IP Library Granted Patent US 12,624,136
Granted Patent B2
US 12,624,136 · App. 18/011,701 · Granted May 12, 2026

Phthalate-free polypropylene homopolymer having high stiffness properties

Inventor: Zhiru Ma (Ellicott City, MD)
Assignee: W.R. Grace & Co.- Conn
C08F110/06C08J3/12C08L23/12C08J2323/12C08J2423/12C08L2205/025
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Quick Facts
Patent No.
US 12,624,136
App. No.
18/011,701
Granted
May 12, 2026
Kind
B2
Abstract

Phthalate-free polypropylene homopolymers and compositions incorporating the homopolymers are described. The phthalate-free polypropylene homopolymers exhibit high molecular weight as well as low XS content. Composition incorporating the phthalate-free polypropylene homopolymer can have relatively high stiffness properties. In addition, the polypropylene compositions can have good melt flow characteristics. Phthalate-free compositions including the homopolymers can be advantageously utilized in forming containers and other articles in food contacting, medical, and personal care applications.

Claims (19)

1 . A polypropylene homopolymer, wherein the polypropylene homopolymer has a weight average molecular weight of 150,000 or greater, a melting temperature of about 160° C. or greater, a molecular weight distribution of 5 or greater, and a xylene soluble content of 1.8% by weight or less, and wherein the polypropylene homopolymer is produced with a Ziegler-Natta catalyst and is phthalate-free.

2 . The polypropylene homopolymer of claim 1 , wherein the polypropylene homopolymer has an XS content of from 0.5% by weight to 1.5% by weight.

3 . The polypropylene homopolymer of claim 1 , wherein the polypropylene homopolymer has a weight average molecular weight of 200000 or greater.

4 . The polypropylene homopolymer of claim 1 , wherein the polypropylene homopolymer has a weight average molecular weight of 350000 or greater.

5 . The polypropylene homopolymer of claim 1 , wherein the polypropylene homopolymer has a molecular weight distribution of 5.5 or greater.

6 . The polypropylene homopolymer of claim 1 , wherein the polypropylene homopolymer has one or more of an isotactic pentad content of 95% or greater, an isotactic triad content of 97% or greater, an isotactic block length of 150 or greater, and a meso run length of 100 or greater.

7 . The polypropylene homopolymer of claim 1 , wherein the polypropylene homopolymer has a melting temperature of 164° C. or greater.

8 . The polypropylene homopolymer of claim 1 , wherein the polypropylene homopolymer has a crystallization temperature of 120° C.

9 . The polypropylene homopolymer of claim 1 , wherein the polypropylene homopolymer is formed in a gas phase reactor.

10 . A composition comprising the phthalate-free polypropylene homopolymer of claim 1 , wherein the composition has a flexural modulus of about 1700 MPa or greater, and a melt flow rate of about 1 g/10 min or greater and about 10 g/10 min or less.

11 . The composition of claim 10 , wherein the composition has an Izod impact strength of 10 J/m or greater.

12 . The composition of claim 10 , wherein the composition has a tensile strength at yield of 20 MPa or greater.

13 . The composition of claim 10 , wherein the composition comprises a nucleating agent.

14 . The composition of claim 10 , wherein the composition does not include a nucleating agent.

15 . The composition of claim 10 , wherein the composition comprises one or more of a mold release agent, a slip agent, an antiblock, a UV stabilizer, a heat stabilizer, a clarifying agent, an antioxidant, an acid scavenger, or a colorant.

16 . The composition of claim 10 , wherein the composition comprises a second polymer.

17 . A molded article comprising the composition of claim 10 .

18 . The molded article of claim 17 , wherein the molded article is a container.

19 . The molded article of claim 17 , wherein the molded article is a food contact article, a medical care article, or a personal care article.

Assignments (7)
RELEASE OF SECURITY INTEREST SUPPLEMENT NO. 1, RECORDED AT REEL/FRAME 063237/0252 Recorded Feb 2, 2026
From: WILMINGTON TRUST, NATIONAL ASSOCIATION
To: W. R. GRACE & CO.-CONN.
Reel/Frame 074612/0939 →
NOTES SECURITY INTEREST Recorded Jan 29, 2026
From: W. R. GRACE & CO.-CONN.; ADVANCED REFINING TECHNOLOGIES LLC
To: WILMINGTON TRUST, NATIONAL ASSOCIATION, AS NOTES COLLATERAL AGENT
Reel/Frame 074532/0229 →
SECURITY AGREEMENT (NOTES) Recorded Aug 19, 2025
From: W. R. GRACE & CO.-CONN.
To: WILMINGTON TRUST, NATIONAL ASSOCIATION, AS NOTES COLLATERAL AGENT
Reel/Frame 072520/0653 →
SECURITY INTEREST Recorded Apr 2, 2023
From: W. R. GRACE & CO.-CONN.
To: JPMORGAN CHASE BANK, N.A.
Reel/Frame 063237/0262 →
SECURITY INTEREST Recorded Apr 2, 2023
From: W. R. GRACE & CO.-CONN.
To: WILMINGTON TRUST, NATIONAL ASSOCIATION
Reel/Frame 063237/0252 →
SECURITY INTEREST Recorded Feb 17, 2023
From: W.R. GRACE & CO.-CONN.
To: WILMINGTON TRUST, NATIONAL ASSOCIATION
Reel/Frame 062792/0510 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 20, 2022
From: MA, ZHIRU
To: W.R. GRACE & CO.-CONN.
Reel/Frame 062160/0554 →
Continuity (2)
Provisional Application 63045348 · Jun 29, 2020
Related Publication 20230312782A1 · Oct 5, 2023
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