IP Library Granted Patent US 10,752,735
Granted Patent B2
US 10,752,735 · App. 16/190,293 · Granted Aug 25, 2020

Mixtures of cyclic branched siloxanes of the D/T type and conversion products thereof

Inventors: Wilfried Knott (Essen, DE); Horst Dudzik (Essen, DE)
Assignee: Evonik Operations GmbH
C08G77/06C07F7/21C08G77/045C08G77/10C08G77/14C08L83/04C08G77/12C08G77/70
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Quick Facts
Patent No.
US 10,752,735
App. No.
16/190,293
Granted
Aug 25, 2020
Kind
B2
Abstract

Mixtures of cyclic branched siloxanes having exclusively D and T units and having no functional groups, with the proviso that the cumulative proportion of the D and T units having Si-alkoxy and/or SiOH groups that are present in the siloxane matrix, determinable by 29 Si NMR spectroscopy, is ≤2 mole percent, are described, as are branched organo-modified siloxanes obtainable therefrom.

Claims (10)

1. A mixture of cyclic branched siloxanes having exclusively D and T units and having no functional groups, wherein the cumulative proportion of the D and T units having Si-alkoxy and/or SiOH groups that are present in the siloxane matrix is determinable by 29 Si NMR spectroscopy, is ≤2 mole percent, based on the totality of silicon detected by spectroscopy.

2. The mixture of cyclic branched siloxanes having exclusively D and T units according to claim 1 , wherein the branching T unit derives from alkyltrialkoxysilanes and/or phenyltrialkoxysilanes.

3. The mixture of cyclic branched siloxanes having exclusively D and T units according to claim 2 , wherein the molar mass ratio of the mixture Mw/Mn is in the range of 2<Mw/Mn<50.

4. The mixture of cyclic branched siloxanes having exclusively D and T units according to claim 1 , wherein the branching T unit derives from methyltriethoxysilane.

5. The mixture of cyclic branched siloxanes having exclusively D and T units according to claim 4 , wherein the molar mass ratio of the mixture Mw/Mn is in the range of 2<Mw/Mn<50.

6. The mixture of cyclic branched siloxanes having exclusively D and T units according to claim 1 , wherein the ratio of D to T units is between 6:1 and 4:1.

7. The mixture of cyclic branched siloxanes having exclusively D and T units according to claim 6 , wherein the molar mass ratio of the mixture Mw/Mn is in the range of 2<Mw/Mn<50.

8. A mixture of cyclic branched siloxanes having exclusively D and T units and having no functional groups, wherein the cumulative proportion of the D and T units having Si-alkoxy and/or SiOH groups that are present in the siloxane matrix; determinable by 29 Si NMR spectroscopy, is ≤2 mole percent, wherein the ratio of D to T units is between 10:1 and 3:1.

9. The mixture of cyclic branched siloxanes having exclusively D and T units according to claim 8 , wherein the molar mass ratio of the mixture Mw/Mn is in the range of 2<Mw/Mn<50.

10. The mixture of cyclic branched siloxanes having exclusively D and T units according to claim 8 , wherein the molar mass ratio of the mixture Mw/Mn is in the range of 2<Mw/Mn<50.

Assignments (1)
CHANGE OF NAME Recorded Dec 27, 2019
From: EVONIK DEGUSSA GMBH
To: EVONIK OPERATIONS GMBH
Reel/Frame 051428/0710 →
Priority Claims (2)
EP 16198809 · Nov 15, 2016 · regional
EP 17156421 · Feb 16, 2017 · regional
Continuity (2)
Division 15719775 · Sep 29, 2017
Related Publication 20190100625A1 · Apr 4, 2019
Cited By (3)
US 12,460,081 US 12,577,351 US 12,674,030