IP Library Granted Patent US 12,441,881
Granted Patent B2
US 12,441,881 · App. 17/446,211 · Granted Oct 14, 2025

Thermal interface materials

Inventors: Chunyong Wu (Plymouth, MN); John Timmerman (Minneapolis, MN); Reid Chesterfield (Eden Prairie, MN); Radesh Jewram (Lakeville, MN)
Assignee: Henkel AG & Co. KGaA
C08L71/00C08G65/336C08K3/22C08K3/36C08K5/0016C08K5/005C08K5/57H01M10/659C08K2003/2227C08K2201/001C08K2201/005
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Quick Facts
Patent No.
US 12,441,881
App. No.
17/446,211
Granted
Oct 14, 2025
Kind
B2
Abstract

A thermally conductive curable composition includes a first part and a second part, wherein the first part comprises a catalyst, a ceramic filler mixture, a low volatile organic liquid, and water, and the second part comprises a silyl modified reactive polymer, a low volatile organic liquid, and the ceramic filler mixture, and the low volatile organic liquid is present in the composition in an amount greater than about 50 wt. % based on the total weight of the silyl modified reactive polymer.

Claims (21)

1. A thermally conductive curable composition comprising a first part and a second part,

wherein the first part comprises a catalyst, a ceramic filler mixture, a low volatile organic liquid, and water,

wherein the second part comprises a silane modified polyether, a low volatile organic liquid, and a ceramic filler mixture,

wherein the low volatile organic liquid has a viscosity of less than 100 cPs, and is present in the composition in an amount greater than about 50 wt. % based on the total weight of the silane modified polyether, and wherein the silane modified polyether is present in an amount of between 1.7 wt. % and 6.5 wt. % based on the total weight of the second part, and wherein the first part and the second part are present in the curable composition in a ratio of about 1:1.

2. The thermally conductive curable composition of claim 1 , wherein the silane modified polyether is dimethoxysilane modified polyether, trimethoxysilane modified polyether, triethoxysilane modified polyether, or a combination thereof.

3. The thermally conductive curable composition of claim 1 , wherein the water is present in the first part in an amount from 500 ppm to 5000 ppm based on the total weight of the first part.

4. The thermally conductive curable composition of claim 1 , wherein the second part further comprises a water scavenger in an amount of between 1 wt. % and 5 wt. % based on the total weight of the silane modified polyether.

5. The thermally conductive curable composition of claim 1 , wherein the first part and/or the second part further comprises a rheology additive.

6. The thermally conductive curable composition of claim 1 , wherein the catalyst is an organotin catalyst, an organobismuth catalyst, or a combination thereof.

7. The thermally conductive curable composition of claim 1 , wherein the first part and the second part have a viscosity at 1/s above 300 Pas and a viscosity at 3000/s below 50 Pas.

8. The thermally conductive curable composition of claim 1 , wherein the ceramic filler mixture is present in each of the first part and the second part in an amount from about 80 wt. % to about 95 wt. % based on the total weight of each of the first part and the second part.

9. The thermally conductive curable composition of claim 1 , wherein the ceramic filler mixture comprises a first ceramic filler having a D50 of 2.4 μm, a second ceramic filler having a D50 of 40 μm, and a third ceramic filler having a D50 of 0.3 μm.

10. The thermally conductive curable composition of claim 9 , wherein the first ceramic filler is present in the composition in an amount of about 4 wt. % based on the total weight of the ceramic filler mixture, the second ceramic filler is present in an amount of about 36 wt. % based on the total weight of the ceramic filler mixture, and the third ceramic filler is present in an amount of about 60 wt. % based on the total weight of the ceramic filler mixture.

11. A method of making the thermally conductive curable composition of claim 1 , the method comprising:

mixing the first part with the second part,

wherein the mixture is a solid after cure.

12. The method of claim 11 , wherein the mixture is cured at room temperature.

13. The method of claim 12 , wherein after cure the composition has a thermal conductivity of about 2.0 to about 5.0 W/mK.

14. The method of claim 12 , wherein the first part and the second part are mixed in a ratio of about 1:1.

15. A battery comprising:

a heat source, a cooling mechanism and the composition of claim 1 disposed therebetween.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 15, 2025
From: WU, CHUNYONG; TIMMERMAN, JOHN; CHESTERFIELD, REID; JEWRAM, RADESH
To: HENKEL IP & HOLDING GMBH
Reel/Frame 072253/0821 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 22, 2022
From: HENKEL IP & HOLDING GMBH
To: HENKEL AG & CO. KGAA
Reel/Frame 059207/0627 →
Continuity (3)
Continuation PCTUS2020019888 · Feb 26, 2020
Provisional Application 62811074 · Feb 27, 2019
Related Publication 20210388203A1 · Dec 16, 2021
References Cited (11)
US 5648427A · Fujita · 1997 [cited by examiner]
US 20070088110A1 · Kohl et al. · 2007 [cited by applicant]
US 20110311767A1 · Elahee et al. · 2011 [cited by applicant]
US 20130178560A1 · Hersee et al. · 2013 [cited by applicant]
US 20180076493A1 · Park et al. · 2018 [cited by applicant]
US 20180251590A1 · Kunitomo et al. · 2018 [cited by applicant]
JP 2002309077A · 2002 [cited by examiner]
WO WO2013051721A1 · 2013 [cited by examiner]
English translation of WO-2013051721-A1 (Year: 2013). [cited by examiner]
English translation of JP-2002309077-A (Year: 2002). [cited by examiner]
Univar Solutions, Dioctyl Adipate Safety Data Sheet (Year: 1). [cited by examiner]