IP Library Granted Patent US 11,104,642
Granted Patent B2
US 11,104,642 · App. 16/869,826 · Granted Aug 31, 2021

Method for preparing methyl mercaptan

Inventors: Georges Fremy (Sauveterre de Bearn, FR); Patrice Barre (Lons, FR); Jean-Michel Raymond (Cauneille, FR)
Assignee: Arkema France
C07C319/06C01B32/75C07C319/02C07C319/24Y02P20/582
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Quick Facts
Patent No.
US 11,104,642
App. No.
16/869,826
Granted
Aug 31, 2021
Kind
B2
Abstract

The present invention relates to a method for preparing methyl mercaptan, in batches or continuously, preferably continuously, said method including at least the following steps: a) reacting at least one hydrocarbon feedstock in the presence of hydrogen sulphide (H 2 S) and optionally sulphur (S) such as to form carbon disulphide (CS 2 ) and hydrogen (H 2 ); b) reacting said carbon disulphide (CS 2 ) by hydrogenation in the presence of said hydrogen (H 2 ) obtained in step a) such as to form methyl mercaptan (CH 3 SH), hydrogen sulphide (H 2 S) and possibly hydrogen (H 2 ); c) optionally recirculating said hydrogen sulphide (H 2 S) formed during step b) to step a); and d) recovering the methyl mercaptan.

Claims (23)

1. Process for preparing methyl mercaptan, said process being batchwise or continuous and comprising at least the following steps:

a) reaction of at least one hydrocarbon charge in the presence of hydrogen sulphide (H 2 S) and optionally of sulphur (S) to form carbon disulphide (CS 2 ) and hydrogen (H 2 ),

b) hydrogenation reaction of said carbon disulphide (CS 2 ) in the presence of said hydrogen (H 2 ), both obtained in step a), to form methyl mercaptan (CH 3 SH), hydrogen sulphide (H 2 S) and optionally hydrogen (H 2 ),

c) optionally, recycling said hydrogen sulphide (H 2 S) formed in step b) to step a), and

d) recovery of the methyl mercaptan.

2. Process according to claim 1 , wherein the hydrocarbon charge is in gaseous, liquid or solid form, and comprises at least one hydrocarbon having a hydrocarbon chain in saturated or unsaturated linear, branched or cyclic form.

3. Process according to claim 1 , wherein the hydrocarbon charge comprises at least one alkane.

4. Process according to claim 1 , wherein the hydrocarbon charge is methane.

5. Process according to claim 1 , wherein the hydrogen sulphide formed in step b) is recycled into step a).

6. Process according to claim 1 , wherein the hydrogen optionally formed in step b) may be reacted with sulphur to form hydrogen sulphide.

7. Process according to claim 1 , wherein the molar H 2 S/hydrocarbon charge ratio is between 0 and about 100.

8. Process according to claim 1 , wherein the reaction temperature in step a) is between 500° C. and 1300° C.

9. Process according to claim 1 , wherein the reaction temperature in step b) is between 100° C. and 400° C.

10. Process according to claim 1 , wherein the methyl mercaptan is reacted with sulphur to form dimethyl disulphide.

11. Process according to claim 1 , wherein the process is a continuous process.

12. Process according to claim 2 , wherein the hydrocarbon charge is in gaseous or liquid form.

13. Process according to claim 2 , wherein the hydrocarbon charge is in gaseous form.

14. Process according to claim 3 , wherein the hydrocarbon charge is at least one of methane, ethane, propane and butane.

15. Process according to claim 7 , wherein the molar H 2 S/hydrocarbon charge ratio is between 0.5 and about 10.

16. Process according to claim 7 , wherein the molar H 2 S/hydrocarbon charge ratio is between 1 and about 3.

17. Process according to claim 8 , wherein the reaction temperature in step a) is between 700° C. and 1100° C.

18. Process according to claim 8 , wherein the reaction temperature in step a) is between 800° C. and 1000° C.

19. Process according to claim 9 , wherein the reaction temperature in step b) is between 200° C. and 300° C.

Assignments (2)
CHANGE OF ADDRESS Recorded Jul 4, 2025
From: ARKEMA FRANCE
To: ARKEMA FRANCE
Reel/Frame 071814/0739 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 14, 2020
From: FREMY, GEORGES; BARRE, PATRICE; RAYMOND, JEAN-MICHEL
To: ARKEMA FRANCE
Reel/Frame 052664/0280 →