IP Library Granted Patent US 12,404,543
Granted Patent B2
US 12,404,543 · App. 16/854,618 · Granted Sep 2, 2025

Hybridization compositions and methods for making and using compositions

Inventor: Jens Mollerup (Roskilde, DK)
Assignee: Agilent Technologies, Inc.
C12Q1/6841C12Q1/6832
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Quick Facts
Patent No.
US 12,404,543
App. No.
16/854,618
Granted
Sep 2, 2025
Kind
B2
Abstract

The present disclosure relates to hybridization buffers for use in hybridization, for example, for use in in situ hybridization (ISH). Hybridization buffers and compositions comprising a sulfone solvent and polyvinyl sulfonic acid or a salt thereof, and methods of making and using, the same are disclosed.

Claims (25)

1. An in situ hybridization buffer comprising:

a sulfone solvent in a concentration from 5 to 30% (v/v); and

a sulfonic acid polymer of formula (I), (Ia), (II), (IIa) or (III):

or a salt of any one of Formulas (I), (Ia), (II), (IIa) or (III), wherein: R 1 is hydrogen or C 1-6 aliphatic; L, when present, is a covalent bond or C 1-6 aliphatic, R 2 , when present, is a covalent bond, C 1-6 aliphatic, phenyl, or a 6-membered heteroaryl ring having 1-3 nitrogens, wherein: R 2 is substituted with 1 or 2-SO 3 H groups or a salt thereof, provided that when R 2 is a covalent bond, only 1-SO 3 H group or a salt thereof is present, and R 2 is optionally substituted with 1-2 groups independently selected from —-R 3 , halogen, —CN, —NO 2 , —OR 3 , —N(R 3 ) 2 , and —SR 3 , wherein each R 3 is independently hydrogen or a C 1-6 alkyl group; and n is an integer greater than 10; and

wherein the sulfonic acid polymer or salt thereof is present in a concentration from 5 to 50% (w/v); and

wherein the hybridization buffer is homogeneous without phase separation after storage at 2-8° C. for 2-24 months.

2. The hybridization buffer of claim 1 , wherein R 1 is hydrogen.

3. The hybridization buffer of claim 1 , wherein R 1 is C 1-6 aliphatic.

4. The hybridization buffer of claim 1 , wherein L is a covalent bond.

5. The hybridization buffer of claim 1 , wherein L is C 1-6 aliphatic.

6. The hybridization buffer of claim 1 , wherein L is methylene.

7. The hybridization buffer of claim 1 , further comprising water.

8. The hybridization buffer of claim 1 , wherein the sulfonic acid polymer or salt thereof is polyvinylsulfonic acid or a salt thereof.

9. The hybridization buffer of claim 1 , wherein the concentration of the sulfone solvent is from 10% to 20% (v/v).

10. The hybridization buffer of claim 1 , wherein the sulfone solvent is selected from the group consisting of dimethyl sulfone, diphenyl sulfone, methyl phenyl sulfone, tetramethylene sulfone (sulfolane), and mixtures thereof.

11. The hybridization buffer of claim 1 , wherein the sulfone solvent is sulfolane.

12. The hybridization buffer of claim 1 , wherein the concentration of the sulfonic acid polymer or salt thereof is from 20% to 40% (w/v).

13. The hybridization buffer of claim 1 , further comprising dextran sulfate in concentration no greater than 20% (w/v).

14. The hybridization buffer of claim 1 , wherein the hybridization buffer has a viscosity at 25° C. of 60 mPa·s, as measured by microviscometry.

15. The hybridization buffer of claim 1 , wherein the hybridization buffer is stable at 2-8° C. for 2-24 months.

16. The hybridization buffer of claim 1 , further comprising NaCl and 3-(N-morpholino) propanesulfonic acid (MOPS).

17. The hybridization buffer claim 1 , further comprising:

an accelerating agent in a concentration no greater than 20% (w/v), wherein

the sulfone solvent is sulfolane in a concentration of 10% (v/v),

the sulfonic acid polymer or salt thereof is in a concentration of 30% (w/v).

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Apr 21, 2020
From: MOLLERUP, JENS
To: AGILENT TECHNOLOGIES, INC.
Reel/Frame 052456/0542 →