IP Library Granted Patent US 10,287,224
Granted Patent B2
US 10,287,224 · App. 12/630,418 · Granted May 14, 2019

Method and apparatus for producing methanol with hydrocarbon recycling

Inventors: Nathan A. Pawlak (Marquette, MI); Vladimir Ivanovich Vedeneev (Moscow, RU)
Assignee: Gas Technologies LLC
C07C29/50B01J12/00B01J19/2415C07C29/78C07C29/80C07C45/33B01J2219/00006B01J2219/00159
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Quick Facts
Patent No.
US 10,287,224
App. No.
12/630,418
Granted
May 14, 2019
Kind
B2
Abstract

An apparatus and method of producing methanol includes reacting a heated hydrocarbon-containing gas and an oxygen-containing gas in a reactor; to provide a product stream comprising methanol; and transferring heat from the product stream to the hydrocarbon-containing gas to heat the hydrocarbon containing gas. After removing methanol and CO 2 from the product stream, unprocessed hydrocarbons are mixed with the hydrocarbon containing gas fro reprocessing through the reactor.

Claims (18)

1. An apparatus for producing methanol, comprising:

a reactor having a reactor input;

a first hydrocarbon-containing gas supply that provides a first hydrocarbon-containing gas into the reactor input as a first hydrocarbon-containing gas stream;

a source of oxygen-containing gas that provides oxygen-containing gas into the reactor so that in said reactor a reaction of oxidation of heated hydrocarbon-containing gas with oxygen of the oxygen-containing gas takes place to produce a product stream comprising formaldehyde and methanol;

an isobaric condenser that condenses a relatively low volatility component of the product stream for separation from a relatively high volatility component of the product stream, the isobaric condenser operating isobarically;

a scrubber that receives the relatively high volatility component of the product stream from the isobaric condenser and removes a methanol-water stream that includes formaldehyde, water, methanol, and CO 2 ;

a rectification column that receives the methanol-water stream from the scrubber and removes a formaldehyde distillate stream including formaldehyde and CO 2 ;

a flash drum that receives the relatively low volatility component of the product stream from the isobaric condenser; and

a methanol rectifier that receives a liquid stream from the flash drum and separates methanol from ethanol,

wherein the first hydrocarbon-containing gas stream comprises a portion of the product stream.

2. The apparatus according to claim 1 further comprising a second hydrocarbon-containing gas supply providing a cold hydrocarbon-containing gas downstream of the first hydrocarbon-containing gas to be directly mixed with a mixture of a hydrocarbon-containing gas and the oxygen-containing gas to produce the product stream comprising formaldehyde and methanol; and

a heat exchanger for transferring heat from the product stream to the hydrocarbon-containing gas supplied by the first hydrocarbon-containing gas supply.

3. The apparatus as defined in claim 2 and further comprising a heater disposed between the heat exchanger and the reactor input for further preheating the hydrocarbon-containing gas prior to its supplying into the reactor.

4. The apparatus of claim 3 wherein the heat exchanger comprises a downstream portion of the reactor.

5. The apparatus as in claim 2 , wherein said second hydrocarbon-containing gas supply is arranged at a location of said reactor where formation of methanol and formaldehyde is substantially completed.

6. The apparatus as in claim 2 wherein a controller adjusts the second hydrocarbon-containing gas supply based on one or more operating parameters.

7. The apparatus as in claim 6 wherein the one or more operating parameters comprise temperature.

8. The apparatus according to claim 1 further comprising a formalin blender that receives a combined stream comprising the formaldehyde distillate stream from the rectification column and a vapor stream from the flash drum, the combined stream including formaldehyde, methanol, and carbon dioxide.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 10, 2025
From: GAS TECHNOLOGIES LLC
To: GASTECHNO CORP.
Reel/Frame 071374/0823 →
Continuity (3)
Division 11351532 · Feb 10, 2006
Continuation In Part 11319093 · Dec 27, 2005
Related Publication 20100158760A1 · Jun 24, 2010
Cited By (2)
US 12,292,009 US 12,522,775