IP Library Granted Patent US 11,618,760
Granted Patent B2
US 11,618,760 · App. 17/718,525 · Granted Apr 4, 2023

Diphosphites with an open, 3-methylated outer unit

Inventors: Anna Chiara Sale (Recklinghausen, DE); Robert Franke (Marl, DE); Alexander Brächer (Haltern am See, DE); Dirk Fridag (Haltern am See, DE); Ana Markovic (Haltern am See, DE); Peter Kucmierczyk (Herne, DE); Johannes Knossalla (Gahlen, DE)
Assignee: EVONIK OPERATIONS GMBH
C07F9/062
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Quick Facts
Patent No.
US 11,618,760
App. No.
17/718,525
Granted
Apr 4, 2023
Kind
B2
Abstract

Diphosphites having an open, 3-methylated outer unit and use thereof in hydroformylation.

Claims (22)

1. A compound of the structure (I):

where R 1 , R 2 , R 3 , R 4 are selected from: —H, —(C 1 -C 12 )-alkyl, —O—(C 1 -C 12 )-alkyl.

2. The compound according to claim 1 ,

wherein R 1 , R 3 are selected from: —H, —(C 1 -C 12 )-alkyl.

3. The compound according to claim 1 ,

where R 3 are —(C 1 -C 12 )-alkyl.

4. The compound according to claim 1 ,

where R 1 , R 3 are the same radical.

5. The compound according to claim 1 ,

wherein R 2 , R 4 are selected from: —H, —O—(C 1 -C 12 )-alkyl.

6. The compound according to claim 1 ,

wherein R 2 , R 4 are —O—(C 1 -C 12 )-alkyl.

7. The compound according to claim 1 ,

where R 2 , R 4 are the same radical.

8. The compound according to claim 1 ,

where the compound has the structure (1):

9. A ligand-metal complex comprising the compound according to claim 1 and a metal selected from: Rh, Ru, Co or Ir.

10. A process comprising the process steps of:

a) initially charging an olefin,

b) adding a compound according to claim 1 and a substance containing a metal selected from: Rh, Ru, Co or Ir,

c) supplying H 2 and CO, and

d) heating the reaction mixture from steps a) to c), to convert the olefin into an aldehyde.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 9, 2024
From: EVONIK OPERATIONS GMBH
To: EVONIK OXENO GMBH & CO. KG
Reel/Frame 066242/0585 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 9, 2023
From: SALE, ANNA CHIARA; FRANKE, ROBERT; BRÄCHER, ALEXANDER; FRIDAG, DIRK; MARKOVIC, ANA; KUCMIERCZYK, PETER; KNOSSALLA, JOHANNES
To: EVONIK OPERATIONS GMBH
Reel/Frame 062310/0660 →