IP Library Granted Patent US 10,655,232
Granted Patent B2
US 10,655,232 · App. 15/870,297 · Granted May 19, 2020

Additives to control hydrogen sulfide release of sulfur containing and/or phosphorus containing corrosion inhibitors

Inventors: Vaithilingam Panchalingam (Friendswood, TX); Bradley G. Harrell (Pearland, TX)
Assignee: Baker Hughes, a GE company, LLC
C23F11/1673C09K8/54C23F11/10C23F11/141C23F11/149C09K2208/20C09K2208/32E21B41/02
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Quick Facts
Patent No.
US 10,655,232
App. No.
15/870,297
Granted
May 19, 2020
Kind
B2
Abstract

An additive, such as an aminal, a dibutylamine, or combinations thereof, may treat a system having a corrosion inhibitor in the form of at least one sulfur species and/or at least one phosphorous-containing compound. The additive may be introduced or added to the corrosion inhibitor within an aqueous system, an aerobic system, and/or an anaerobic system to inactivate the sulfur species and/or the phosphorous-containing compounds.

Claims (26)

1. A treated system comprising:

a system containing fluid selected from the group consisting of an aqueous system, an aerobic system, an anaerobic system, and combinations thereof; and

a corrosion inhibitor comprising (1) at least one phosphorous-containing compound selected from the group consisting of O,O-disubstituted dithiophosphoric acid, pyrophosphates, and combinations thereof and

(2) at least one additive selected from the group consisting of an aminal, a dialkylamine, and combinations thereof;

wherein the aminal has a formula of (R1)(R2)N—CH 2 —N(R3)(R4) where each of R1-R4 is an alkyl group, an aryl group, a substituted aryl group, and/or an alkylalkoxylate, and where R1, R2, R3, and R4 are the same or different.

2. The treated system of claim 1 , wherein the amount of the additive present in the treated system ranges from about 1 wt % to about 15 wt % based on the total amount of fluid in the system.

3. The treated system of claim 1 , wherein the corrosion inhibitor further comprises at least one sulfur species.

4. The treated system of claim 3 , further comprising a first reaction product produced from a first reaction between the at least one additive and the at least one sulfur species.

5. The treated system of claim 4 , further comprising a second reaction product produced from a second reaction between the first reaction product and the at least one phosphorous containing compound.

6. The treated system of claim 5 , wherein the second reaction product is a stable reaction product.

7. A treated system comprising:

a system selected from the group consisting of an aqueous system, an aerobic system, an anaerobic system, and combinations thereof; and

a corrosion inhibitor comprising at least one sulfur species and at least one phosphorous-containing compound selected from the group consisting of O,O-disubstituted dithiophosphoric acid, pyrophosphates, and combinations thereof;

at least one additive selected from the group consisting of an aminal, a dialkylamine, and combinations thereof, wherein the aminal has a formula of (R1)(R2)N—CH 2 —N(R3)(R4) where each of R1-R4 is an alkyl group, an aryl group, a substituted aryl group, and/or an alkylalkoxylate, and where R1, R2, R3, and R4 are the same or different; and

at least one inactivated composition selected from the group consisting of at least one inactivated sulfur species, at least one inactivated phosphorous-containing compounds, and combinations thereof.

8. A method comprising:

introducing at least one additive to a corrosion inhibitor comprising at least one phosphorous-containing compound selected from the group consisting of O,O-disubstituted dithiophosphoric acid, pyrophosphates, and combinations thereof; wherein the at least one phosphorous-containing compound exists within a system containing fluid selected from the group consisting of an aqueous system an aerobic system, an anaerobic system, and combinations thereof; wherein the at least one additive is selected from the group consisting of an aminal, a dialkylamine, and combinations thereof; wherein the aminal has a formula of (R1)(R2)N—CH 2 —N(R3)(R4) where each of R1-R4 is an alkyl group, an aryl group, a substituted aryl group, and/or an alkylalkoxylate, and where R1, R2, R3, and R4 are the same or different.

9. The method of claim 8 , wherein the dialkylamine comprises an alkyl group that is a straight or branched chain having from 1 carbon to 5 carbons.

10. The method of claim 8 , wherein the amount of the additive ranges from about 1 wt % to about 15 wt % based on the total amount of fluid in the system.

11. The method of claim 8 , further comprising inactivating the at least one phosphorous-containing compound within the system to form at least one inactivated phosphorous-containing compound.

12. The method of claim 8 , wherein the corrosion inhibitor further comprises at least one sulfur species.

13. The method of claim 12 , further comprising reacting the at least one additive with the at least one sulfur species to form a first reaction product.

14. The method of claim 13 , further comprising reacting the first reaction product with the at least one phosphorous-containing compound to form a second reaction product; and wherein the second reaction product is a stable reaction product.

15. A method comprising:

circulating a corrosion inhibitor containing at least one additive, at least one sulfur species, and at least one phosphorous-containing compound selected from the group consisting of O,O-disubstituted dithiophosphoric acid, pyrophosphates, and combinations thereof within a system; wherein the system is selected from the group consisting of an aqueous system an aerobic system, an anaerobic system, and combinations thereof; wherein the at least one additive is selected from the group consisting of an aminal, a dialkylamine, and combinations thereof; and wherein the aminal has a formula of (R1)(R2)N—CH 2 —N(R3)(R4) where each of R1-R4 is an alkyl group, an aryl group, a substituted aryl group, and/or an alkylalkoxylate, and where R1, R2, R3, and R4 are the same or different; and

inactivating the at least one phosphorous-containing compound, the at least one sulfur species, and combinations thereof with the at least one additive.

Assignments (2)
CHANGE OF NAME Recorded Feb 16, 2022
From: BAKER HUGHES, A GE COMPANY, LLC
To: BAKER HUGHES HOLDINGS LLC
Reel/Frame 059128/0907 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 27, 2018
From: PANCHALINGAM, VAITHILINGAM; HARRELL, BRADLEY G.
To: BAKER HUGHES, A GE COMPANY, LLC
Reel/Frame 046221/0029 →
Continuity (2)
Continuation In Part 14476438 · Sep 3, 2014
Related Publication 20180135189A1 · May 17, 2018