IP Library Granted Patent US 11,377,514
Granted Patent B2
US 11,377,514 · App. 16/797,844 · Granted Jul 5, 2022

Combined seals, compositions, and methods of making the same

Inventors: Krishnamachari Gopalan (Troy, MI); Robert J. Lenhart (Fort Wayne, IN); Gending Ji (Canton, MI); Roland Herd-Smith (Brignancourt, FR)
Assignee: COOPER-STANDARD AUTOMOTIVE, INC.
C08F255/02C08J3/24C08J9/0061C08J9/228C08K3/011C08K3/36C08K5/0025C08L23/0815C08L23/12C08L23/14C08L23/142C08L23/16C09K3/10C08F2500/21C08J2351/06C08J2423/08C08J2423/12C08J2423/14C08L2205/025C08L2312/08C09K2003/1068C09K2200/0494C09K2200/062
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Quick Facts
Patent No.
US 11,377,514
App. No.
16/797,844
Granted
Jul 5, 2022
Kind
B2
Abstract

A combined sealing member is provided that includes a composition comprising two or more polyolefin elastomers selected from the group consisting of a dense, a micro-dense and a dynamic silane-crosslinked polyolefin elastomer having a respective density of less than 0.90 g/cm 3 , less than 0.70 g/cm 3 , and less than 0.60 g/cm 3 . The combined sealing member exhibits a compression set of from about 5.0% to about 35.0%, as measured according to ASTM D 395 (22 hrs @ 70° C.).

Claims (44)

1. A combined sealing member comprising: a composition comprising two or more polyolefin elastomers selected from the group consisting of

a dense silane-crosslinked polyolefin elastomer having a density of less than 0.90 g/cm 3 , a tensile strength ranging from 10.4 to about 14.5 MPa as measured according to ASTM D412, a Shore A hardness ranging from about 76 to about 88 as measured according to ASTM D412, and a crystallinity of from about 5% to about 15%, wherein from about 1 wt % to about 20 wt % of the dense silane-crosslinked polyolefin elastomer is a polypropylene filler having a crystallinity greater than 40%,

a microdense silane-crosslinked polyolefin elastomer having a density of less than 0.70 g/cm 3 , a tensile strength ranging from about 5.0 to about 8.7 MPa as measured according to ASTM D412, a Shore A hardness ranging from 60 to 87 as measured according to ASTM D412, and a crystallinity of from about 5% to about 15%, wherein from about 1 wt % to about 20 wt % of the microdense silane-crosslinked polyolefin elastomer is a polypropylene filler having a crystallinity greater than 40%, and

a dynamic silane-crosslinked polyolefin elastomer having a density of less than 0.60 g/cm 3 , a tensile strength ranging from about 2.0 to about 2.9 MPa as measured according to ASTM D412 and a crystallinity of from about 5% to about 15%,

wherein the polyolefin elastomers do not display a Mullins effect or a Payne effect,

wherein the combined sealing member and the foamed silane-crosslinked polyolefin elastomers are thermosets, and

wherein the combined sealing member exhibits a compression set of from about 5.0% to about 35.0%, as measured according to ASTM D 395 (22 hrs @ 70° C.).

2. The combined sealing member of claim 1 , wherein the compression set is from about 15.0% to about 35.0%, as measured according to ASTM D 395 (22 hrs @ 70° C.).

3. The combined sealing member of claim 1 , wherein the two or more polyolefin elastomers are selected from the group consisting of

a dense silane-crosslinked polyolefin elastomer having a density of about 0.80 g/cm 3 to about 0.89 g/cm 3 ,

a microdense silane-crosslinked polyolefin elastomer having a density of about 0.40 g/cm 3 to about 0.59 g/cm 3 , and

a dynamic silane-crosslinked polyolefin elastomer having a density of about 0.40 g/cm 3 to about 0.59 g/cm 3 .

4. The combined sealing member of claim 1 , wherein the silane-crosslinked polyolefin elastomers exhibit crystallinities of from about 5% to about 10%.

5. The combined sealing member of claim 1 , wherein the silane-crosslinked polyolefin elastomers exhibit glass transition temperatures of from about −75° C. to about −25° C.

6. The combined sealing member of claim 1 , wherein the sealing member exhibits a weathering color difference of from about 0.25 ΔE to about 2.0 ΔE, as measured according to ASTM D2244.

7. The combined sealing member of claim 1 , further comprising:

a coloring agent.

8. A combined sealing member comprising:

comprising a first and a second polyolefin elastomer,

wherein the first elastomer comprises a microdense silane-crosslinked polyolefin elastomer having a density of less than 0.70 g/cm 3 , a tensile strength ranging from about 5.0 to about 8.7 MPa as measured according to ASTM D412, and a Shore A hardness ranging from 60 to 87 as measured according to ASTM D412, and a crystallinity of from about 5% to about 15%, wherein from about 1 wt % to about 20 wt % of the microdense silane-crosslinked polyolefin elastomer is a polypropylene filler having a crystallinity greater than 40%, and

wherein the second elastomer comprises

a dense silane-crosslinked polyolefin elastomer having a density of less than 0.90 g/cm 3 , a tensile strength ranging from 10.4 to about 14.5 MPa as measured according to ASTM D412, a Shore A hardness ranging from about 76 to about 88 as measured according to ASTM D412, and a crystallinity of from about 5% to about 15%, wherein from about 1 wt % to about 20 wt % of the dense silane-crosslinked polyolefin elastomer is a polypropylene filler having a crystallinity greater than 40%, or

a dynamic silane-crosslinked polyolefin elastomer having a density of less than 0.60 g/cm 3 , a tensile strength ranging from about 2.0 to about 2.9 MPa as measured according to ASTM D412, and a crystallinity of from about 5% to about 15%,

wherein the polyolefin elastomers do not display a Mullins effect or a Payne effect,

wherein the combined sealing member and the foamed silane-crosslinked polyolefin elastomers are thermosets, and

wherein the combined sealing member exhibits a compression set of from about 5.0% to about 35.0%, as measured according to ASTM D 395 (22 hrs @ 70° C.).

9. The combined sealing member of claim 8 , wherein the compression set is from about 15.0% to about 35.0%, as measured according to ASTM D 395 (22 hrs @ 70° C.).

10. The combined sealing member of claim 8 , wherein

the first polyolefin elastomer is a microdense silane-crosslinked polyolefin elastomer having a density of about 0.40 g/cm 3 to about 0.59 g/cm 3 and

the second polyolefin elastomer comprises a dense silane-crosslinked polyolefin elastomer having a density of about 0.80 g/cm 3 to about 0.89 g/cm 3 , or a dynamic silane-crosslinked polyolefin elastomer having a density of about 0.40 g/cm 3 to about 0.59 g/cm 3 .

11. The combined sealing member of claim 8 , wherein the silane-crosslinked polyolefin elastomers exhibit crystallinities of from about 5% to about 10%.

12. The combined sealing member of claim 8 , wherein the silane-crosslinked polyolefin elastomers exhibit glass transition temperatures of from about −75° C. to about −25° C.

13. A combined sealing member comprising:

a dense silane-crosslinked polyolefin elastomer having a density of less than 0.90 g/cm 3 , a tensile strength ranging from 10.4 to about 14.5 MPa as measured according to ASTM D412, a Shore A hardness ranging from about 76 to about 88 as measured according to ASTM D412, and a crystallinity of from about 5% to about 15%, wherein from about 1 wt % to about 20 wt % of the dense silane-crosslinked polyolefin elastomer is a polypropylene filler having a crystallinity greater than 40%, and

a dynamic silane-crosslinked polyolefin elastomer having a density of less than 0.60 g/cm 3 , a tensile strength ranging from about 2.0 to about 2.9 MPa as measured according to ASTM D412 and a crystallinity of from about 5% to about 15%,

wherein the polyolefin elastomers do not display a Mullins effect or a Payne effect,

wherein the combined sealing member and the foamed silane-crosslinked polyolefin elastomers are thermosets, and

wherein the combined sealing member exhibits a compression set of from about 5.0% to about 35.0%, as measured according to ASTM D 395 (22 hrs @ 70° C.).

14. The combined sealing member of claim 13 , wherein the compression set is from about 15.0% to about 35.0%, as measured according to ASTM D 395 (22 hrs @ 70° C.).

15. The combined sealing member of claim 13 , wherein the dense silane-crosslinked polyolefin elastomer has a density of about 0.80 g/cm 3 to about 0.89 g/cm 3 , and the dynamic silane-crosslinked polyolefin elastomer has a density of about 0.40 g/cm 3 to about 0.59 g/cm 3 .

16. The combined sealing member of claim 13 , wherein the silane-crosslinked polyolefin elastomers exhibit crystallinities of from about 5% to about 10%.

17. The combined sealing member of claim 13 , wherein the silane-crosslinked polyolefin elastomers exhibit glass transition temperatures of from about −75° C. to about −25° C.

18. The combined sealing member of claim 13 , further comprising:

a coloring agent.

Assignments (6)
PATENT SECURITY AGREEMENT Recorded Mar 5, 2026
From: COOPER-STANDARD AUTOMOTIVE INC.
To: U.S. BANK TRUST COMPANY, NATIONAL ASSOCIATION
Reel/Frame 075019/0478 →
RELEASE OF SECURITY INTEREST IN PATENTS PREVIOUSLY RECORDED AT REEL/FRAME (062545/0715) Recorded Mar 4, 2026
From: U.S. BANK TRUST COMPANY, NATIONAL ASSOCIATION, AS COLLATERAL AGENT
To: COOPER-STANDARD AUTOMOTIVE INC.; COOPER-STANDARD INDUSTRIAL AND SPECIALTY GROUP, LLC
Reel/Frame 075022/0267 →
RELEASE OF SECURITY INTEREST IN PATENTS PREVIOUSLY RECORDED REEL/FRAME (062544/0357) Recorded Mar 4, 2026
From: U.S. BANK TRUST COMPANY, NATIONAL ASSOCIATION, AS COLLATERAL AGENT
To: COOPER-STANDARD AUTOMOTIVE INC.; COOPER-STANDARD INDUSTRIAL AND SPECIALTY GROUP, LLC
Reel/Frame 075022/0543 →
PATENT SECURITY AGREEMENT (1ST LIEN) Recorded Jan 30, 2023
From: COOPER-STANDARD AUTOMOTIVE INC.; COOPER-STANDARD INDUSTRIAL AND SPECIALTY GROUP, LLC
To: U.S. BANK TRUST COMPANY, NATIONAL ASSOCIATION, AS COLLATERAL AGENT
Reel/Frame 062544/0357 →
PATENT SECURITY AGREEMENT (3RD LIEN) Recorded Jan 30, 2023
From: COOPER-STANDARD AUTOMOTIVE INC.; COOPER-STANDARD INDUSTRIAL AND SPECIALTY GROUP, LLC
To: U.S. BANK TRUST COMPANY, NATIONAL ASSOCIATION, AS COLLATERAL AGENT
Reel/Frame 062545/0715 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 21, 2020
From: GOPALAN, KRISHNAMACHARI; LENHART, ROBERT J.; JI, GENDING; HERD-SMITH, ROLAND
To: COOPER-STANDARD AUTOMOTIVE, INC.
Reel/Frame 051890/0947 →