IP Library Granted Patent US 10,829,846
Granted Patent B2
US 10,829,846 · App. 16/156,612 · Granted Nov 10, 2020

Process for producing nanostructured metal substrates for use in Surface Enhanced Raman Spectroscopy or similar applications

Inventors: Lloyd Ploof (Lee Center, NY); Jody Ray McRedmond (Ilion, NY); Thomas Joseph Basile (Clinton, NY)
C23C8/42C23C8/02C23C8/80C23C28/32C23C28/345
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Quick Facts
Patent No.
US 10,829,846
App. No.
16/156,612
Granted
Nov 10, 2020
Kind
B2
Abstract

A framework of copper oxide dendrites is formed on a copper substrate, and these are then coated or plated with silver, gold, or an equivalent metal to create metal-coated dendrites with nano-structures, favorably in range of 50 to 200 nanometers. The framework of metal-coated dendrites are well suited for use in surface-enhanced Raman spectroscopy and other practical applications.

Claims (12)

1. Process for forming a nano-scale substrate suitable for use in Surface Enhanced Raman Spectroscopy (SERS) and/or other similar Raman spectroscopy applications, comprising:

starting with a substrate having thereon a layer of copper;

subjecting the copper layer to oxidation in a process bath to form a layer of copper oxide dendrites thereon having sizes on the order of up to 100 μm and of one μm;

cleaning the substrate and the copper oxide dendrites;

depositing on the copper oxide dendrites a coating of a noble metal; and

cleaning and rinsing the noble-metal coating to render the substrate and coated dendrites suitable for SERS and/or other suitable Raman spectroscopy applications.

2. The process of claim 1 wherein said step of starting with a layer of copper is followed by a step of chemically polishing said layer of copper.

3. The process of claim 1 wherein step of subjecting the copper layer to oxidation in a process bath includes employing an aqueous reagent bath with sulfur compounds and oxidizers.

4. The process of claim 1 wherein said step of subjecting the copper layer to oxidation in a process bath results in dendrites in a plurality of sizes from less than one micron up to a hundred microns.

5. The process of claim 1 wherein said subjecting the copper layer to oxidation in a process bath is carried out at an elevated temperature of about 90° C.

6. The process of claim 1 wherein said noble metal is selected from the group consisting of Ag, Au, Pa and Pt.

7. The process of claim 1 wherein said noble metal consists of one or more from the group consisting of Ag, Au, Sn, Ni, Cu, Pt, Pa, Rh and Zn.

Assignments (2)
SECURITY INTEREST Recorded Nov 13, 2024
From: SQUARE ONE COATING SYSTEMS LLC; SELAS HEAT TECHNOLOGY COMPANY LLC
To: PNC BANK, NATIONAL ASSOCIATION
Reel/Frame 069242/0715 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 14, 2023
From: PLOOF, LLOYD; MCREDMOND, JODY; BASILE, THOMAS
To: SQUARE ONE COATING SYSTEMS, LLC
Reel/Frame 065872/0707 →
Continuity (2)
Provisional Application 62723635 · Aug 28, 2018
Related Publication 20200071812A1 · Mar 5, 2020