IP Library Granted Patent US 12,402,798
Granted Patent B2
US 12,402,798 · App. 16/958,882 · Granted Sep 2, 2025

Pressure sensing layer useful in pressure sensing devices and that comprises film comprising layer of porous matrix material

Inventors: Mathieu Tauban (Lyons, FR); Mickaël Pruvost (Paris, FR); Annie Colin (Bordeaux, FR); Philippe Poulin (Talence, FR); Lise Trouillet-Fonti (Villette-de-Vienne, FR); Olivier Sanseau (Lyons, FR)
Assignees: L'ÉCOLE SUPÉRIEURE DEPHYSIQUE ET DE CHIMIEINDUSTRIELLES DE LA VILLE DE PARIS; LE CENTRE NATIONAL DE LARECHERCHE SCIENTIFIQUE
A61B5/02108A61B5/02028A61B5/02141A61B5/6802B32B5/18B32B27/065B32B27/36C08J5/18C08J9/0061C08J9/0066C08J9/009C08J9/283G01L1/146G01L1/148A61B2560/0214A61B2560/0468A61B2562/0247A61B2562/12B32B2266/0214B32B2305/022B32B2307/304B32B2457/00C08J2201/026C08J2201/0504C08J2205/044C08J2205/052C08J2205/06C08J2207/10C08J2383/07C08J2483/05C08J2483/12
View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 12,402,798
App. No.
16/958,882
Granted
Sep 2, 2025
Kind
B2
Abstract

Pressure sensing layers, devices comprising same, pressure sensing monitors and composite materials comprising a) a porous matrix material comprising a siloxane polymer, comprising a closed porosity volume fraction, and, optionally, an open porosity volume fraction, and b) a conductive or semiconductive filler substantially present in the closed porosity volume fraction of the porous matrix material a), and films, coated substrates and multilayer structures comprising the composite material and the use thereof in pressure sensing devices.

Claims (44)

1. A pressure sensing layer comprising a film comprising:

a) a first layer of porous matrix material comprising a siloxane polymer, comprising a closed porosity volume fraction, and an open porosity volume fraction, and

b) a conductive or semiconductive filler present in said closed porosity volume fraction of said first layer of porous matrix material a);

wherein at least 70% and up to 90% of the conductive or semiconductive filler is present in the closed porosity volume fraction.

2. The pressure sensing layer of claim 1 , wherein the conductive or semiconductive filler is selected from the group consisting of carbon nanotubes, carbon nanohorns, graphite, graphene and carbon black; or selected from the group consisting of metal particles and intrinsically conducting polymers (ICPs); or selected from the group consisting of Si, Si—Ge, GaAs, InP, GaN, SiC, ZnS, ZnSe, CdSe, CdS, and metal oxide particles.

3. The pressure sensing layer of claim 1 , wherein the pressure sensing layer has a thickness in the range of from 0.1 to 500 μm.

4. The pressure sensing layer in accordance with claim 1 , wherein the pressure sensing layer comprises a first layer and, adjacent thereto, a second layer which is an insulating layer.

5. The pressure sensing layer in accordance with claim 4 wherein the second layer is a polyester layer.

6. The pressure sensing layer in accordance with claim 1 , wherein the pressure sensing layer is a sensing layer for sensing low pressures.

7. A pressure sensing piezocapacitive device comprising at least one electrode and at least one pressure sensing layer in accordance with claim 1 .

8. The pressure sensing piezocapacitive device in accordance with claim 7 , wherein the pressure sensing piezocapacitive device provides a signal in response to a pressure variation wherein the pressure variation is a pulse wave event.

9. A pressure sensing monitor comprising:

a) at least one pressure sensing layer in accordance with claim 1 providing a capacitance change signal in response to a pressure variation,

b) a power supply,

c) at least one signal converting unit capable of converting the capacitance change signal provided by the pressure sensing layer into an analog or digital electric signal, optionally with filters and amplifiers for the signal,

d) at least one microcontroller unit capable of digitalizing an analog signal provided by signal converting unit c) and/or communicating digitally with the at least one signal converting unit c) and capable to convert the signal obtained from the at least one signal converting unit c) into other formats using suitable algorithms stored in the at least one controlling unit as readable code.

10. The pressure sensing monitor in accordance with claim 9 , wherein the pressure variation is a pulse wave event.

11. The pressure sensing monitor in accordance with claim 9 wherein the at least one controlling unit c) converts the signal obtained from the at least one signal converting unit b) into hemodynamic parameters.

12. The pressure sensing monitor in accordance with claim 9 , wherein the pressure sensing monitor is a wearable piezocapacitive device.

13. The pressure sensing monitor according to claim 9 , wherein the conductive or semiconductive filler of the at least one pressure sensing layer is selected from the group consisting of carbon nanotubes, carbon nanohorns, graphite, graphene and carbon black; or selected from the group consisting of metal particles and intrinsically conducting polymers (ICPs); or selected from the group consisting of Si, Si—Ge, GaAs, InP, GaN, SiC, ZnS, ZnSe, CdSe, CdS, and metal oxide particles.

14. The pressure sensing layer of claim 1 , wherein up to 99% of the total content of the conductive or semiconductive filler is present in the closed porosity volume fraction.

15. A composite material comprising:

a) a porous matrix material comprising a siloxane polymer, comprising a closed porosity volume fraction, and an open porosity volume fraction, and

b) a conductive or semiconductive filler substantially present in said closed porosity volume fraction of said porous matrix material a),

wherein at least 70% and up to 90% of the conductive or semiconductive filler is present in the closed porosity volume fraction.

16. The composite material of claim 15 , wherein the conductive or semiconductive filler is selected from the group consisting of carbon nanotubes, carbon nanohorns, graphite, graphene, carbon black, metal particles, and intrinsically conducting polymers (ICPs), or selected from the group consisting of Si, Si—Ge, GaAs, InP, GaN, SiC, ZnS, ZnSe, CdSe, CdS, and metal oxide particles.

17. A film comprising the composite material of claim 15 , wherein the film has a thickness in the range of from 0.1 to 500 μm.

18. A multilayer system comprising a first layer of a film in accordance with claim 17 and, adjacent thereto, a second layer which is an insulating layer.

19. A pressure sensing piezocapacitive device comprising the composite material in accordance with claim 15 .

20. The pressure sensing piezocapacitive device in accordance with claim 19 , wherein the pressure sensing piezocapacitive device is a blood pressure sensing device.

21. The pressure sensing piezocapacitive device according to claim 19 , wherein the conductive or semiconductive filler of the composite material is selected from the group consisting of carbon nanotubes, carbon nanohorns, graphite, graphene and carbon black; or selected from the group consisting of metal particles and intrinsically conducting polymers (ICPs); or selected from the group consisting of Si, Si—Ge, GaAs, InP, GaN, SiC, ZnS, ZnSe, CdSe, CdS, and metal oxide particles.

22. The pressure sensing piezocapacitive device according to claim 19 , comprising a film comprising:

a) a first layer of porous matrix material comprising a siloxane polymer, comprising a closed porosity volume fraction, and an open porosity volume fraction, and

b) a conductive or semiconductive filler present in said closed porosity volume fraction of said first layer of porous matrix material a) and

c) one or more additional layers;

wherein at least 70% and up to 90% of the conductive or semiconductive filler is present in the closed porosity volume fraction.

23. The pressure sensing piezocapacitive device according to claim 19 , wherein the conductive filler is selected from the group consisting of carbon nanotubes, carbon nanohorns, graphite, graphene, carbon black.

24. A process for the manufacture of a composite material in accordance with claim 15 , the process comprising the following steps:

a) providing a first non-aqueous phase comprising a siloxane polymer precursor and a curing agent and,

b) providing a second aqueous phase comprising a conductive or semiconductive filler dispersed in water,

c) preparing an emulsion by adding aqueous phase b) to the non-aqueous phase a) under stirring,

d) reticulating the product obtained in step c) and, finally,

e) subjecting the product obtained in step d) to a heat treatment to remove the water.

25. The composite material of claim 15 , wherein up to 99% of the total content of the conductive or semiconductive filler is present in the closed porosity volume fraction.

Assignments (3)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 5, 2025
From: SPECIALTY OPERATIONS FRANCE
To: L'ÉCOLE SUPÉRIEURE DE PHYSIQUE ET DE CHIMIE INDUSTRIELLES DE LA VILLE DE PARIS; LE CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE
Reel/Frame 071536/0084 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 22, 2024
From: TAUBAN, MATHIEU; PRUVOST, MICKAËL; COLIN, ANNIE; POULIN, PHILIPPE; TROUILLET-FONTI, LISE; SANSEAU, OLIVIER
To: RHODIA OPERATIONS; ECOLE SUPERIEURE DE PHYSIQUE ET DE CHIMIE INDUSTRIELLES DE LA VILLE DE PARIS; CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE
Reel/Frame 068965/0441 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 26, 2024
From: RHODIA OPERATIONS
To: SPECIALTY OPERATIONS FRANCE
Reel/Frame 066374/0642 →
Priority Claims (2)
WO PCT/EP2018/050002 · Jan 1, 2018 · international
WO PCT/EP2018/050003 · Jan 1, 2018 · international
Continuity (1)
Related Publication 20200337569A1 · Oct 29, 2020
References Cited (23)
US 8643463B2 · Samah · 2014 [cited by examiner]
US 20150320356A1 · Toth · 2015 [cited by examiner]
CN 106633891A · 2017 [cited by applicant]
KR 2016133094A · 2016 [cited by applicant]
WO 2017172978A1 · 2017 [cited by applicant]
WO WO2021107884A1 · 2021 [cited by examiner]
Pang, et al., “Highly Skin-Conformal Microhairy Sensor for Pulse Signal Amplification”, Advanced Materials, 2015, vol. 27, Issue 4, pp. 634-640. [cited by applicant]
Kwon, et al., “Highly Sensitive, Flexible, and Wearable Pressure Sensor Based on a Giant Piezocapacitive Effect of Three-Dimensional Microporous Elastomeric Dielectric Layer”, ACS Applied Materials & Interfaces, 2016, v… [cited by applicant]
Aezinia, PhD thesis, “Design of Interface Circuits for Capacitive Sensing Applications”, School of Mechatronic Systems Engineering, Faculty of Applied Sciences, Simon Fraser University, Aug. 8, 2014, pp. 22 to 27. [cited by applicant]
Cecelja, et al., “Role of Arterial Stiffness in Cardiovascular Disease”, Journal of he Royal Society of Medicine Cardiovascular Disease, 2012, 1:11, downloaded from cvd.sagepub.com at SAGE Publications on Jun. 20, 2016,… [cited by applicant]
Donley, et al., “Aerobic exercise training reduces arterial stiffness in metabolic syndrome”, Journal of Applied Physiology , vol. 116, No. 11, 2014, pp. 1396-1404. [cited by applicant]
Baruch, et al., “Validation of the pulse decomposition analysis algorithm using central arterial blood pressure”, BioMedical Engineering Online, 2014, 13:96, 19 pages. [cited by applicant]
Munir, et al., “Peripheral Augmentation Index Defines the Relationship Between Central and Peripheral Pulse Pressure”, Hypertension, http://hyper.ahajournals.org, 2008, vol. 51, Issue 1, pp. 112-118. [cited by applicant]
Lee, B-K, “Computational Fluid Dynamics in Cardiovascular Disease”, The Korean Society of Cardiology, 2011, vol. 41, Issue 8, pp. 423-430. [cited by applicant]
King, et al., “Optical blood pressure estimation with photoplethysmography and FFT-based neural networks”, Biomedical Optics Express, 2016, vol. 7. Issue 8, pp. 3007-3020. [cited by applicant]
Ananth, “Project milestone report for CS229: Blood Pressure detection from PPG signal—Sharath Ananth (SUID: sharath2)”, available online at http://cs229.stanford.edu/proj2014/Sharath%20Ananth,Blood%20Pressure%20Detectio… [cited by applicant]
Jin, et al., “Advanced Materials for Health Monitoring with Skin-Based Wearable Devices”, Advanced Healthcare Materials, 2017, vol. 6, 20 pages. [cited by applicant]
King, et al., “Porous PDMS force sensitive resistors”, Proceedings of the Eurosensors XXIII conference, Procedia Chemistry, 2009, vol. 1, Issue 1, pp. 568-571. [cited by applicant]
Dusek, et al., “Carbon Black-PDMS Composite Conformal Pressure Sensor Arrays for Near-Body Flow Detection”, EEE, Conference—Oceans—Europe > Oceans 2014—Taipei, Taiwan, Apr. 7-10, 2014, 7 pages. [cited by applicant]
Lee, B-Y, et al. “Low-cost flexible pressure sensor based on dielectric elastomer film with micro-pores—Sensors and Actuators A: Physical”, ScienceDirect, 2016, vol. 240, pp. 103-109. [cited by applicant]
Majerus, et al., “Flexible, Structured MWCNT/PDMS Sensor for Chronic Vascular Access Monitoring”, IEEE 2016 IEEE Sensors Book Series, 2016, Conference 15th IEEE Sensors, Orlando, FL., Oct. 30-Nov. 3, 2016. [cited by applicant]
Pruvost, SIMM ESPCI Lab, “Formulation of Composites for Vibrationnal Energy Harvesting”, Presentation—European Polymer Congress, Lyon, France, Jul. 2, 2017, 21 pages. [cited by applicant]
Mickael Pruvost et al.; “Polymeric foams for flexiable and highly sensitive low-pressure;” npj Flexible Electronics; Apr. 4, 2019; (6 pages). [cited by applicant]