IP Library Granted Patent US 11,098,190
Granted Patent B2
US 11,098,190 · App. 16/097,426 · Granted Aug 24, 2021

Polybutylene terephthalate resin composition and molded article

Inventors: Souki Yoshida (Hiratsuka, JP); Yasushi Yamanaka (Hiratsuka, JP)
Assignee: Mitsubishi Engineering-Plastics Corporation
C08L67/02C08J5/00C08L23/08C08L63/00H01R13/533C08L2201/02C08L2203/20C08L2205/025C08L2205/035C08L2205/06H01B3/40H01R2201/26
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Quick Facts
Patent No.
US 11,098,190
App. No.
16/097,426
Granted
Aug 24, 2021
Kind
B2
Abstract

Provided is a polybutylene terephthalate resin composition containing, with respect to 100 parts by mass of (A) a polybutylene terephthalate resin, (B) a total of 30 to 60 parts by mass of at least two different brominated flame retardants selected from the group consisting of a brominated epoxy compound, a brominated polycarbonate compound and a brominated polystyrene compound, (C) 5 to 15 parts by mass of an antimony compound, (D) 5 to 30 parts by mass of an elastomer, and (E) 0.5 to 3 parts by mass of a mold-release agent.

Claims (21)

1. A polybutylene terephthalate resin composition, comprising:

(A) 100 parts by mass of a polybutylene terephthalate resin,

(B) a total of 30 to 60 parts by mass of at least two different brominated flame retardants selected from the group consisting of a brominated epoxy compound, a brominated polycarbonate compound and a brominated polystyrene compound,

(C) 5 to 15 parts by mass of an antimony compound,

(D) 5 to 30 parts by mass of an elastomer, and

(E) 0.5 to 3 parts by mass of a mold-release agent,

wherein the polybutylene terephthalate resin composition has a crystallization temperature of from 175 to 193° C.

2. The polybutylene terephthalate resin composition of claim 1 , wherein the at least two different brominated flame retardants (B) comprise:

a brominated flame retardant (B1), which is selected from among a brominated epoxy compound and a brominated polycarbonate compound and which has a weight average molecular weight of 1000 to 8000, and

a brominated flame retardant (B2), which is selected from among a brominated epoxy compound and a brominated polystyrene compound and which has a weight average molecular weight of more than 8000 to 70000.

3. The polybutylene terephthalate resin composition of claim 1 , wherein the polybutylene terephthalate resin composition has a crystallization temperature of from 180 to 193° C.

4. The polybutylene terephthalate resin composition of claim 1 , wherein the at least two different brominated flame retardants (B) are each independently a brominated epoxy compound.

5. The polybutylene terephthalate resin composition of claim 1 , comprising a brominated epoxy compound, wherein the brominated epoxy compound is terminally capped by tribromophenol.

6. The polybutylene terephthalate resin composition of claim 2 , wherein a mass ratio (B1)/(B2) of the flame retardant (B1) and the flame retardant (B2) is 90/10 to 30/70.

7. The polybutylene terephthalate resin composition of claim 1 , wherein the elastomer (D) is an ethylenic elastomer.

8. The polybutylene terephthalate resin composition of claim 7 , wherein the ethylenic elastomer is an ethylene-alkyl acrylate ester-glycidyl methacrylate copolymer.

9. The polybutylene terephthalate resin composition of claim 1 , wherein the mold-release agent (E) is a montanic acid ester mold-release agent.

10. The polybutylene terephthalate resin composition of claim 1 , wherein a moisture content of the polybutylene terephthalate resin composition is 500 ppm or less.

11. A molded article, comprising the polybutylene terephthalate resin composition of claim 1 .

12. A vehicular electrical component, comprising the molded article of claim 11 .

13. The polybutylene terephthalate resin composition of claim 1 , which is free of a polycarbonate resin.

Assignments (2)
CONFIRMATORY ASSIGNMENT Recorded Dec 5, 2023
From: MITSUBISHI ENGINEERING-PLASTICS CORPORATION
To: MITSUBISHI CHEMICAL CORPORATION
Reel/Frame 065775/0613 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 29, 2018
From: YOSHIDA, SOUKI; YAMANAKA, YASUSHI
To: MITSUBISHI ENGINEERING-PLASTICS CORPORATION
Reel/Frame 047340/0191 →