IP Library Granted Patent US 11,597,664
Granted Patent B2
US 11,597,664 · App. 16/194,559 · Granted Mar 7, 2023

Disinfection method for water and wastewater

Inventors: Philip Block (Garnet Valley, PA); Weidong An (Williamsville, PA); Angela Thompson (East Amherst, NY); Coryn Mittiga (Tonawanda, NY)
Assignee: Evonik Operations GmbH
C02F1/722C02F1/505C02F1/68C02F1/725C02F1/688C02F2103/001C02F2103/02C02F2303/04
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Quick Facts
Patent No.
US 11,597,664
App. No.
16/194,559
Granted
Mar 7, 2023
Kind
B2
Abstract

Provided herein are methods and compositions for water disinfection. The methods and compositions, which can include a peracid and a source of copper ions, are useful for treatment of water contaminated with recalcitrant microbes.

Claims (28)

1. A method of reducing the concentration of microorganisms in water by the combined effect of one or more peracids and one or more water-soluble copper-containing salts, wherein the method consists of:

a) adding the one or more peracids (or an aqueous solution of the one or more peracids) and the one or more water-soluble copper-containing salts to the water to a final concentration of 0.1 ppm to 20 ppm peracid and 0.01 to 10 ppm copper ions; wherein:

i) the water is selected from the group consisting of: sewage, industrial wastewater, municipal wastewater, combined sewer overflow, process water, rain water, flood water, and storm runoff water; and

ii) the one or more peracids and the one or more water-soluble copper-containing salts are added together in a single solution;

b) maintaining contact between the water, the one or more peracids and the copper ions for a time sufficient to reduce the concentration of microorganisms in the water.

2. The method of claim 1 , wherein, in step b), contact between the water, the one or more peracids and the copper ions is maintained for 5-180 minutes.

3. The method of claim 1 , wherein, in step b), contact between the water, the one or more peracids and the copper ions is maintained for 5-90 minutes.

4. The method of claim 1 , wherein, in step b), contact between the water, the one or more peracids and the copper ions is maintained for 5-45 minutes.

5. The method of claim 1 , wherein, in step b), contact between the water, the one or more peracids and the copper ions is maintained for 5-20 minutes.

6. The method of claim 1 , wherein, in step b), contact between the water, the one or more peracids and the copper ions is maintained for 5-10 minutes.

7. The method of claim 1 , wherein the microorganism is a bacterium, a bacteriophage, a virus, a fungus, a protozoa, a parasite or a microbial indicator organism.

8. The method of claim 1 , wherein one of the peracids is peracetic acid or performic acid or a combination thereof.

9. A method of reducing the concentration of microorganisms in water by the combined effect of one or more peracids and one or more water-soluble copper-containing salts, wherein the method consists of:

a) adding the one or more peracids and the one or more water-soluble copper-containing salts to the water to a final concentration of 0.5 ppm to 50 ppm peracid and a concentration of copper ions effective to increase antimicrobial activity of the peracid; wherein:

i) the water is selected from the group consisting of: sewage, industrial wastewater, municipal wastewater, combined sewer overflow, process water, rain water, flood water, and storm runoff water; and

ii) the one or more peracids and the one or more water-soluble copper-containing salts are added together in a single solution;

b) maintaining contact between the water, the one or more peracids and the copper ions for a time sufficient to reduce the concentration of microorganisms in the water.

10. The method of claim 9 , wherein the final concentration of the one or more peracids in the water being disinfected is from about 0.5 ppm to about 5 ppm.

11. The method of claim 10 , wherein the final concentration of the copper ions in the water being disinfected is from about 0.05 ppm to about 5 ppm.

12. The method of claim 11 , wherein one of the peracids is peracetic acid or performic acid and one of the water soluble copper-containing salts is copper sulfate, copper chloride, or copper nitrate.

13. The method of claim 12 , wherein the microorganism is a bacterium, a bacteriophage, a virus, a fungus, a protozoa, a parasite or a microbial indicator organism.

14. The method of claim 13 , wherein the method results in at least a three log reduction in the number of colony forming units present in a sample of the water.

15. The method of claim 9 , wherein a single type of peracid and a single type of copper-containing salt is added to the water.

16. The method of claim 15 , wherein the microorganism is a bacterium, a bacteriophage, a virus, a fungus, a protozoa, a parasite or a microbial indicator organism.

17. The method of claim 16 , wherein the peracid is peracetic acid or performic acid and the water soluble copper-containing salt is copper sulfate, copper chloride, or copper nitrate.

18. The method of claim 16 , wherein, in step b), contact between the water, the peracid and the copper containing ions is maintained for 5-180 minutes.

19. The method of claim 16 , wherein, in step b), contact between the water, the peracid and the copper containing ions is maintained for 5-45 minutes.

20. The method of claim 16 , wherein, in step b), contact between the water, the peracid and the copper containing ions is maintained for 5-10 minutes.

Assignments (4)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 17, 2021
From: PEROXYCHEM LLC
To: EVONIK OPERATIONS GMBH
Reel/Frame 055627/0087 →
RELEASE OF SECURITY INTEREST IN PATENTS RECORDED AT R/F 050605/0305 Recorded Feb 3, 2020
From: BARCLAYS BANK PLC, AS ADMINISTRATIVE AGENT
To: PEROXYCHEM LLC
Reel/Frame 051777/0957 →
SECURITY INTEREST Recorded Oct 2, 2019
From: PEROXYCHEM LLC
To: BARCLAYS BANK PLC, AS ADMINISTRATIVE AGENT
Reel/Frame 050605/0305 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 19, 2018
From: BLOCK, PHILIP; AN, WEIDONG; THOMPSON, ANGELA; MITTIGA, CORYN
To: PEROXYCHEM LLC
Reel/Frame 047538/0029 →
Continuity (2)
Provisional Application 62588514 · Nov 20, 2017
Related Publication 20190152817A1 · May 23, 2019