IP Library Granted Patent US 11,229,899
Granted Patent B2
US 11,229,899 · App. 16/467,635 · Granted Jan 25, 2022

Catalyst composition

Inventors: Hong-Xin Li (Lansdale, PA); Richard Berend Mauer (Amsterdam, NL); Gisela Sabater Pujadas (Amsterdam, NL)
Assignee: SHELL OIL COMPANY
B01J29/80B01J23/22B01J23/26B01J23/28B01J23/30B01J23/34B01J23/36B01J23/42B01J23/44B01J23/464B01J29/18B01J29/185B01J29/22B01J29/24B01J29/26B01J29/40B01J29/405B01J29/44B01J29/46B01J29/48B01J35/002B01J35/0066B01J35/023B01J37/0009B01J37/0018B01J37/0201B01J37/04B01J37/088C01B39/023C07C6/126B01J2229/18B01J2229/186B01J2229/20B01J2229/42C01P2004/64C07C2523/42C07C2529/18C07C2529/22C07C2529/24C07C2529/26C07C2529/40C07C2529/44C07C2529/46C07C2529/48C07C2529/80Y02P20/52
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Quick Facts
Patent No.
US 11,229,899
App. No.
16/467,635
Granted
Jan 25, 2022
Kind
B2
Abstract

A catalyst composition comprising (a) carrier comprising (i) 5 to 95 wt % mordenite type zeolite having a mean crystallite length parallel to the direction of the 12-ring channels of 60 nm or less and a mesopore volume of at least 0.10 cc/gram, (ii) 5 to 95 wt % ZSM-5 type zeolite; and (iii) 10 to 60 wt % inorganic binder; and (b) 0.001 to 10 wt % of one or more catalytically active metals, wherein the inorganic binder comprises titania, its preparation and its use in alkylaromatic conversion.

Claims (15)

1. A catalyst composition useful in the transalkylation and dealkylation of alkyaromatics, wherein the catalyst composition comprises:

(a) a carrier consisting essentially of: (i) mordenite type zeolite having a mean crystallite length parallel to the direction of the 12-ring channels of from 10 to 60 nm and a mesopore volume of at least 0.10 cc/gram in an amount in the range of from 20 to 90 wt %, based on total weight of carrier, (ii) ZSM-5 type zeolite having a silica-to-alumina molar ratio in the range of from 10 to 50 and present in an amount of from 10 to 70 wt %, based on total weight of carrier, wherein the ZSM-5 type zeolite has a number average particle size in the range of from 20 to 500 nm; and (iii) titania as a binder in an amount in the range of from 10 to 60 wt %, based on total weight of carrier; and

(b) of from 0.001 to 10 wt % of one or more catalytically active metals selected from the group consisting of tin, tungsten, vanadium, molybdenum, rhenium, nickel, cobalt, chromium, manganese, platinum and palladium.

2. The catalyst composition according to claim 1 , in which the carrier comprises mordenite type zeolite in an amount in the range of from 30 to 70 wt %, based on total weight of carrier.

3. The catalyst composition according to claim 1 , in which the carrier comprises ZSM-5 type zeolite in an amount of from 15 to 60 wt %, based on total weight of carrier.

4. The catalyst composition according to claim 1 , wherein the ZSM-5 type zeolite has a silica to alumina molar ratio in the range of from 15 to 40.

5. The catalyst composition according to claim 1 , wherein the ZSM-5 type zeolite has a number average crystal size in the range of from 25 to 200 nm, as determined by X-ray diffraction.

6. The catalyst composition according to claim 1 , wherein the catalytically active metals include platinum and tin.

7. A catalyst composition useful in the transalkylation and dealkylation of alkyaromatics, wherein the catalyst composition comprises:

(a) a carrier consisting essentially of: (i) mordenite type zeolite having a mean crystallite length parallel to the direction of the 12-ring channels of from 10 to 60 nm and a mesopore volume of at least 0.10 cc/gram in an amount in the range of from 20 to 90 wt %, based on total weight of carrier, (ii) ZSM-5 type zeolite having a silica-to-alumina molar ratio in the range of from 10 to 50 and present in an amount of from 10 to 70 wt %, based on total weight of carrier, wherein the ZSM-5 type zeolite has a number average crystal size in the range of from 25 to 200 nm, as determined by X-ray diffraction; and (iii) titania as a binder in an amount in the range of from 10 to 60 wt %, based on total weight of carrier; and

(b) of from 0.001 to 10 wt % of one or more catalytically active metals selected from the group consisting of tin, tungsten, vanadium, molybdenum, rhenium, nickel, cobalt, chromium, manganese, platinum and palladium.

8. The catalyst composition according to claim 7 , in which the carrier comprises mordenite type zeolite in an amount in the range of from 30 to 70 wt %, based on total weight of carrier.

9. The catalyst composition according to claim 7 , in which the carrier comprises ZSM-5 type zeolite in an amount of from 15 to 60 wt %, based on total weight of carrier.

10. The catalyst composition according to claim 7 , wherein the ZSM-5 type zeolite has a silica to alumina molar ratio in the range of from 15 to 40.

11. The catalyst composition according to claim 7 , wherein the catalytically active metals include platinum and tin.

Assignments (2)
CHANGE OF NAME Recorded Mar 7, 2022
From: SHELL OIL COMPANY
To: SHELL USA, INC.
Reel/Frame 059694/0819 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 9, 2021
From: LI, HONG-XIN; MAUER, RICHARD BEREND; PUJADAS, GISELA SABATER
To: SHELL OIL COMPANY
Reel/Frame 057430/0038 →