IP Library Granted Patent US 11,384,242
Granted Patent B2
US 11,384,242 · App. 16/525,121 · Granted Jul 12, 2022

Nylon terpolymers

Inventors: Jacob G. Ray (Pace, FL); Douglas Hoffman (Pensacola Beach, FL); Scott E. Powers (Rockford, MI)
Assignee: Ascend Performance Materials Operations LLC
C08L77/06C08G69/14C08G69/265C08L77/02C08L2203/16C08L2205/02
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Quick Facts
Patent No.
US 11,384,242
App. No.
16/525,121
Granted
Jul 12, 2022
Kind
B2
Abstract

A terpolymer composition is described that contains a statistical amount of 50-98 wt % of a first repeating AA-BB comonomer unit; 1-25 wt % of a second repeating AA-BB comonomer unit; and 1-25 wt % of a repeating lactam comonomer unit or 1-25 wt % of a third repeating AA-BB comonomer unit, where the terpolymer composition exhibits a high melting point similar to that of PA66 while also exhibiting a significantly reduced crystallization rate and crystallization temperature.

Claims (44)

1. A terpolymer comprising:

50-98 wt % of a first repeating AA-BB comonomer unit;

1-25 wt % of a second repeating AA-BB comonomer unit; and

1-25 wt % of a repeating lactam comonomer unit, wherein wt % is based upon total terpolymer weight;

wherein the terpolymer has a relative viscosity according to ASTM D789 (9.34) of 45 to 350 and a melting point greater than 215° C.; and the terpolymer is of Formula (3):

wherein in Formula (3):

a=2-16;

b=2-16;

c=50-98 wt %;

d=2-16;

e=1-25 wt %;

f=2-16; and

g=1-25 wt %.

2. The terpolymer according to claim 1 , wherein the terpolymer has a relative viscosity according to ASTM D789 (9.34) of 80 to 300.

3. The terpolymer according to claim 1 , wherein the first repeating AA-BB unit is Nylon 6,6.

4. The terpolymer according to claim 1 , wherein e=10-24 wt %.

5. A composition comprising the terpolymer according to claim 1 , further comprising greater than 60 ppm and less than 500 ppm copper.

6. A composition comprising the terpolymer according to claim 1 , further comprising a lubricant.

7. A composition comprising the terpolymer according to claim 1 , further comprising an anti-block agent.

8. A film comprising the terpolymer according to claim 1 .

9. The film according to claim 8 , where the film is a blown film.

10. The film according to claim 9 , where the blown film is a multilayer film.

11. The multilayer film according to claim 10 , where the film comprises 3 to 10 layers.

12. The multilayer film according to claim 11 , where at least two of the 3 to 10 layers comprise non-terpolymer layers selected from the group consisting of low density polyethylene (LDPE), ethylene acrylic acid copolymer (EAA), ethylene methacrylic acid copolymer (EMAA), ethylene vinyl acetate copolymer (EVA), ethylene methacrylate copolymer (EMA), anhydride modified polyethylene (AMP), nylon (PA) and ethylene vinyl alcohol copolymer (EVOH).

13. The film according to claim 8 , where the film is a cast film.

14. The film according to claim 8 , where the film is biaxially oriented.

15. The film according to claim 14 , where the biaxially oriented film is a multilayer film.

16. The multilayer film according to claim 15 , where the film comprises 3 to 10 layers.

17. The multilayer film according to claim 16 , where at least two of the 3 to 10 layers comprise non-terpolymer layers selected from the group consisting of low density polyethylene (LDPE), ethylene acrylic acid copolymer (EAA), ethylene methacrylic acid copolymer (EMAA), ethylene vinyl acetate copolymer (EVA), ethylene methacrylate copolymer (EMA), anhydride modified polyethylene (AMP), nylon (PA) and ethylene vinyl alcohol copolymer (EVOH).

18. The terpolymer according to claim 1 , wherein the terpolymer is selected from the group consisting of:

PA66-s-6 10 -s-6, I 4 ;

PA66-s-6 20 -s-6, I 8 ;

PA66-s-6 14 -s-6, I 13 ; and

PA66-s-6 12 -s-6, I 20 .

19. A film comprising a terpolymer of Formula (3):

wherein in Formula (3):

a=2-16;

b=2-16;

c=50-98 wt %;

d=2-16;

e=1-25 wt %;

f=2-16; and

g=1-25 wt %; and

wherein the terpolymer has a relative viscosity according to ASTM D789 (9.34) of 45 to 350, a melting point greater than 220° C.; and is characterized by an 8° C. to 15° C. increase in T melt −T crystallization (T m −T c ) as compared with copolyamide PA66-s-6.

Assignments (9)
RELEASE OF SECURITY INTEREST Recorded Dec 23, 2025
From: WILMINGTON SAVINGS FUND SOCIETY, FSB
To: ASCEND PERFORMANCE MATERIALS OPERATIONS LLC
Reel/Frame 074050/0090 →
SECURITY INTEREST Recorded Dec 23, 2025
From: ASCEND PERFORMANCE MATERIALS OPERATIONS LLC
To: WILMINGTON SAVINGS FUND SOCIETY, FSB
Reel/Frame 074056/0183 →
RELEASE OF SECURITY INTEREST Recorded Dec 23, 2025
From: WILMINGTON SAVINGS FUND SOCIETY, FSB
To: ASCEND PERFORMANCE MATERIALS OPERATIONS LLC
Reel/Frame 074049/0662 →
SECURITY INTEREST Recorded Dec 19, 2025
From: ASCEND PERFORMANCE MATERIALS OPERATIONS LLC
To: WELLS FARGO BANK, NATIONAL ASSOCIATION
Reel/Frame 074007/0183 →
SECURITY INTEREST Recorded Apr 10, 2025
From: BANK OF AMERICA, N.A.
To: WILMINGTON SAVINGS FUND SOCIETY, FSB
Reel/Frame 070811/0692 →
SECURITY INTEREST Recorded Apr 10, 2025
From: BANK OF AMERICA, N.A.
To: WILMINGTON SAVINGS FUND SOCIETY, FSB
Reel/Frame 070811/0705 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 9, 2022
From: RAY, JACOB G.; HOFFMAN, DOUGLAS; POWERS, SCOTT E.
To: ASCEND PERFORMANCE MATERIALS OPERATIONS LLC
Reel/Frame 059208/0711 →
SECURITY INTEREST Recorded Aug 28, 2019
From: ASCEND PERFORMANCE MATERIALS OPERATIONS LLC
To: BANK OF AMERICA, N.A.
Reel/Frame 050207/0184 →
SECURITY INTEREST Recorded Aug 27, 2019
From: ASCEND PERFORMANCE MATERIALS OPERATIONS LLC
To: WELLS FARGO CAPITAL FINANCE, LLC
Reel/Frame 050177/0150 →