety, wherein the first moiety is selected from the group consisting of Si(CH 3 ) 3 O, Si(CH 3 ) 2 O 2 , SiC 2 O 2 , Si(CH 3 )(OH)O 2 , SiCO 3 , SiO 4 , esters, ketones, sp 2 carbon structures, sp 2 carbon structures containing 6 to 20 carbons, —C—O—C—, —C—O—Si—, alkanes, terminal end Si(CH 3 ) 2 O, —Si—C—Si—, —Si(CH 3 ) 2 O 2 , and Si(CH 3 )O 2 ;

and a second composition comprising silicon and a second moiety; and

wherein the first and second compositions are different compositions.

2. The nanocomposite of claim 1 , wherein the first moiety and the second moiety are the same.

3. The nanocomposite of claim 1 , wherein the first moiety and the second moiety are different.

4. The nanocomposite of claim 1 , comprising a third composition; and wherein the third composition is different from the first and second compositions.

5. The nanocomposite of claim 2 , comprising a third composition; and wherein the third composition is different from the first and second compositions.

6. The nanocomposite of claim 3 , comprising a third composition; and wherein the third composition is different from the first and second compositions.

7. The nanocomposite of claim 1 , wherein the first composition is a bulk phase.

8. The nanocomposite of claim 2 , wherein the first composition is a bulk phase.

9. The nanocomposite of claim 3 , wherein the first composition is a bulk phase.

10. The nanocomposite of claim 1 , wherein the second composition is a bulk phase.

11. The nanocomposite of claim 2 , wherein the second composition is a polymer derived ceramic composition and is a bulk phase.

12. The nanocomposite of claim 3 , wherein the second composition is a polymer derived ceramic composition and is a bulk phase.

13. The nanocomposite of claim 1 , wherein the second composition is selected from the group consisting of Si(CH 3 ) 3 O, SiC 3 O, SiC 4 , Si(CH 3 ) 2 O 2 , SiC 2 O 2 , Si(CH 3 )(OH)O 2 , SiCO 3 , and SiO 4 .

14. The nanocomposite of claim 3 , wherein the second composition is selected from the group consisting of Si(CH 3 ) 3 O, SiC 3 O, SiC 4 , Si(CH 3 ) 2 O 2 , SiC 2 O 2 , Si(CH 3 )(OH)O 2 , SiCO 3 , and SiO 4 .

15. The nanocomposite of claim 9 , wherein the second composition is selected from the group consisting of Si(CH 3 ) 3 O, SiC 3 O, SiC 4 , Si(CH 3 ) 2 O 2 , SiC 2 O 2 , Si(CH 3 )(OH)O 2 , SiCO 3 , and SiO 4 .

16. The nanocomposite of claim 1 , wherein the second composition comprises a moiety selected from the group consisting of esters, ketones, sp 2 carbon structures, —C—O—C—, —C—O—Si—, alkanes, terminal end Si(CH 3 ) 2 O, —Si—C—Si—, —Si(CH 3 ) 2 O 2 , and Si(CH 3 )O 2 .

17. The nanocomposite of claim 2 , wherein the second composition comprises a moiety selected from the group consisting of esters, ketones, aromatic sp 2 carbon structures having 6 or more carbons, —C—O—C—, —C—O—Si—, alkanes, terminal end Si(CH 3 ) 2 O, —Si—C—Si—, —Si(CH 3 ) 2 O 2 , and Si(CH 3 )O 2 .

18. The nanocomposite of claim 4 , wherein the second composition comprises a moiety selected from the group consisting of esters, ketones, sp 2 carbon, —C—O—C—, —C—O—Si—, alkanes, terminal end Si(CH 3 ) 2 O, —Si—C—Si—, Si(CH 3 )O 3 , —Si(CH 3 ) 2 O 2 , and Si(CH 3 )O 2 .

19. The nanocomposite of claim 10 , wherein the second composition comprises a moiety selected from the group consisting of esters, ketones, sp 2 carbon structures, —C—O—C—, —C—O—Si—, alkanes, terminal end Si(CH 3 ) 2 O, —Si—C—Si—, Si(CH 3 )O 3 , —Si(CH 3 ) 2 O 2 , and Si(CH 3 )O 2 .

20. The nanocomposite of 1, having a specific gravity of from about 1.8 to about 2.2 and being substantial free of nano-voids larger than 0.01 μm.

21. The nanocomposite of 2, having a specific gravity of from about 1.8 to about 2.2 and being substantial free of nano-voids larger than 0.01 μm.

22. The nanocomposite of 3, having a specific gravity of from about 1.8 to about 2.2 and being substantial free of nano-voids larger than 0.01 μm.

23. The nanocomposite of 7, having a specific gravity of from about 1.8 to about 2.2 and being substantial free of nano-voids larger than 0.1 μm.

24. The nanocomposite of 10, having a specific gravity of from about 1.8 to about 2.5 and being substantial free of nano-voids larger than 0.001 μm.

25. The nanocomposite of 14, having a specific gravity of from about 1.8 to about 2.2 and being substantial free of nano-voids larger than 0.01 μm.

26. The nanocomposite of 9, having a specific gravity of from about 1.8 to about 2.5 and being substantial free of nano-voids larger than 0.01 μm.

27. The nanocomposite of 17, having a specific gravity of from about 1.8 to about 2.2 and being substantial free of nano-voids larger than 0.001 μm.

28. The nanocomposite of 13, having a specific gravity of from about 1.8 to about 2.5 and being substantial free of nano-voids larger than 0.01 μm.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 19, 2020
From: HOPKINS, ANDREW; DUKES, DOUGLAS M; BENAC, BRIAN L; DIWANJI, ASHISH P; RINZLER, CHARLES C; LAND, MARK S
To: MELIOR INNOVATIONS, INC.
Reel/Frame 052159/0453 →
Continuity (4)
Continuation In Part 14634814 · Feb 28, 2015
Continuation In Part 14634819 · Feb 28, 2015
Provisional Application 62335556 · May 12, 2016
Related Publication 20180065995A1 · Mar 8, 2018