IP Library Granted Patent US 11,111,205
Granted Patent B2
US 11,111,205 · App. 16/631,945 · Granted Sep 7, 2021

Process for preparing alkanediol and dialkyl carbonate

Inventors: Henri Preising (Sachsen-Anhalt, DE); Frederik Hendrik Van Der Steen (Amsterdam, NL); Garo Garbis Vaporciyan (Amsterdam, NL); Wolfgang Dirk Lose (Sachsen-Anhalt, DE); Silke Eva Sabine Leonhardt (Sachsen-Anhalt, DE)
Assignee: SHELL OIL COMPANY
C07C68/065B01J27/1802B01J37/031B01J37/04B01J37/08C01B25/36C07C29/48
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Quick Facts
Patent No.
US 11,111,205
App. No.
16/631,945
Granted
Sep 7, 2021
Kind
B2
Abstract

The invention relates to a process for the preparation of an alkanediol and a dialkyl carbonate comprising reacting an alkylene carbonate and an alkanol in the presence of a catalyst, wherein the catalyst is aluminum phosphate.

Claims (14)

1. A process for the preparation of an alkanediol and a dialkyl carbonate comprising reacting an alkylene carbonate and an alkanol in the presence of a catalyst, wherein the catalyst is aluminum phosphate.

2. The process according to claim 1 , wherein the aluminum phosphate catalyst is amorphous.

3. The process according to claim 2 , wherein more than 90% of the catalyst is amorphous.

4. The process according to claim 1 , wherein the aluminum phosphate catalyst has a molar (or atomic) ratio [Al]/[P] of from 0.1:1 to 20:1.

5. The process according to claim 1 , wherein the aluminum phosphate is synthesized aluminum phosphate.

6. The process according to claim 5 , wherein the aluminum phosphate catalyst is a catalyst obtained by a process for preparing an aluminum phosphate catalyst, which comprises:

(a) mixing an aluminum containing salt with phosphoric acid in a molar ratio [Al]/[P] of from 0.1:1 to 20:1;

(b) mixing a base with the mixture resulting from step (a), resulting in the formation of an aluminum phosphate precipitate;

(c) optionally heating the precipitate containing mixture; and

(d) recovering the precipitate.

7. The process according to claim 1 , wherein the alkylene carbonate is a C 2 -C 6 alkylene carbonate.

8. The process according to claim 7 , wherein the alkylene carbonate is ethylene carbonate or propylene carbonate.

9. The process according to claim 1 , wherein the alkanol is a C 1 -C 4 alkanol.

10. The process according to claim 9 , wherein the alkanol is methanol, ethanol or isopropanol.

Assignments (2)
CHANGE OF NAME Recorded Mar 7, 2022
From: SHELL OIL COMPANY
To: SHELL USA, INC.
Reel/Frame 059694/0819 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 29, 2021
From: PREISING, HENRI; VAN DER STEEN, FREDERIK HENDRIK; VAPORCIYAN, GARO GARBIS; LOSE, WOLFGANG DIRK; LEONHARDT, SILKE EVA SABINE
To: SHELL OIL COMPANY
Reel/Frame 057959/0619 →