IP Library Granted Patent US 11,117,837
Granted Patent B2
US 11,117,837 · App. 15/720,433 · Granted Sep 14, 2021

Polyamide powder for selective sintering methods

Inventors: Wolfgang Diekmann (Waltrop, DE); Maik Grebe (Bochum, DE); Franz-Erich Baumann (Dülmen, DE); Sylvia Monsheimer (Haltern am See, DE); Beatrice Küting (Marl, DE)
Assignee: Evonik Operations GbmH
C04B35/63468B29C64/165B33Y70/00C08G69/14C08G69/28C08J3/14B29C64/153C08J2377/02C08J2377/06
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Quick Facts
Patent No.
US 11,117,837
App. No.
15/720,433
Granted
Sep 14, 2021
Kind
B2
Abstract

A polyamide powder for selective absorbing sintering, SAS, or selective inhibition sintering, SIS. The polyamide powder has a solution viscosity to ISO 307 of 1.8 to 2 and a rise in the solution viscosity of 0% to 25% when it is subjected to a temperature 20° C. below its melting temperature under air for 20 hours.

Claims (14)

1. A polyamide powder for selective absorbing sintering, SAS, or selective inhibition sintering, SIS, wherein the polyamide has a solution viscosity to ISO 307 of 1.8 to 2, a rise in the solution viscosity of 5% to 25%, when subjected to a temperature 20° C. below its melting temperature under air for 20 hours, and an excess of carboxylic acid end groups over amine end groups of 20 to 60 mmol/kg,

wherein a surface energy of the polyamide, determined by a contact angle measurement by a capillary rise height method by use of the Washburn equation and the evaluation method according to Owens, Wendt, Rabel and Kaelble, is not more than 35 mN/m and

a BET surface area of the polyamide powder, measured to DIN ISO 9277, is from 10 m 2 /g to 30 m 2 /g.

2. The polyamide powder according to claim 1 , wherein the polyamide has a rise in solution viscosity of 5 to 15% when subjected to a temperature 20° C. below its melting temperature under air for 20 hours.

3. The polyamide powder according to claim 1 , wherein the excess is achieved by dicarboxylic acids.

4. The polyamide powder according claim 1 , wherein the powder has open mesopores and the cumulative pore volume distribution of the mesopores, measured to DIN 66134, is at least 0.01 cm 3 /g.

5. The polyamide powder according to claim 1 , wherein the polyamide powder absorbs liquid in a volume of 1,000 pl/g to 30,000 pl/g.

6. The polyamide powder according to claim 1 , wherein a weight-average particle diameter d 50 of the polyamide powder, measured by laser diffraction, is not more than 100 μm.

7. The polyamide powder according to claim 1 , wherein a weight-average particle diameter d 50 of the polyamide powder, measured by laser diffraction, is from 10 μm to 80 μm.

8. The polyamide powder according to claim 1 , wherein a bulk density of the polyamide powder, measured to DIN 53466, is between 300 g/l and 600 g/l.

9. The polyamide powder according to claim 1 , wherein a surface energy of the polyamide, determined by a contact angle measurement by a capillary rise height method by use of the Washburn equation and the evaluation method according to Owens, Wendt, Rabel and Kaelble, is from 25 mN/m to 32 mN/m.

10. The polyamide powder according to claim 1 , wherein the polyamide powder is obtained by a precipitation process.

11. Shaped bodies which are obtained at least partly from the polyamide powder according to claim 1 .

12. The polyamide powder according to claim 10 , wherein a suspension obtained by precipitation is left at a temperature of 2-4 K above the precipitation temperature for 10 to 180 min, after precipitation.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 23, 2019
From: DIEKMANN, WOLFGANG; GREBE, MAIK; BAUMANN, FRANZ-ERICH; MONSHEIMER, SYLVIA; KÜTING, BEATRICE
To: EVONIK DEGUSSA GMBH
Reel/Frame 051098/0378 →
CHANGE OF NAME Recorded Nov 18, 2019
From: EVONIK DEGUSSA GMBH
To: EVONIK OPERATIONS GMBH
Reel/Frame 051045/0872 →
Priority Claims (1)
DE 102016219080.6 · Sep 30, 2016 · national
Continuity (1)
Related Publication 20180093925A1 · Apr 5, 2018
Cited By (3)
US 12,351,538 US 12,570,800 US 12,605,909