IP Library Granted Patent US 11,781,400
Granted Patent B2
US 11,781,400 · App. 17/646,807 · Granted Oct 10, 2023

Nanoparticle-based shear-thickening materials

Inventors: Abeer Mohammad Saleh Al-Olayan (Dammam, SA); Alfredo Alexander-Katz (Cambridge, MA); Jason R. Cox (Ashland, MA)
Assignees: Saudi Arabian Oil Company; Massachusetts Institute of Technology, aka MIT
E21B33/14C04B24/42C04B28/02C04B40/0039C09K8/42C09K8/467C09K8/506C09K8/516C09K8/588C09K2208/10
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Quick Facts
Patent No.
US 11,781,400
App. No.
17/646,807
Granted
Oct 10, 2023
Kind
B2
Abstract

A composition includes an aqueous colloidal dispersion of a nanomaterial. The nanomaterial includes, disposed on a surface of the nanomaterial, a first coupling agent including silane and a functional group including an amino acid. The nanomaterial includes, disposed on the surface of the nanomaterial, a second coupling agent including silane and a polymer with a molecular weight between 1,000 and 20,000.

Claims (15)

1. A method comprising:

forming a nanomaterial, wherein an average particle size of the nanomaterial is equal to or less than approximately 1 μm, the forming comprising:

disposing, on a surface of a silica nanoparticle, a first coupling agent comprising a silane having a functional group comprising an amino acid; and

disposing, on the surface of the silica nanoparticle, a second coupling agent comprising a silane coupled to a polymer with a molecular weight between 1,000 and 20,000; and

dispersing the nanomaterial in a fluid comprising water to form an aqueous colloidal dispersion, wherein the aqueous colloidal dispersion is a shear-thickening material.

2. The method of claim 1 , wherein the amino acid is a polar amino acid.

3. The method of claim 1 , wherein the polymer is polyethylene glycol or polyethylene oxide.

4. The method of claim 1 , wherein a ratio between the first coupling agent and the second coupling agent disposed on the surface of the silica nanoparticle is between 1:1 and 20:1.

5. A method comprising introducing an aqueous colloidal dispersion to a subterranean zone, the aqueous colloidal dispersion comprising a nanomaterial including, disposed on a surface thereof:

a first coupling agent comprising a silane having a functional group comprising an amino acid; and

a second coupling agent comprising a silane coupled to a polymer with a molecular weight between 1,000 and 20,000, wherein the aqueous colloidal dispersion is a shear-thickening material.

6. The method of claim 5 , wherein a ratio between the first coupling agent and the second coupling agent disposed on the surface of the nanomaterial is between 1:1 and 20:1.

7. The method of claim 5 , further comprising mixing the aqueous colloidal dispersion with a cement before introducing the aqueous colloidal dispersion to the subterranean zone.

8. The method of claim 5 , wherein the aqueous colloidal dispersion is a shear-thickening material, and applying a shear on the aqueous colloidal dispersion causes a viscosity of the aqueous colloidal dispersion to reversibly increase by a factor of 1.1 to 3.

9. The method of claim 5 , wherein heating the aqueous colloidal dispersion to above 90° C. causes a viscosity of the aqueous colloidal dispersion to reversibly increase by a factor of 1.5 to 15.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 4, 2022
From: ALEXANDER-KATZ, ALFREDO
To: MASSACHUSETTS INSTITUTE OF TECHNOLOGY
Reel/Frame 058540/0307 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 4, 2022
From: AL-OLAYAN, ABEER MOHAMMAD SALEH; COX, JASON R.
To: SAUDI ARABIAN OIL COMPANY
Reel/Frame 058540/0368 →
Continuity (4)
Continuation 16654678 · Oct 16, 2019
Division 15812720 · Nov 14, 2017
Provisional Application 62422250 · Nov 15, 2016
Related Publication 20220127927A1 · Apr 28, 2022