IP Library Granted Patent US 11,156,074
Granted Patent B2
US 11,156,074 · App. 16/561,646 · Granted Oct 26, 2021

Thermally activated strong acids

Inventors: Paul Richard Weider (Houston, TX); Robert Lawrence Blackbourn (Houston, TX); Ying Zhang (Sugar Land, TX); Lee Nicky Morgenthaler (Houston, TX); Ryan Matthew Van Zanten (Katy, TX)
Assignee: SHELL OIL COMPANY
E21B43/36C09K8/506C09K8/516C09K8/72E21B43/25
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Quick Facts
Patent No.
US 11,156,074
App. No.
16/561,646
Granted
Oct 26, 2021
Kind
B2
Abstract

An acid-generating fluid includes a thermally activated strong acid precursor. The thermally activated strong acid precursor can include a component selected from aldehydes, ketones, and combinations thereof, in combination with a precursor of a compound adapted to react to liberate sulfur dioxide; or it can include sulfur dioxide in combination with a precursor of a compound adapted to react to liberate a component selected from aldehydes, ketones, and combinations thereof.

Claims (49)

1. A method comprising:

providing an acid-generating fluid that comprises water and a thermally activated strong acid precursor, the thermally activated strong acid precursor comprising:

a precursor of a compound adapted to react to liberate sulfur dioxide, wherein said precursor is a sulfone; and

a component selected from aldehydes, ketones, and combinations thereof;

placing the acid-generating fluid into a subterranean formation;

thermally activating the precursor, thereby liberating sulfur dioxide; and

reacting the sulfur dioxide and the component selected from aldehydes, ketones, and combinations thereof to form a thermally activated strong acid.

2. The method of claim 1 , wherein the precursor is selected from the group consisting of a sulfone adduct of butadiene, a sulfone adduct of piperylene, a sulfone adduct of isoprene, and combinations thereof.

3. The method of claim 1 , wherein the acid-generating fluid further comprises a dienophile.

4. The method of claim 3 , wherein the dienophile and the thermally activated strong acid precursor are provided in a 1:1 molar ratio.

5. The method of claim 1 , wherein the acid-generating fluid further comprises a base.

6. The method of claim 5 , wherein the base is CaCO 3 .

7. The method of claim 1 , wherein the acid-generating fluid has a pH of greater than 4.

8. A method comprising:

providing an acid-generating fluid that comprises water and a thermally activated strong acid precursor, the thermally activated strong acid precursor comprising:

a precursor of a compound adapted to react to liberate sulfur dioxide, and

a component selected from aldehydes, ketones, and combinations thereof;

placing the acid-generating fluid into a subterranean formation;

thermally activating the precursor, thereby liberating sulfur dioxide; and

reacting the sulfur dioxide and the component selected from aldehydes, ketones, and combinations thereof to form a thermally activated strong acid;

wherein the acid-generating fluid is an emulsion.

9. The method of claim 8 , wherein said precursor is a sulfone.

10. The method of claim 8 , wherein the precursor is selected from the group consisting of a sulfone adduct of butadiene, a sulfone adduct of piperylene, a sulfone adduct of isoprene, and combinations thereof.

11. The method of claim 8 , wherein said precursor is a sulfite.

12. The method of claim 8 , wherein said precursor is a sulfite ester.

13. The method of claim 8 , wherein said precursor is selected from the group consisting of: ethylene sulfite and dimethyl sulfite, diethyl sulfite, 1,2-propylene sulfite, and 1,3-propylene sulfite, and combinations thereof.

14. The method of claim 8 , wherein the acid-generating fluid further comprises a dienophile.

15. The method of claim 14 , wherein the dienophile and the thermally activated strong acid precursor are provided in a 1:1 molar ratio.

16. The method of claim 8 , wherein the acid-generating fluid further comprises a base.

17. The method of claim 16 , wherein the base is CaCO 3 .

18. The method of claim 8 , wherein the acid-generating fluid has a pH of greater than 4.

19. A method comprising:

providing an acid-generating fluid that comprises water and a thermally activated strong acid precursor, the thermally activated strong acid precursor comprising:

a precursor of a compound adapted to react to liberate sulfur dioxide, and

a component selected from aldehydes, ketones, and combinations thereof;

placing the acid-generating fluid into a subterranean formation;

thermally activating the precursor, thereby liberating sulfur dioxide; and

reacting the sulfur dioxide and the component selected from aldehydes, ketones, and combinations thereof to form a thermally activated strong acid;

wherein the acid generating fluid is a component of a fluid loss control pill.

20. The method of claim 19 , wherein said precursor is a sulfone.

21. The method of claim 19 , wherein the precursor is selected from the group consisting of a sulfone adduct of butadiene, a sulfone adduct of piperylene, a sulfone adduct of isoprene, and combinations thereof.

22. The method of claim 19 , wherein said precursor is a sulfite.

23. The method of claim 19 , wherein said precursor is a sulfite ester.

24. The method of claim 19 , wherein said precursor is selected from the group consisting of: ethylene sulfite and dimethyl sulfite, diethyl sulfite, 1,2-propylene sulfite, and 1,3-propylene sulfite, and combinations thereof.

25. The method of claim 19 , wherein the acid-generating fluid further comprises a dienophile.

26. The method of claim 25 , wherein the dienophile and the thermally activated strong acid precursor are provided in a 1:1 molar ratio.

27. The method of claim 19 , wherein the acid-generating fluid further comprises a base.

28. The method of claim 27 , wherein the base is CaCO 3 .

29. The method of claim 19 , wherein the acid-generating fluid has a pH of greater than 4.

Assignments (2)
CHANGE OF NAME Recorded Mar 7, 2022
From: SHELL OIL COMPANY
To: SHELL USA, INC.
Reel/Frame 059694/0819 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 5, 2019
From: BLACKBOURN, ROBERT LAWRENCE; MORGENTHALER, LEE NICKY; VAN ZANTEN, RYAN MATTHEW; WEIDER, PAUL RICHARD; ZHANG, YING
To: SHELL OIL COMPANY
Reel/Frame 050282/0568 →