IP Library Granted Patent US 12,342,813
Granted Patent B2
US 12,342,813 · App. 15/704,113 · Granted Jul 1, 2025

Amine and amine oxide surfactants for controlling herbicide spray drift

Inventors: Brandon Matthew Downer (Lebanon, IN); Mei Li (Westfield, IN); Lei Liu (Carmel, IN); Kuide Qin (Chapel Hill, NC); Holger Tank (Indianapolis, IN); Stephen L. Wilson (Zionsville, IN); Hong Zhang (Carmel, IN)
Assignee: CORTEVA AGRISCIENCE LLC
A01N25/24A01N25/06A01N25/30A01N37/40A01N57/20
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Quick Facts
Patent No.
US 12,342,813
App. No.
15/704,113
Granted
Jul 1, 2025
Kind
B2
Abstract

Spray drift during the application of an aqueous mixture of glyphosate and an auxinic herbicide is reduced by incorporating certain tertiary amine or tertiary amine oxide surfactants into the aqueous solution or mixture to be sprayed.

Claims (37)

1. A method of reducing spray drift of an aqueous herbicidal spray mixture, comprising:

formulating an aqueous herbicidal spray mixture comprising:

glyphosate;

an auxinic herbicide; and

from about 0.02 to about 2 weight percent of a tertiary amine surfactant of the formula:

wherein R 1 represents a straight or branched chain (C 12 -C 18 ) alkyl and R 2 and R 3 independently represent a straight or branched chain (C 1 -C 18 ) alkyl, and

wherein the aqueous herbicidal spray mixture comprises a plurality of spray droplets having a volume mean diameter greater than 165 μm.

2. The method of claim 1 , wherein the auxinic herbicide is a water soluble salt of 2,4-D, a water soluble salt of triclopyr, a water soluble salt of dicamba, or mixtures thereof.

3. The method of claim 1 , wherein the tertiary amine surfactant is selected from the group consisting of cocoalkyldimethylamine, dimethyltallowalkylamine, and mixtures thereof.

4. The method of claim 2 , wherein the water-soluble salt of the auxinic herbicide is selected from the group consisting of isopropyl ammonium salt, dimethyl ammonium salt, trietbyl ammonium salt, monoethanol ammonium salt, diethanol ammonium salt, diethyleneglycol ammonium salt, triisopropanol ammonium salt, tetramethyl ammonium salt, tetraethyl ammonium salt, and choline salt.

5. The method of claim 1 , wherein the plurality of spray droplets has a volume percent of spray droplets smaller than 150 μm in diameter that is less than that of an aqueous spray mixture that does not include the tertiary amine surfactant.

6. The method of claim 1 , wherein the aqueous spray mixture is homogeneous and free-flowing at temperatures between 54° C. and −10° C.

7. The method of claim 2 , wherein the tertiary amine surfactant is selected from the group consisting of cocoalkyldimethylamine, dimethyltallowalkylamine, and mixtures thereof.

8. The method of claim 3 , wherein the water-soluble salt of the auxinic herbicide is selected from the group consisting of isopropyl ammonium salt, dimethyl ammonium salt, triethyl ammonium salt, monoethanol ammonium salt, diethanol ammonium salt, diethyleneglycol ammonium salt, triisopropanol ammonium salt, tetramethyl ammonium salt, tetraethyl ammonium salt, and choline salt.

9. The method of claim 1 , wherein the plurality of spray droplets has a volume percent of spray droplets smaller than 150 μm in diameter that is equal to or less than about 15.7%.

10. A reduced spray drift aqueous herbicidal spray formulation, comprising:

a plurality of spray droplets having a volume mean diameter greater than 165 μm comprising:

glyphosate;

an auxinic berbicide; and

from about 0.02 to about 2 weight percent of a tertiary amine surfactant of the formula:

wherein R 1 represents a straight or branched chain (C 12 -C 18 ) alkyl and R 2 and R 3 independently represent a straight or branched chain (C 1 -C 18 ) alkyl.

11. The formulation of claim 10 , wherein the auxinic herbicide is a water soluble salt of 2,4-D, a water soluble salt of triclopyr, a water soluble salt of dicamba, or mixtures thereof.

12. The formulation of claim 10 , wherein the tertiary amine surfactant is selected from the group consisting of cocoalkyldimethylamine, dimethyltallowalkylamine, and mixtures thereof.

13. The formulation of claim 11 , wherein the water-soluble salt of the auxinic herbicide is selected from the group consisting of isopropyl ammonium salt, dimethyl ammonium salt, triethyl ammonium salt, monoethanol ammonium salt, diethanol ammonium salt, diethyleneglycol ammonium salt, triisopropanol ammonium salt, tetramethyl ammonium salt, tetraethyl ammonium salt, and choline salt.

14. The formulation of claim 10 , wherein the plurality of spray droplets has a volume percent of spray droplets smaller than 150 μm in diameter that is less than that of an aqueous spray mixture that does not include the tertiary amine surfactant.

15. The formulation of claim 10 , wherein the aqueous spray mixture is homogeneous and free-flowing at temperatures between 54° C. and −10° C.

16. The formulation of claim 11 , wherein the tertiary amine surfactant is selected from the group consisting of cocoalkyldimethylamine, dimethyltallowalkylamine, and mixtures thereof.

17. The formulation of claim 12 , wherein the water-soluble salt of the auxinic herbicide is selected from the group consisting of isopropyl ammonium salt, dimethyl ammonium salt, triethyl ammonium salt, monoethanol ammonium salt, diethanol ammonium salt, diethyleneglycol ammonium salt, triisopropanol ammonium salt, tetramethyl ammonium salt, tetraethyl ammonium salt, and choline salt.

18. The formulation of claim 10 , wherein the plurality of spray droplets has a volume percent of spray droplets smaller than 150 μm in diameter that is equal to or less than about 15.7%.

19. A method of reducing spray drift of an aqueous herbicidal spray mixture, comprising:

formulating an aqueous herbicidal spray mixture comprising:

glyphosate;

an auxinic herbicide; and

from about 0.02 to about 2 weight percent of a tertiary amine surfactant of the formula:

wherein R 1 represents a straight or branched chain (C 12 -C 18 ) alkyl and R 2 and R 3 independently represent a straight or branched chain (C 1 -C 18 ) alkyl, and

wherein the aqueous herbicidal spray mixture comprises a plurality of spray droplets having a volume mean diameter greater than 165 μm; and

spraying the formulation with a flat fan nozzle at 40 psi.

Assignments (3)
CHANGE OF NAME Recorded Nov 11, 2022
From: DOW AGROSCIENCES LLC
To: CORTEVA AGRISCIENCE LLC
Reel/Frame 061931/0688 →
CHANGE OF NAME Recorded Nov 8, 2021
From: DOW AGROSCIENCES LLC
To: CORTEVA AGRISCIENCE LLC
Reel/Frame 058044/0184 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 14, 2018
From: DOWNER, BRANDON MATTHEW; LI, MEI; LIU, LEI; QIN, KUIDE; TANK, HOLGER; WILSON, STEPHEN L.; ZHANG, HONG
To: DOW AGROSCIENCES LLC
Reel/Frame 046780/0259 →
Continuity (3)
Continuation 13232377 · Sep 14, 2011
Provisional Application 61383074 · Sep 15, 2010
Related Publication 20180168146A1 · Jun 21, 2018
References Cited (10)
US 5710103A · Magin et al. · 1998 [cited by applicant]
US 5998332A · Sato · 1999 [cited by examiner]
US 6930075B1 · Mason · 2005 [cited by examiner]
US 9781922B2 · Downer · 2017 [cited by examiner]
US 20010019996A1 · Soula · 2001 [cited by examiner]
US 20050261130A1 · Lennon et al. · 2005 [cited by applicant]
US 20090318294A1 · Malec et al. · 2009 [cited by applicant]
US 20100099569A1 · Ogawa · 2010 [cited by examiner]
US 20110190130A1 · Carranza Garzon · 2011 [cited by examiner]
WO 0269718A2 · 2002 [cited by applicant]