IP Library Granted Patent US 11,541,359
Granted Patent B2
US 11,541,359 · App. 16/497,977 · Granted Jan 3, 2023

Use of nanoporous carbon membranes for separating aqueous/organic mixtures

Inventors: Lyderic Bocquet (Paris, FR); Alessandro Siria (Paris, FR); Benoit Laborie (Paris, FR); Hiroaki Yoshida (Paris, FR); Simon Gravelle (Londres, GB)
Assignees: Paris Sciences et Lettres; Université Paris Cité; Centre National De La Recherche Scientifique (CNRS); Sorbonne Universite
B01D71/021B01D61/027B01D61/362B01D69/10C07B63/00B01D2325/02
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Quick Facts
Patent No.
US 11,541,359
App. No.
16/497,977
Granted
Jan 3, 2023
Kind
B2
Abstract

The invention relates to the extraction of organic compounds from mixtures of said compounds with water, using a nanoporous carbon membrane. The invention can be used in any field where it is desired to separate an organic compound of interest from water, such as the drying of alcohols or alkanes.

Claims (11)

1. A method for extracting an organic compound from a fluid mixture of the organic compound with water, wherein the method comprises:

contacting a nanoporous carbon membrane before its use with a pure preparation of the organic compound to be extracted to provide an activated nanoporous carbon membrane in which the pure preparation of the organic compound is adsorbed and fills pores of the membrane;

contacting the mixture with one side of the activated nanoporous carbon membrane in which the pores of the membrane contain the adsorbed pure preparation of the organic compound;

recovering the organic compound from the other side of the nanoporous carbon membrane, wherein the nanoporous carbon membrane is a multilayer graphene oxide (GO) or a reduced graphene oxide (rGO) membrane and the organic compound is an alcohol.

2. The method of claim 1 , wherein the nanoporous carbon membrane has pore size greater than about 0.9 nm and less than about 1.5 mm.

3. The method of claim 1 , wherein the alcohol is a C 1 -C 12 alcohol.

4. The method of claim 3 , wherein the C 1 -C 12 alcohol is selected from the group consisting of methanol, ethanol, propanol, butanol, ethylene glycol, propylene glycol, glycerol, and mixtures thereof.

5. The method of claim 1 , wherein the nanoporous carbon membrane is placed on a porous support layer.

6. The method of claim 1 , wherein the step of contacting the mixture with one side of the activated nanoporous carbon membrane is carried out while the membrane is still wet with the pure preparation of organic compound.

7. The method of claim 1 , wherein the nanoporous carbon membrane is a multilayer graphene oxide (GO).

8. The method of claim 1 , wherein the nanoporous carbon membrane has a thickness from 0.05 to 1 μm.

Assignments (9)
CORRECTIVE ASSIGNMENT TO CORRECT THE PROPERTY NUMBER 16930208 PREVIOUSLY RECORDED AT REEL: 060390 FRAME: 0122. ASSIGNOR(S) HEREBY CONFIRMS THE CHANGE OF NAME. Recorded Jan 11, 2023
From: UNIVERSITE DE PARIS
To: UNIVERSITÉ PARIS CITÉ
Reel/Frame 062387/0489 →
CORRECTIVE ASSIGNMENT TO CORRECT THE PROPERTY NUMBER 16930208 PREVIOUSLY RECORDED AT REEL: 060541 FRAME: 0336. ASSIGNOR(S) HEREBY CONFIRMS THE MERGER AND CHANGE OF NAME. Recorded Jan 11, 2023
From: UNIVERSITE PARIS DESCARTES; UNIVERSITE PARIS DIDEROT - PARIS 7
To: UNIVERSITE DE PARIS
Reel/Frame 062387/0346 →
CHANGE OF NAME Recorded Jun 20, 2022
From: UNIVERSITE DE PARIS
To: UNIVERSITÉ PARIS CITÉ
Reel/Frame 060390/0122 →
MERGER AND CHANGE OF NAME Recorded Jun 20, 2022
From: UNIVERSITE PARIS DESCARTES; UNIVERSITE PARIS DIDEROT - PARIS 7; UNIVERSITE DE PARIS
To: UNIVERSITE DE PARIS
Reel/Frame 060541/0336 →
CHANGE OF NAME Recorded Jan 19, 2022
From: PARIS SCIENCES ET LETTRES - QUARTIER LATIN
To: PARIS SCIENCES ET LETTRES
Reel/Frame 058772/0593 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 27, 2021
From: GRAVELLE, SIMON
To: PARIS SCIENCES ET LETTRES - QUARTIER LATIN; UNIVERSITE PARIS DIDEROT PARIS 7; CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE (CNRS); SORBONNE UNIVERSITE
Reel/Frame 056376/0150 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 27, 2021
From: ECOLE NORMALE SUPERIEURE
To: PARIS SCIENCES ET LETTRES - QUARTIER LATIN
Reel/Frame 056376/0238 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 27, 2021
From: YOSHIDA, HIROAKI
To: ECOLE NORMALE SUPERIEURE
Reel/Frame 056376/0215 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 27, 2021
From: BOCQUET, LYDERIC; SIRIA, ALESSANDRO; LABORIE, BENOIT
To: ECOLE NORMALE SUPERIEURE; UNIVERSITE PARIS DIDEROT PARIS 7; CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE (CNRS); SORBONNE UNIVERSITE
Reel/Frame 056376/0164 →