IP Library Granted Patent US 11,319,284
Granted Patent B2
US 11,319,284 · App. 16/096,493 · Granted May 3, 2022

Process for the synthesis of nitriles

Inventors: Poul Erik Højlund Nielsen (Fredensborg, DK); Burcin Temel McKenna (Hellerup, DK); John Bøgild Hansen (Humlebæk, DK); Rasmus Munksgård Nielsen (Måløv, DK)
Assignee: HALDOR TOPSØE A/S
C07C253/18B01J8/0285B01J23/14B01J23/75B01J35/0033C07C253/00H05B6/108B01J2208/00433B01J2208/00469C07C255/03
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Quick Facts
Patent No.
US 11,319,284
App. No.
16/096,493
Granted
May 3, 2022
Kind
B2
Abstract

In a process for the synthesis of a nitrile by endothermic catalyzed reaction of ammonia with a hydrocarbon using heating obtained by passing an alternating current through a metallic coil, the endothermic reaction between ammonia and the hydrocarbon takes place in a reactor with direct inductive heating in the reaction zone. The heating is extremely fast, which makes the reaction practically instantaneous.

Claims (20)

1. A process for the synthesis of a nitrile by catalyzed reaction of ammonia with a hydrocarbon using heating obtained by passing an alternating current through a metallic coil in a synthesis reactor with a catalyst,

wherein the endothermic reaction between ammonia and the hydrocarbon takes place in the synthesis reactor with direct inductive heating in a reaction zone,

wherein the coil is mounted within the synthesis reactor, and all of the catalyst is placed inside the coil.

2. A process for the synthesis of a nitrile by catalyzed reaction of ammonia with a hydrocarbon using heating obtained by passing an alternating current through a metallic coil in a synthesis reactor with a catalyst,

wherein the endothermic reaction between ammonia and the hydrocarbon takes place in the synthesis reactor with direct inductive heating in a reaction zone,

wherein the coil is mounted within the synthesis reactor, and the catalyst is placed inside the coil,

wherein the coil is made of Fe—Cr—Al alloy wire.

3. The process according to claim 1 , wherein the inductive heating is carried out using an induction heater which is a ferromagnetic metal structure provided with a suitable coating, and wherein the heating is generated by magnetic hysteresis losses.

4. The process according to claim 3 , wherein the metal structure is a metal selected from Fe—Cr and Al—Ni—Co alloys.

5. The process according to claim 4 , wherein the metal structure is coated with a porous oxide surface impregnated with a catalytic phase.

6. The process according to claim 5 , wherein the catalytic phase contains a catalyst based on Co or Sn.

7. The process according to claim 1 , wherein the hydrocarbon is methane, ethane, propane, iso-butane or an olefin.

8. The process according to claim 3 , wherein the induction heater comprises a ferromagnetic catalyst.

9. The process according to claim 8 , wherein the catalyst is diluted with a magnetic material.

10. The process according to claim 1 , wherein the coil is arranged to have a direct electrical contact to the catalyst.

11. The process according to claim 10 , wherein the coil is not subject to electrical isolation.

12. The process according to claim 1 , wherein the coil is a wire comprising at least one selected from copper, constantan, an iron-chromium-aluminum alloy, and a copper-manganese-nickel alloy.

13. A process for the synthesis of a nitrile by catalyzed reaction of ammonia with a hydrocarbon using heating obtained by passing an alternating current through a metallic coil in a synthesis reactor with a catalyst,

wherein the endothermic reaction between ammonia and the hydrocarbon takes place in the synthesis reactor with direct inductive heating in a reaction zone,

wherein the coil is a wire comprising at least one selected from copper, constantan, an iron-chromium-aluminum alloy, and a copper-manganese-nickel alloy.

Assignments (3)
CHANGE OF NAME Recorded Dec 19, 2023
From: HALDOR TOPSØE A/S
To: TOPSOE A/S
Reel/Frame 066076/0685 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 6, 2019
From: HØJLUND NIELSEN, POUL ERIK; TEMEL MCKENNA, BURCIN; HANSEN, JOHN BØGILD; NIELSEN, RASMUS MUNKSGÅRD
To: HALDOR TOPSØE A/S
Reel/Frame 048517/0085 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 25, 2018
From: HOJLUND NIELSEN, POUL ERIK; TEMEL MCKENNA, BURCIN; HANSEN, JOHN BOGILD; NIELSEN, RASMUS MUNKSGÅRD
To: HALDOR TOPSØE A/S
Reel/Frame 047312/0625 →
Priority Claims (1)
DK PA 2016 00246 · Apr 26, 2016 · national
Continuity (1)
Related Publication 20190144376A1 · May 16, 2019