IP Library Granted Patent US 11,739,108
Granted Patent B2
US 11,739,108 · App. 17/479,144 · Granted Aug 29, 2023

Diphosphites having an open, 2,4-methylated outer unit

Inventors: Anna Chiara Sale (Recklinghausen, DE); Robert Franke (Marl, DE); Alexander Brächer (Haltern am See, DE); Dirk Fridag (Haltern am See, DE); Johannes Knossalla (Gahlen, DE)
Assignee: EVONIK OPERATIONS GMBH
C07F9/65746B01J31/185B01J2231/321B01J2531/821B01J2531/822B01J2531/827B01J2531/845
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Quick Facts
Patent No.
US 11,739,108
App. No.
17/479,144
Granted
Aug 29, 2023
Kind
B2
Abstract

Diphosphites having an open, 2,4-methylated outer unit and use thereof in hydroformylation.

Claims (22)

1. A compound having structure (I):

where R 1 and R 3 are selected from: —H, —(C 1 -C 12 )-alkyl or —O—(C 1 -C 12 )-alkyl and where R 2 and R 4 are selected from: —H or —O—(C 1 -C 12 ) alkyl.

2. The compound according to claim 1 ,

where R 1 and R 3 are selected from: —H or —(C 1 -C 12 )-alkyl.

3. The compound according to claim 1 ,

where R 1 and R 3 are —(C 1 -C 12 )-alkyl.

4. The compound according to claim 1 ,

where R 1 and R 3 are the same radical.

5. The compound according to claim 1 ,

wherein R 2 and R 4 are —O—(C 1 -C 12 )-alkyl.

6. The compound according to claim 1 ,

where R 2 and R 4 are the same radical.

7. The compound according to claim 1 ,

where R 1 , R 2 , R 3 and R 4 are not all simultaneously —CH 3 .

8. The compound according to claim 1 ,

where the compound has the structure (1):

9. A ligand-metal complex comprising a compound according to claim 1 and a metal selected from: Rh, Ru, Co or Ir.

10. A process comprising the process steps of:

a) initially charging an olefin,

b) adding a compound according to claim 1 and a substance containing a metal selected from: Rh, Ru, Co or Ir,

c) supplying H 2 and CO, and

d) heating the reaction mixture from steps a) to c), with conversion of the olefin to an aldehyde.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 9, 2024
From: EVONIK OPERATIONS GMBH
To: EVONIK OXENO GMBH & CO. KG
Reel/Frame 066242/0585 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 31, 2022
From: SALE, ANNA CHIARA; FRANKE, ROBERT; BRÄCHER, ALEXANDER; FRIDAG, DIRK; KNOSSALLA, JOHANNES
To: EVONIK OPERATIONS GMBH
Reel/Frame 060059/0194 →
Priority Claims (1)
EP 20197484 · Sep 22, 2020 · regional
Continuity (1)
Related Publication 20220089623A1 · Mar 24, 2022