IP Library Granted Patent US 11,873,355
Granted Patent B2
US 11,873,355 · App. 16/972,863 · Granted Jan 16, 2024

Propylene-ethylene copolymer compositions suitable for hot fill packaging of foodstuffs

Inventors: Matthew John Fedec (Columbia, MD); Jan Willem Van Egmond (Columbia, MD); Manu Rego (Columbia, MD); John Kalevi Kaarto (Columbia, MD); Li-Min Tau (Columbia, MD)
Assignee: W.R. Grace & Co.-Conn.
C08F210/06C08F210/16C08K5/053C08K5/1575C08K5/5419C08L23/14C08L23/16C08L2203/30C08L2314/02
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Quick Facts
Patent No.
US 11,873,355
App. No.
16/972,863
Granted
Jan 16, 2024
Kind
B2
Abstract

Propylene-ethylene copolymer compositions and production methods are provided. The copolymer compositions can be particularly advantageous for use in hot fill packaging of foodstuffs. The propylene-ethylene copolymers can be produced using a Ziegler-Natta catalyst and an alkoxysilane electron donor. The compositions can have propylene as a primary monomer with an ethylene content ranging from 2.0 to 6.0 percent by weight with a xylene soluble content of less than 7.0 percent by weight.

Claims (23)

1. A propylene-ethylene copolymer comprising:

propylene as a primary monomer;

an ethylene content (ET) of from 2.0% to 5% by weight;

a melt flow rate greater than 45 g/10 min and less than 100 g/10 min;

a xylene soluble fraction (XS) of from 2.0% to 7.0% by weight; and

a xylene soluble fraction to ethylene content ratio (XS/ET) of less than or equal to 1.51.

2. The propylene-ethylene copolymer of claim 1 , wherein the ethylene content is from 3.0% to 4.2% by weight.

3. The propylene-ethylene copolymer of claim 1 , wherein the ratio XS/ET is from 0.90 to 1.50.

4. The propylene-ethylene copolymer of claim 1 , wherein the ratio XS/ET is less than 1.30.

5. The propylene-ethylene copolymer of claim 1 , wherein the ratio XS/ET is less than 1.00.

6. The propylene-ethylene copolymer of claim 1 , wherein the xylene soluble fraction (XS) and the ethylene content (ET) are below a line defined by equation XS=2.1e 0.297(ET) .

7. The propylene-ethylene copolymer of claim 1 , wherein the xylene soluble fraction (XS) and the ethylene content (ET) are above a line defined by equation XS=1.4e 0.297(ET) .

8. The propylene-ethylene copolymer of claim 1 , wherein the propylene-ethylene copolymer is formed using a Ziegler-Natta catalyst and a dicyclopentyldimethoxysilane (DCPDMS) based donor.

9. The propylene-ethylene copolymer of claim 1 , wherein the propylene-ethylene copolymer is formed using a Ziegler-Natta catalyst and a n-propyltrimethoxysilane (NPTMS) based donor.

10. A polymer composition containing the propylene-ethylene copolymer of in claim 1 , wherein the propylene-ethylene copolymer is present in the polymer composition in an amount greater than about 70% by weight.

11. The polymer composition of claim 10 , further comprising a clarifying agent.

12. The polymer composition of claim 11 , wherein the clarifying agent comprises a dibenzyl sorbitol.

13. The polymer composition of claim 11 , wherein the clarifying agent comprises a nonitol.

14. The polymer composition of claim 11 , wherein the polymer composition displays a haze at 40 mil of less than about 15% and wherein after thermal aging for 24 hours at 55° C., the haze decreases by no more than about 15%.

15. An injection molded article comprising the propylene-ethylene copolymer of claim 1 .

16. The propylene-ethylene copolymer of claim 1 having a molecular weight distribution (Mw/Mn) of greater than about 3.5.

17. A hot fill packaging container comprising the propylene-ethylene copolymer of claim 1 .

18. The hot fill packaging container of claim 17 , wherein the hot fill packaging container has been formed through at least one of injection molding, blow molding, or thermoforming.

Assignments (7)
RELEASE OF SECURITY INTEREST SUPPLEMENT NO. 1, RECORDED AT REEL/FRAME 063237/0252 Recorded Feb 2, 2026
From: WILMINGTON TRUST, NATIONAL ASSOCIATION
To: W. R. GRACE & CO.-CONN.
Reel/Frame 074612/0939 →
NOTES SECURITY INTEREST Recorded Jan 29, 2026
From: W. R. GRACE & CO.-CONN.; ADVANCED REFINING TECHNOLOGIES LLC
To: WILMINGTON TRUST, NATIONAL ASSOCIATION, AS NOTES COLLATERAL AGENT
Reel/Frame 074532/0229 →
SECURITY AGREEMENT (NOTES) Recorded Aug 19, 2025
From: W. R. GRACE & CO.-CONN.
To: WILMINGTON TRUST, NATIONAL ASSOCIATION, AS NOTES COLLATERAL AGENT
Reel/Frame 072520/0653 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jul 17, 2023
From: FEDEC, MATTHEW; VAN EGMOND, JAN; REGO, MANU; KAARTO, JOHN; TAU, LI-MIN
To: W.R. GRACE & CO.-CONN.
Reel/Frame 064282/0830 →
SECURITY INTEREST Recorded Apr 2, 2023
From: W. R. GRACE & CO.-CONN.
To: JPMORGAN CHASE BANK, N.A.
Reel/Frame 063237/0262 →
SECURITY INTEREST Recorded Apr 2, 2023
From: W. R. GRACE & CO.-CONN.
To: WILMINGTON TRUST, NATIONAL ASSOCIATION
Reel/Frame 063237/0252 →
SECURITY INTEREST Recorded Feb 17, 2023
From: W.R. GRACE & CO.-CONN.
To: WILMINGTON TRUST, NATIONAL ASSOCIATION
Reel/Frame 062792/0510 →