IP Library Granted Patent US 12,410,349
Granted Patent B2
US 12,410,349 · App. 17/282,128 · Granted Sep 9, 2025

Aqueous binder composition

Inventors: Dorte Bartnik Johansson (Roskilde, DK); Ib Johannsen (Aarhus, DK); Bjørn Sjøgren Kilsgaard (Aarhus C, DK); Miroslav Nikolic (Aarhus C, DK)
Assignee: Rockwool A/S
C09J197/005C03C25/25C03C25/328C03C25/36C07G1/00D04H1/4209D04H1/587D04H1/64
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Quick Facts
Patent No.
US 12,410,349
App. No.
17/282,128
Granted
Sep 9, 2025
Kind
B2
Abstract

The invention is directed to an aqueous binder composition for mineral fibers.

Claims (49)

1. A mineral fiber product, wherein the product comprises mineral fibers in contact with a binder resulting from curing an aqueous binder composition which comprises:

a component (i) in the form of one or more oxidized lignins;

a component (ii) in the form of one or more cross-linkers;

a component (iii) in the form of one or more plasticizers.

2. The mineral fiber product of claim 1 , wherein

component (i) is in the form of one or more oxidized lignins, the lignins being selected from kraft

lignins, soda lignins, lignosulfonate lignins, organosolv lignins, lignins from biorefining processes of lignocellulosic feedstocks, or any mixture thereof.

3. The mineral fiber product of claim 1 , wherein component (i) is in the form of one or more oxidized kraft lignins.

4. The mineral fiber product of claim 1 , wherein component (i) is in the form of one or more oxidized soda lignins.

5. The mineral fiber product of claim 1 , wherein component (i) is in the form of one or more ammonia-oxidized lignins.

6. The mineral fiber product of claim 5 , wherein the ammonia-oxidized lignin comprises one or more compounds selected from ammonia, amines, or any salts thereof.

7. The mineral fiber product of claim 1 , wherein component (i) has a carboxylic acid group content of from 0.05 to 10 mmol/g, based on a dry weight of component (i).

8. The mineral fiber product of claim 1 , wherein component (i) has an average carboxylic acid group content of more than 1.5 groups per macromolecule of component (i).

9. The mineral fiber product of claim 1 , wherein component (ii) is in the form of one or more cross-linkers selected from β-hydroxyalkylamide-cross-linkers and oxazoline-cross-linkers.

10. The mineral fiber product of claim 1 , wherein component (ii) comprises one or more cross-linkers selected from multifunctional organic amines.

11. The mineral fiber product of claim 1 , wherein component (ii) comprises one or more flexible oligomers or polymers or an epoxidized oil based on a fatty acid triglyceride.

12. The mineral fiber product of claim 1 , wherein component (ii) comprises a molecule having 3 or more epoxy groups.

13. The mineral fiber product of claim 1 , wherein component (ii) is present in a concentration of from 1 to 40 wt.-%, based on a dry weight of component (i).

14. The mineral fiber product of claim 1 , wherein component (iii) comprises one or more plasticizers selected from polyethylene glycols, polyethylene glycol ethers, polyethers, hydrogenated sugars, phthalates and/or acids, acrylic polymers, polyvinyl alcohol, polyurethane dispersions, ethylene carbonate, propylene carbonate, lactones, lactams, lactides, acrylic based polymers with free carboxy groups and/or polyurethane dispersions with free carboxy groups.

15. The mineral fiber product of claim 1 , wherein component (iii) comprises one or more plasticizers having a boiling point of from 100° C. to 280° C.

16. The mineral fiber product of claim 1 , wherein component (iii) comprises one or more polyethylene glycols having an average molecular weight of from 150 to 50,000 g/mol.

17. The mineral fiber product of claim 1 , wherein component (iii) is present in a concentration of from 0.5 to 50 wt.-%, based on a dry weight of component (i).

18. The mineral fiber product of claim 1 , wherein the binder composition consists essentially of

a component (i) in the form of one or more oxidized lignins;

a component (ii) in the form of one or more cross-linkers;

a component (iii) in the form of one or more plasticizers;

a component (iv) in the form of one or more coupling agents;

optionally a component in the form of one or more compounds selected from ammonia, amines, or any salts thereof;

optionally a component in the form of urea;

optionally a component in the form of one or more reactive or non-reactive silicones;

optionally a hydrocarbon oil;

optionally one or more surface active agents;

water.

19. A method of producing a bonded mineral fiber product, wherein the method comprises contacting mineral fibers with an aqueous binder composition and curing the binder composition, the binder composition comprising:

a component (i) in the form of one or more oxidized lignins;

a component (ii) in the form of one or more cross-linkers;

a component (iii) in the form of one or more plasticizers.

20. An aqueous binder composition, wherein the composition in its cured state is capable of binding mineral fibers to afford a bonded mineral fiber product, and comprises:

a component (i) in the form of one or more oxidized lignins;

a component (ii) in the form of one or more cross-linkers;

a component (iii) in the form of one or more plasticizers.

21. The mineral fiber product of claim 1 , wherein component (iii) comprises one or more polyethylene glycols.

22. The mineral fiber product of claim 1 , wherein component (i) is in the form of one or more oxidized lignins, the lignins being selected from kraft lignins, soda lignins, organosolv lignins, lignins from Biorefining processes of lignocellulosic feedstocks, or any mixture thereof.

23. The mineral fiber product of claim 1 , wherein component (ii) is in the form of one or more cross-linkers selected from β-hydroxyalkylamide-cross-linkers and/or oxazoline-cross-linkers, one or more flexible oligomers or polymers, an epoxidized oil based on a fatty acid triglyceride, and a molecule having 3 or more epoxy groups, and component (iii) is in the form of one or more plasticizers comprising one or more polyethylene glycols.

24. The mineral fiber product of claim 23 , wherein component (iii) comprises one or more polyethylene glycols having an average molecular weight of 150 to 50,000 g/mol.

25. The mineral fiber product of claim 23 , wherein component (ii) is in the form of one or more cross-linkers selected from β-hydroxyalkylamide-cross-linkers and/or oxazoline-cross-linkers.

26. The mineral fiber product of claim 23 , wherein component (i) is in the form of one or more oxidized lignins, the lignins being selected from kraft lignins, soda lignins, organosolv lignins, lignins from Biorefining processes of lignocellulosic feedstocks, or any mixture thereof.

27. The mineral fiber product of claim 23 , wherein component (i) is in the form of one or more oxidized kraft lignins or one or more oxidized soda lignins.

28. The mineral fiber product of claim 1 , wherein component (ii) is in the form of one or more cross-linkers selected from β-hydroxyalkylamide-cross-linkers and/or oxazoline-cross-linkers, and component (iii) is in the form of one or more plasticizers comprising one or more polyethylene glycols having an average molecular weight of 150 to 50,000 g/mol.

Assignments (2)
CHANGE OF NAME Recorded Aug 4, 2023
From: ROCKWOOL INTERNATIONAL A/S
To: ROCKWOOL A/S
Reel/Frame 064502/0506 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jul 8, 2021
From: JOHANSSON, DORTE BARTNIK; JOHANNSEN, IB; KILSGAARD, BJØRN SJØGREN; NIKOLIC, MIROSLAV
To: ROCKWOOL INTERNATIONAL A/S
Reel/Frame 056797/0818 →
Priority Claims (1)
EP 18198999 · Oct 5, 2018 · regional
Continuity (1)
Related Publication 20220106508A1 · Apr 7, 2022
References Cited (73)
US 3093604A · Ayers · 1963 [cited by applicant]
US 3227667A · Moffitt et al. · 1966 [cited by applicant]
US 3285801A · Sarjeant · 1966 [cited by applicant]
US 5318990A · Strauss · 1994 [cited by applicant]
US 6238475B1 · Gargulak et al. · 2001 [cited by applicant]
US 6706853B1 · Stanssens et al. · 2004 [cited by applicant]
US 6818699B2 · Kajimaru et al. · 2004 [cited by applicant]
US 7265169B2 · Li et al. · 2007 [cited by applicant]
US 20040034154A1 · Tutin et al. · 2004 [cited by applicant]
US 20070077837A1 · Lundquist · 2007 [cited by examiner]
US 20070173588A1 · Espiard et al. · 2007 [cited by applicant]
US 20090098387A1 · Brady et al. · 2009 [cited by applicant]
US 20090169867A1 · Kelly · 2009 [cited by applicant]
US 20100069533A1 · Brady et al. · 2010 [cited by applicant]
US 20100112242A1 · Medoff · 2010 [cited by applicant]
US 20110054154A1 · Park · 2011 [cited by examiner]
US 20110086567A1 · Hawkins et al. · 2011 [cited by applicant]
US 20110159768A1 · Crescimanno et al. · 2011 [cited by applicant]
US 20130065012A1 · Parker et al. · 2013 [cited by examiner]
US 20140030540A1 · Valkonen · 2014 [cited by applicant]
US 20140163142A1 · Zhang et al. · 2014 [cited by applicant]
US 20160168435A1 · Amen-Chen · 2016 [cited by examiner]
US 20160244364A1 · Kalliola et al. · 2016 [cited by applicant]
US 20180312625A1 · Phanopoulos et al. · 2018 [cited by applicant]
US 20190136062A1 · Alvarado et al. · 2019 [cited by applicant]
US 20190338168A1 · Laine et al. · 2019 [cited by applicant]
US 20190390374A1 · Fournier et al. · 2019 [cited by applicant]
CN 107286873A · 2017 [cited by examiner]
CN 107459385A · 2017 [cited by applicant]
CN 107556946A · 2018 [cited by examiner]
EP 0583086A · 1994 [cited by applicant]
EP 0990727A1 · 2000 [cited by applicant]
EP 1741726A1 · 2007 [cited by applicant]
EP 3299421A1 · 2018 [cited by applicant]
JP 2014065779A · 2014 [cited by applicant]
RU 2345112C2 · 2009 [cited by applicant]
WO 9831763A1 · 1998 [cited by applicant]
WO 9936368A1 · 1999 [cited by applicant]
WO 0105725A1 · 2001 [cited by applicant]
WO 0196460A2 · 2001 [cited by applicant]
WO 0206178A1 · 2002 [cited by applicant]
WO 2004007615A1 · 2004 [cited by applicant]
WO 2006061249A1 · 2006 [cited by applicant]
WO 2008023032A1 · 2008 [cited by applicant]
WO 2008073186A2 · 2008 [cited by applicant]
WO 2011042610A1 · 2011 [cited by applicant]
WO 2012113058A1 · 2012 [cited by applicant]
WO 2012136894A1 · 2012 [cited by applicant]
WO 2014080033A1 · 2014 [cited by applicant]
WO 2015049424A1 · 2015 [cited by applicant]
WO 2016009054A1 · 2016 [cited by applicant]
WO 2017067769A1 · 2017 [cited by applicant]
WO 2017188874A1 · 2017 [cited by applicant]
WO 2018122470A1 · 2018 [cited by applicant]
WO 2018138450A1 · 2018 [cited by applicant]
English Machine Translation of CN107286873 ( A ) obtained on Nov. 1, 2023 https://worldwide.espacenet.com/publicationDetails/biblio?CC=CN&NR=107286873A&KC=A&FT=D&ND=3&date=20171024&DB=EPODOC&locale=en_EP (Year: 2017). [cited by examiner]
English Machine Translation of CN107556946 ( A ) obtained on Nov. 7, 2023 https://worldwide.espacenet.com/publicationDetails/biblio?ll=0&ND=3&adjacent=true&locale=en_EP&FT=D&date=20180109&CC=CN&NR=107556946A&KC=A (Year:… [cited by examiner]
English Machine Translation of EP3299421 ( A1 ) obtained on Nov. 7, 2023 https://worldwide.espacenet.com/publicationDetails/description?CC=EP&NR=3299421A1&KC=A1&FT=D&ND=3&date=20180328&DB=EPODOC&locale=en_EP (Year: 2018… [cited by examiner]
Chen et al. (Journal of applied Polymer Science, vol. 42, 2073-2079 (1991)) (Year: 1991). [cited by examiner]
Bouajila et al., “Some Laws of Lignin Plasticization”, Journal of Applied Polymer Science, vol. 102, 2006, pp. 1445-1451. [cited by applicant]
Urkhanova et al., “Fiber-reinforced concrete with mineral fibers and nanosilica”, Procedia Engineering 195 (Jul. 20, 2017), pp. 147-154. [cited by applicant]
Xiangwei Zhu et al., “Bio-Based Wood Adhesive from Camelina Protein (a Biodiesel Residue) and Depolymerized Lignin with Improved Water Resistance”, ACS Omega, (Nov. 16, 2017), vol. 2, No. 11, ISSN 2470-1343, pp. 7996-80… [cited by applicant]
Richard J.A. Gosselink et al., “Effect of periodate on lignin for wood adhesive application”, Holzforschung: International Journal of the Biology, Chemistry, Physics and Technology of Wood, DE, (Jan. 1, 2011), vol. 65, … [cited by applicant]
Venla Hemmila et al., “Lignin: an adhesive raw material of the future or waste of research energy?”, Northern European Network for Wood Science and Engineering (WSE), (Jan. 1, 2013), pp. 98-103. [cited by applicant]
Masoumeh Ghorbani et al., “Ammoxidized Fenton-Activated Pine Kraft Lignin Accelerates Synthesis and Curing of Resole Resins”, Polymers, (Jan. 28, 2017), vol. 9, No. 12, p. 43, p. 54, p. 55. [cited by applicant]
Dietrich Meier et al., “Conversion of technical lignins into slow-release nitrogenous fertilizers by ammoxidation in liquid phase”, Bioresource Technology, (Jan. 1, 1994), pp. 121-128. [cited by applicant]
U.S. Appl. No. 17/282,126, filed Apr. 1, 2021. [cited by applicant]
U.S. Appl. No. 17/282,130, filed Apr. 1, 2021. [cited by applicant]
U.S. Appl. No. 17/282,131, filed Apr. 1, 2021. [cited by applicant]
“Properties of Hydrogen Peroxide”, Editorial board of «Inorganic Chemistry», «Inorganic Chemistry vol. II», Peoples Education Press, 1st Edition, 2nd Print, Oct. 1978, pp. 82-83 (CN). [cited by applicant]
Tsuneo Koike, “Progress in Development of Epoxy Resin Systems Based on Wood Biomass in Japan”, Polymer Engineering and Science, 2012, 701-717. [cited by applicant]
Ajinkya More, “A review of lignin hydrogen peroxide oxidation chemistry with emphasis on aromatic aldehyde and acids”, Lignin hydrogen peroxide oxidation chemistry, published Mar. 17, 2021. [cited by applicant]
“Chemoselective Metal-Free Aerobic Alcohol Oxidation in Lignin”, J. Am. Chem. Soc. 2013, 135, pp. 6415-6418. [cited by applicant]