IP Library Granted Patent US 10,988,596
Granted Patent B2
US 10,988,596 · App. 15/746,142 · Granted Apr 27, 2021

Method for stabilising a composition made from poly(arylene-ether-ketone) (PAEK)

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Quick Facts
Patent No.
US 10,988,596
App. No.
15/746,142
Granted
Apr 27, 2021
Kind
B2
Abstract

A method for stabilizing a composition made from PAEK, said method including a step of incorporating a stabilizing agent against thermo-oxidation phenomena, said method being characterized in that said incorporated stabilizing agent is a phosphate salt, or a mixture of phosphate salts. The phosphate salt is incorporated into the composition based on PAEK by one of the following techniques: dry blending, compounding, wet impregnation or during the process for synthesizing the PAEK polymer.

Claims (20)

1. A process for the stabilization of a composition based on PAEK, said process comprising:

incorporating by wet impregnation an aqueous solution comprising a stabilizing agent, wherein the stabilizing agent stabilizes with regard to the phenomena of thermal oxidation; and

stabilizing the composition, while the composition is at a temperature of greater than 350° C., to obtain the composition in molten state,

wherein the stabilizing agent is a water-soluble phosphate salt or a mixture of water-soluble phosphate salts, wherein the stabilizing agent does not comprise phosphite or phosphonite.

2. The process as claimed in claim 1 , wherein the phosphate salt(s) is (are) chosen from at least one of the following salts: one (or more) phosphate salt(s) of ammonium, of sodium, of calcium, of zinc, of potassium, of aluminum, of magnesium, of zirconium, of barium, of lithium, or of rare earths.

3. The process as claimed in claim 1 , wherein the phosphate salt(s) is (are) chosen from at least one of the following compounds: anhydrous monosodium phosphate, monosodium phosphate monohydrate or monosodium phosphate dihydrate, anhydrous disodium phosphate, disodium phosphate dihydrate, disodium phosphate heptahydrate, disodium phosphate octahydrate or disodium phosphate dodecahydrate, anhydrous hexagonal trisodium phosphate, anhydrous cubic trisodium phosphate, trisodium phosphate hemihydrate, trisodium phosphate hexahydrate, trisodium phosphate octahydrate, trisodium phosphate dodecahydrate, or ammonium dihydrogen phosphate.

4. The process as claimed in claim 1 , wherein the phosphate salt is incorporated into the composition in proportions of between 10 ppm and 50,000 ppm.

5. The process as claimed in claim 1 , wherein the composition based on PAEK is a composition based on one of the following polymers: PEKK, PEEK, PEEKK, PEKEKK, PEEEK or PEDEK.

6. The process as claimed in claim 1 , wherein the composition based on PAEK is a poly(ether ketone ketone) (PEKK) composition.

7. The process as claimed in claim 4 , wherein the composition based on PAEK is a composition based on PEKK, and comprises, in addition to the PEKK, at least one of the following polymers: PEK, PEEKEK, PEEK, PEEKK, PEKEKK, PEEEK, PEDEK, with a content of less than 50% by weight of the composition.

8. A process for the stabilization of a composition based on PAEK, said process comprising:

incorporating by wet impregnation an aqueous solution comprising a stabilizing agent, wherein the stabilizing agent stabilizes with regard to the phenomena of thermal oxidation; and

stabilizing the composition, while the composition is at a temperature of greater than 350° C., to obtain the composition in molten state,

wherein the stabilizing agent is a water-soluble phosphate salt or a mixture of water-soluble phosphate salts.

9. The process as claimed in claim 8 , wherein the phosphate salt(s) is (are) chosen from at least one of the following salts: one (or more) phosphate salt(s) of ammonium, of sodium, of calcium, of zinc, of potassium, of aluminum, of magnesium, of zirconium, of barium, of lithium, or of rare earths.

10. The process as claimed in claim 8 , wherein the phosphate salt(s) is (are) chosen from at least one of the following compounds: anhydrous monosodium phosphate, monosodium phosphate monohydrate or monosodium phosphate dihydrate, anhydrous disodium phosphate, disodium phosphate dihydrate, disodium phosphate heptahydrate, disodium phosphate octahydrate or disodium phosphate dodecahydrate, anhydrous hexagonal trisodium phosphate, anhydrous cubic trisodium phosphate, trisodium phosphate hemihydrate, trisodium phosphate hexahydrate, trisodium phosphate octahydrate, trisodium phosphate dodecahydrate, or ammonium dihydrogen phosphate.

11. The process as claimed in claim 8 , wherein the phosphate salt is incorporated into the composition in proportions of between 10 ppm and 50,000 ppm.

12. The process as claimed in claim 11 , wherein the composition based on PAEK is a composition based on PEKK, and comprises, in addition to the PEKK, at least one of the following polymers: PEK, PEEKEK, PEEK, PEEKK, PEKEKK, PEEEK, PEDEK, with a content of less than 50% by weight of the composition.

13. The process as claimed in claim 8 , wherein the composition based on PAEK is a composition based on one of the following polymers: PEKK, PEEK, PEEKK, PEKEKK, PEEEK or PEDEK.

14. The process as claimed in claim 8 , wherein the composition based on PAEK is a poly(ether ketone ketone) (PEKK) composition.

Assignments (2)
CHANGE OF ADDRESS Recorded Jul 4, 2025
From: ARKEMA FRANCE
To: ARKEMA FRANCE
Reel/Frame 071814/0739 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 7, 2018
From: LE, GUILLAUME; BUSSI, PHILIPPE
To: ARKEMA FRANCE
Reel/Frame 045133/0553 →