IP Library Granted Patent US 11,059,719
Granted Patent B2
US 11,059,719 · App. 16/087,943 · Granted Jul 13, 2021

Process for producing hydrogen or syngas by methanol cracking

Inventors: Peter Mølgaard Mortensen (Roskilde, DK); Martin Østberg (Tune, DK); Poul Erik Højlund Nielsen (Fredensborg, DK)
Assignee: HALDOR TOPSØE A/S
C01B3/22B01J19/0013H05B6/22B01J2219/00139C01B2203/0277C01B2203/0855C01B2203/1076C01B2203/1082C01B2203/1223
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Quick Facts
Patent No.
US 11,059,719
App. No.
16/087,943
Granted
Jul 13, 2021
Kind
B2
Abstract

In a process for producing hydrogen or syngas by methanol cracking, whereby methanol is catalytically decomposed into hydrogen and carbon monoxide in an endothermal reaction, said reaction takes place in a reactor with direct inductive heating in the reaction zone. The heating is obtained by passing an alternating current through a metallic coil located inside the reactor or by using induction heated catalyzed hardware in the shape of a ferromagnetic structure, which is coated with an oxide impregnated with the catalytically active phase.

Claims (26)

1. A process for producing hydrogen/carbon dioxide or syngas by methanol cracking, whereby methanol is catalytically decomposed into hydrogen and carbon monoxide in a first endothermal reaction:

CH 3 OH→CO+2H 2

and/or into hydrogen and carbon dioxide in a second endothermic reaction:

CH 3 OH+H 2 O↔3H 2 +CO 2

said reactions taking place in a reactor with a reaction zone, the reaction zone comprising a catalyst in the form of induction heated catalyzed hardware, with direct inductive heating in the reaction zone,

wherein the direct inductive heating is obtained using the induction heated catalyzed hardware, wherein the induction heated catalyzed hardware is a ferromagnetic structure, which is coated with a non-catalyst oxide impregnated with a catalytically active phase.

2. Process according to claim 1 , wherein the direct inductive heating is obtained by passing an alternating current through a metallic coil located inside the reactor.

3. Process according to claim 2 , wherein the metallic coil is copper wire.

4. Process according to claim 3 , wherein the metallic coil is in electrical contact with the catalyst.

5. Process according to claim 2 , wherein the direct inductive heating is obtained by an alternating magnetic field.

6. Process according to claim 1 , wherein the catalyst comprises Cu.

7. Process according to claim 1 , wherein the ferromagnetic structure is composed of metals of Fe—Cr or Al—Ni—Co alloys.

8. Process according to claim 1 , wherein the oxide coated onto the ferromagnetic structure is an oxide comprising at least one of Al, Zr, and Ce.

9. Process according to claim 8 , wherein a surface of the oxide is impregnated with a catalytic phase suitable for methanol cracking.

10. Process according to claim 9 , wherein the catalytic phase comprises Cu.

11. Process according to claim 1 , wherein the direct inductive heating takes place by both ferromagnetic/hysteresis heating and ohmic/eddy current heating.

12. Process according to claim 1 , wherein the catalytically active phase is ferromagnetic.

13. Process according to claim 1 , wherein the methanol is gaseous methanol.

14. A process for producing hydrogen/carbon dioxide or syngas by methanol cracking, whereby methanol is catalytically decomposed into hydrogen and carbon monoxide in a first endothermal reaction:

CH 3 OH→CO+2H 2

and/or into hydrogen and carbon dioxide in a second endothermic reaction:

CH 3 OH+H 2 O↔3H 2 +CO 2

said reactions taking place in a reactor with a reaction zone, the reaction zone comprising a catalyst in the form of induction heated catalyzed hardware, with direct inductive heating in the reaction zone,

wherein the direct inductive heating is obtained using the induction heated catalyzed hardware, wherein the induction heated catalyzed hardware is a ferromagnetic support structure.

15. Process according to claim 14 , wherein the methanol is gaseous methanol.

16. Process according to claim 15 , wherein the induction heated catalyzed hardware is a ferromagnetic structure, which is coated with a non-catalyst oxide impregnated with a catalytically active phase.

Assignments (2)
CHANGE OF NAME Recorded Dec 19, 2023
From: HALDOR TOPSØE A/S
To: TOPSOE A/S
Reel/Frame 066076/0685 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 24, 2018
From: MORTENSEN, PETER MØLGAARD; ØSTBERG, MARTIN; HØJLUND NIELSEN, POUL ERIK
To: HALDOR TOPSØE A/S
Reel/Frame 046953/0733 →
Priority Claims (1)
DK PA 2016 00242 · Apr 26, 2016 · national
Continuity (1)
Related Publication 20190112187A1 · Apr 18, 2019