IP Library Granted Patent US 11,326,017
Granted Patent B2
US 11,326,017 · App. 16/410,082 · Granted May 10, 2022

Tin-free catalysis of silane-functional polyurethane crosslinkers

Inventors: Tobias Unkelhäußer (Lüdinghausen, DE); Emmanouil Spyrou (Schermbeck, DE); Stephanie Hösl (Dorsten, DE); Dennis Menne (Haltern am See, DE); Guido Streukens (Wuppertal, DE)
Assignee: Evonik Operations GmbH
C08G18/1875C08G18/10C08G18/161C08G18/168C08G18/1816C08G18/1858C08G18/289C08G18/307C08G18/3206C08G18/4825C08G18/58C08G18/6229C08G18/6484C08G18/6607C08G18/718C08G18/758C08G18/792C08G77/04C08K3/013C08K5/5419C09D175/04C09D183/04C08K2201/001
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Quick Facts
Patent No.
US 11,326,017
App. No.
16/410,082
Granted
May 10, 2022
Kind
B2
Abstract

The present invention relates to a composition at least comprising A) an adduct of isocyanatosilanes with hydroxy-functional compounds and B) a tin-free catalyst, and also to a coating composition comprising at least the composition and to the use of the coating composition.

Claims (23)

1. An aminosilane-free composition comprising

A) an adduct of an isocyanatosilane with a hydroxy-functional compound wherein the adduct A) comprises <0.05% free NCO groups,

B) a tin-free catalyst selected from the group consisting of alkylammonium halides, wherein the hydroxy-functional compound is selected from the group consisting of monoalcohols, diols, triols, tetrols and hydroxyl group-containing polymers having an OH number of from 10 to 500 mg KOH/gram and a number-average molar mass of from 250 to 6000 g/mol, and

C) a polyether siloxane copolymer,

wherein the hydroxyl group-containing polymers are selected from the group consisting of polyesters, polyethers, polyacrylates, polycarbonates, epoxy resins, FEVE (fluoroethylene vinyl ether), alkyds and polyurethanes, wherein the polyurethanes consist of polyols and diisocyanate monomers; and

wherein the amount of component A) is from 40 to 99% by weight and the amount of component B) is from 0.01 to 3% by weight, based in each case on the total composition.

2. The aminosilane-free composition according to claim 1 , wherein the isocyanatosilane is selected from the group consisting of 3-isocyanatopropyltrimethoxysilane, 3-isocyanatopropyltriethoxysilane, 3-isocyanatopropyldimethoxyethoxysilane and/or 3-isocyanatopropyldiethoxymethoxysilane.

3. The aminosilane-free composition according to claim 2 , wherein the ratio of OH groups of the hydroxy-functional compounds to NCO groups of the isocyanatosilanes is from 1 to 1.

4. The aminosilane-free composition according to claim 1 , wherein the tin-free catalyst B) is selected from the group consisting of alkylammonium fluorides.

5. The aminosilane-free composition according to claim 1 , wherein the tin-free catalyst B) is tetramethylammonium fluoride, tetrapropylammonium fluoride, tetraethylammonium fluoride, tetrabutylammonium fluoride or a mixture thereof.

6. A one-component (1K) coating composition comprising at least the aminosilane-free composition according to claim 1 .

7. A one-component coating composition according to claim 6 which comprises at least one auxiliary and/or additive and/or at least one solvent.

8. The one-component coating composition according to claim 7 , wherein the at least one auxiliary and/or additive is selected from the group consisting of stabilizers, light stabilizers, pigments, levelling agents or rheological assistants, microgels, fumed silicon dioxide, inorganic or organic color pigments and/or effect pigments or mixtures of two or more thereof.

9. A composite comprising the one-component coating composition according to claim 6 wherein the composite comprises wood, plastic, glass or metal.

10. A coating comprising the one-component coating composition according to claim 6 .

11. The aminosilane-free composition according to claim 2 , wherein the tin-free catalyst B) is an alkylammonium fluoride.

12. A two-component (2K) coating composition comprising at least the aminosilane-free composition according to claim 1 .

13. A two-component coating composition according to claim 12 which comprises at least one auxiliary and/or additive and/or at least one solvent.

14. The two-component coating composition according to claim 13 , wherein the at least one auxiliary and/or additive is selected from the group consisting of stabilizers, light stabilizers, levelling agents or rheological assistants, microgels, fumed silicon dioxide, inorganic or organic color pigments and/or effect pigments or mixtures of two or more thereof.

15. A composite comprising the two-component coating composition according to claim 12 wherein the composite comprises wood, plastic, glass or metal.

16. A coating comprising the two-component coating composition according to claim 12 .

17. The aminosilane-free composition according to claim 1 , wherein the hydroxy-functional compound is selected from the group consisting of a diol, triol and tetrol.

18. The aminosilane-free composition according to claim 1 , wherein the hydroxy-functional compound is a diol or a triol.

Assignments (2)
CHANGE OF NAME Recorded Dec 27, 2019
From: EVONIK DEGUSSA GMBH
To: EVONIK OPERATIONS GMBH
Reel/Frame 051428/0710 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 16, 2019
From: UNKELHÄUSSER, TOBIAS; SPYROU, EMMANOUIL; HÖSL, STEPHANIE; MENNE, DENNIS; STREUKENS, GUIDO
To: EVONIK DEGUSSA GMBH
Reel/Frame 050728/0501 →
Priority Claims (1)
EP 18193333 · Sep 10, 2018 · regional
Continuity (1)
Related Publication 20200079894A1 · Mar 12, 2020