IP Library Granted Patent US 10,774,025
Granted Patent B2
US 10,774,025 · App. 16/607,018 · Granted Sep 15, 2020

Method for producing polyfunctional acrylate

Inventors: Keisuke Ito (Hakusan, JP); Shigeaki Matsumoto (Hakusan, JP); Keita Shigematsu (Hakusan, JP)
Assignee: OSAKA ORGANIC CHEMICAL INDUSTRY LTD.
C07C67/03C07C67/54C07C69/54
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Quick Facts
Patent No.
US 10,774,025
App. No.
16/607,018
Granted
Sep 15, 2020
Kind
B2
Abstract

The present invention provides a production method of a multifunctional acrylate with a reduced tin content which includes adding an acid to a mixture containing an organotin compound and a multifunctional acrylate and distilling the mixture containing the acid.

Claims (24)

1. A method for producing a multifunctional acrylate with a reduced tin content comprising adding an acid to a mixture comprising a dialkyltin oxide and a multifunctional acrylate and distilling the mixture comprising the acid.

2. The production method according to claim 1 wherein the amount of the acid to be added is 50-500 parts by weight per 100 parts by weight of the content of tin in the mixture comprising the dialkyltin oxide and the multifunctional acrylate.

3. A method for producing a multifunctional acrylate comprising

step 1 comprising a transesterification reaction of an acrylate and a polyhydric alcohol in the presence of a dialkyltin oxide to give a reaction mixture comprising the dialkyltin oxide and a multifunctional acrylate,

step 2 comprising evaporating a compound having a boiling point lower than the dialkyltin oxide and the multifunctional acrylate from the reaction mixture to give a residue comprising the dialkyltin oxide and the multifunctional acrylate,

step 3 comprising distilling the residue to give a distillate comprising the dialkyltin oxide and the multifunctional acrylate and a distillation residue comprising the dialkyltin oxide, and

step 4 comprising adding an acid to the distillate and distilling the mixture comprising the acid to give a multifunctional acrylate with a reduced tin content.

4. The production method according to claim 3 wherein the amount of the acid to be added is 50-500 parts by weight per 100 parts by weight of the content of tin in the distillate comprising the dialkyltin oxide and the multifunctional acrylate.

5. The production method according to claim 3 wherein the distillation residue obtained in step 3 is reused in a transesterification reaction in a new step 1.

6. The production method according to claim 3 wherein the polyhydric alcohol is a dihydric alcohol.

7. The production method according to claim 6 wherein the dihydric alcohol is a C 2-10 alkanediol.

8. The production method according to claim 1 wherein the multifunctional acrylate is a difunctional acrylate.

9. The production method according to claim 1 wherein the acid is an inorganic acid.

10. The production method according to claim 1 wherein the dialkyltin oxide has two alkyl groups independently having a carbon number of 3-18.

11. The production method according to claim 4 wherein the distillation residue obtained in step 3 is reused in a transesterification reaction in a new step 1.

12. The production method according to claim 11 wherein the polyhydric alcohol is a dihydric alcohol.

13. The production method according to claim 12 wherein the dihydric alcohol is a C 2-10 alkanediol.

14. The production method according to claim 13 wherein the multifunctional acrylate is a difunctional acrylate.

15. The production method according to claim 14 wherein the acid is an inorganic acid.

16. The production method according to claim 15 wherein the dialkyltin oxide has two alkyl groups independently having a carbon number of 3-18.

17. The production method according to claim 3 wherein the multifunctional acrylate is a difunctional acrylate.

18. The production method according to claim 3 wherein the acid is an inorganic acid.

19. The production method according to claim 3 wherein the dialkyltin oxide has two alkyl groups independently having a carbon number of 3-18.

20. The production method according to claim 3 wherein the multifunctional acrylate is a difunctional acrylate, the acid is an inorganic acid, and the dialkyltin oxide has two alkyl groups independently having a carbon number of 3-18.

Assignments (2)
CHANGE OF ADDRESS Recorded Apr 15, 2022
From: OSAKA ORGANIC CHEMICAL INDUSTRY LTD.
To: OSAKA ORGANIC CHEMICAL INDUSTRY LTD.
Reel/Frame 059721/0809 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 22, 2019
From: ITO, KEISUKE; MATSUMOTO, SHIGEAKI; SHIGEMATSU, KEITA
To: OSAKA ORGANIC CHEMICAL INDUSTRY LTD.
Reel/Frame 050787/0439 →