IP Library Granted Patent US 10,826,076
Granted Patent B1
US 10,826,076 · App. 16/057,485 · Granted Nov 3, 2020

Patterned electrode catalyst

Inventors: Natalia Macauley (Los Alamos, NM); Siddharth Komini Babu (Santa Fe, NM); Rangachary Mukundan (Los Alamos, NM); Mahlon S. Wilson (Los Alamos, NM); Rodney L. Borup (Los Alamos, NM); Stephen Grot (New Castle, DE)
Assignee: Triad National Security, LLC
H01M4/926H01M4/8663H01M4/8807H01M8/1004
View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 10,826,076
App. No.
16/057,485
Granted
Nov 3, 2020
Kind
B1
Abstract

Disclosed herein are embodiments of a patterned electrode comprising regions of catalyst and segregating regions that separate the regions of catalyst. The segregating regions may be regions of non-catalytic material. The catalyst regions may correspond to the channels of a flow field. The electrode provides improved fuel cell performance, particularly at high current densities. The electrode may be for all suitable applications, such as in a membrane electrode assembly and/or a fuel cell. Also disclosed is a method for making the patterned electrode. The method may comprise using masks to apply the catalyst and non-catalyst material to a substrate.

Claims (40)

1. An electrode, comprising:

a flow field comprising a flow field channel that is defined by flow field walls;

a substrate layer in direct physical contact with the flow field; and

a plurality of catalyst regions separated by non-catalyst regions and in direct physical contact with the substrate layer, the plurality of catalyst regions being located such that multiple catalyst regions and multiple non-catalyst regions are arranged under the flow field channel, the catalyst regions comprising a catalyst material;

wherein the plurality of catalyst regions are located under the flow field channel and the flow field walls.

2. The electrode of claim 1 , wherein the non-catalyst regions are empty regions.

3. The electrode of claim 1 , wherein the catalyst material comprises platinum and a carbon support.

4. The electrode of claim 3 , wherein the carbon support is a high surface area carbon support.

5. The electrode of claim 1 , wherein the non-catalyst regions comprise non-catalyst material comprising carbon, an ionomer, or a combination thereof.

6. The electrode of claim 1 , wherein:

the catalyst regions each have a first width of from greater than zero to 2 mm;

the non-catalyst regions each have a second width of from greater than zero to 2 mm;

or a combination thereof.

7. A membrane electrode assembly, comprising

a cathode comprising the electrode of claim 1 ;

an anode; and

a membrane.

8. A fuel cell, comprising the electrode of claim 1 .

9. A stationary power device comprising the electrode of claim 1 .

10. The electrode of claim 1 , wherein the substrate layer comprises a gas dispersion layer and a microporous layer, and the flow field directly contact the gas dispersion layer and the plurality of catalyst regions directly contact the microporous layer.

11. An electrode, comprising:

a flow field comprising a flow field channel that is defined by flow field walls;

a substrate layer in direct physical contact with the flow field; and

a plurality of catalyst regions separated by non-catalyst regions and in direct physical contact with the substrate layer, the plurality of catalyst regions being located such that multiple catalyst regions and multiple non-catalyst regions are arranged under the flow field channel, the catalyst regions comprising a catalyst material;

wherein the plurality of catalyst regions are located under the flow field channel, but not under the flow field walls.

12. The electrode of claim 11 , wherein the catalyst material comprises platinum and a carbon support.

13. The electrode of claim 12 , wherein the carbon support is a high surface area carbon support.

14. The electrode of claim 11 , wherein the non-catalyst regions comprise non-catalyst material comprising carbon, an ionomer, or a combination thereof.

15. The electrode of claim 11 , wherein the non-catalyst regions are empty regions.

16. The electrode of claim 11 , wherein the substrate layer comprises a gas dispersion layer and a microporous layer, and the flow field directly contact the gas dispersion layer and the plurality of catalyst regions directly contact the microporous layer.

17. The electrode of claim 11 , wherein:

the catalyst regions each have a first width of from greater than zero to 2 mm;

the non-catalyst regions each have a second width of from greater than zero to 2 mm;

or a combination thereof.

18. A membrane electrode assembly, comprising

a cathode comprising the electrode of claim 11 ;

an anode; and

a membrane.

19. A fuel cell, comprising the electrode of claim 11 .

20. A stationary power device comprising the electrode of claim 11 .

Assignments (3)
CONFIRMATORY LICENSE Recorded May 18, 2020
From: TRIAD NATIONAL SECURITY, LLC
To: U.S. DEPARTMENT OF ENERGY
Reel/Frame 052686/0087 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 7, 2018
From: LOS ALAMOS NATIONAL SECURITY, LLC
To: TRIAD NATIONAL SECURITY, LLC
Reel/Frame 048007/0803 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 7, 2018
From: MACAULEY, NATALIA; BABU, SIDDHARTH KOMINI; MUKUNDAN, RANGACHARY; WILSON, MAHLON S.; BORUP, RODNEY L.
To: LOS ALAMOS NATIONAL SECURITY, LLC
Reel/Frame 046577/0073 →
Continuity (1)
Provisional Application 62542485 · Aug 8, 2017