IP Library Granted Patent US 10,961,418
Granted Patent B2
US 10,961,418 · App. 16/099,817 · Granted Mar 30, 2021

Use of block copolymers in adhesives

Inventors: Nicolai Kolb (Recklinghausen, DE); Gabriele Brenner (Dülmen, DE); Patrick Glöckner (Haltern am See, DE); Bernhard Schleimer (Marl, DE)
Assignee: Evonik Operations GmbH
C09J153/00C08G18/4063C08G18/694C08G18/698C08G18/7671C08G63/08C08G81/027C09J175/14C08G2170/20C08K5/0025
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Quick Facts
Patent No.
US 10,961,418
App. No.
16/099,817
Granted
Mar 30, 2021
Kind
B2
Abstract

The present invention relates to the use of block copolymers produced from OH-functionalized polyolefins and polyesters in adhesives or sealants and to adhesives or sealants containing said block co-polymers.

Claims (33)

1. An adhesive composition comprising block copolymers formed from OH-, or COOH-terminated polybutadiene and polyesters in adhesives or sealants, wherein the block copolymer is B(A) x block systems

with A=polyester,

with B═OH-, or COOH-terminated polybutadiene and

with x≥1 wherein the adhesive composition contains at least one further polyol component, and

wherein the functionality of the OH-terminated polybutadienes used is from 1 to 5.

2. The adhesive composition according to claim 1 , wherein the OH— or COOH functionalized terminated polybutadienes are partially or completely hydrogenated, and

wherein the functionality of the OH-terminated polybutadienes used is from 1.5 to 3.5.

3. The adhesive composition according to claim 2 , wherein the block copolymers are based on polyesters made from a lactone.

4. The adhesive composition according to claim 2 , wherein the block copolymers are based on polyesters made from a lactide.

5. The adhesive composition according to claim 1 , wherein

the block copolymer is B(A) x block systems are B′-(-Y-A′-X) x systems

with A′=polyester radical, B′═OH—, or COOH-terminated polybutadiene,

Y═O, or COO groups,

X═OH or COOH terminal groups and x≥1, and

wherein the functionality of the OH-terminated polybutadienes used is from 2 to 3.

6. The adhesive composition according to claim 1 , wherein the block copolymers are based on polyesters made from a lactone.

7. The adhesive composition according to claim 1 , wherein the block copolymers are based on polyesters made from a lactide.

8. The adhesive composition according to claim 1 , wherein

the block copolymer is B(A) x block systems are B′-(-Y-A′-X) x systems

with A′=polyester radical,

B′═OH-, or COOH-terminated polybutadiene,

Y═O, or COO groups,

X═OH or COOH terminal groups and x>1 and

the block copolymers are based on polyesters made from a lactone and/or a lactide.

9. The adhesive composition according to claim 1 , wherein the OH- or COOH-functionalized terminated polybutadienes are OH-functionalized terminated polybutadienes having a functionality of the OH-terminated polybutadienes from 1.5 to 3.5.

10. The adhesive composition according to claim 1 , wherein the OH- or COON-functionalized terminated polybutadienes are OH-functionalized terminated polybutadienes having a functionality of the OH-terminated polybutadienes from 2 to 3.

11. An adhesive composition comprising block copolymers formed from OH-, or COOH-terminated polybutadiene and polyesters in adhesives or sealants, wherein the block copolymer is B(A) x block systems

with A=polyester,

with B═OH—, or COOH-terminated polybutadiene comprising the 1,3-butadiene-derived monomer units

wherein the proportion of (I) in the entirety of the 1,3-butadiene-derived monomer units present in the polybutadiene is 10 to 60 mole percent, and wherein the sum total of the proportions of (II) and (III) in the entirety of the 1,3-butadiene-derived monomer units present in the polybutadiene is 40 to 90 mole percent, and

with x≥1 wherein the adhesive composition contains at least one further polyol component.

12. The adhesive composition according to claim 11 , wherein the OH- or COOH-functionalized terminated polybutadienes are OH-functionalized terminated polybutadienes having a functionality of the OH-terminated polybutadienes from 1.5 to 3.5.

13. The adhesive composition according to claim 11 , wherein the OH- or COOH-functionalized terminated polybutadienes are OH-functionalized terminated polybutadienes having a functionality of the OH-terminated polybutadienes from 2 to 3.

Assignments (2)
CHANGE OF NAME Recorded Dec 27, 2019
From: EVONIK DEGUSSA GMBH
To: EVONIK OPERATIONS GMBH
Reel/Frame 051428/0710 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 6, 2019
From: KOLB, NICOLAI; SCHLEIMER, BERNHARD; GLÖCKNER, PATRICK; BRENNER, GABRIELE
To: EVONIK DEGUSSA GMBH
Reel/Frame 049087/0428 →
Priority Claims (1)
EP 16168681 · May 9, 2016 · regional
Continuity (1)
Related Publication 20190112511A1 · Apr 18, 2019
Cited By (1)
US 12,534,564