IP Library Granted Patent US 8,057,988
Granted Patent B2
US 8,057,988 · App. 12/779,819 · Granted Nov 15, 2011

Catalyst for microelectromechanical systems microreactors

Assignee: Lawrence Livermore National Security, LLC
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Quick Facts
Patent No.
US 8,057,988
App. No.
12/779,819
Granted
Nov 15, 2011
Kind
B2
Abstract

A microreactor comprising a silicon wafer, a multiplicity of microchannels in the silicon wafer, and a catalyst coating the microchannels. In one embodiment the catalyst coating the microchannels comprises a nanostructured material. In another embodiment the catalyst coating the microchannels comprises an aerogel. In another embodiment the catalyst coating the microchannels comprises a solgel. In another embodiment the catalyst coating the microchannels comprises carbon nanotubes.

Claims (23)

1. A method of producing a microreactor, comprising the steps of:

providing a silicon wafer,

coating a photoresist on said silicon wafer,

using a mask with UV exposure to develop a desired pattern in said photoresist,

anisotropic etching said silicon wafer to produce microchannels in said silicon wafer,

applying a liquid containing a catalyst to said microchannels filling said microchannels with said liquid containing a catalyst,

aligning a substrate over said microchannels in said silicon wafer wherein said step of aligning a substrate over said microchannels in said silicon wafer comprises aligning a silicon wafer substrate or a glass substrate over said microchannels in said silicon wafer,

allowing surface tension to spread said liquid containing a catalyst over said microchannels by surface tension,

bonding said silicon wafer and said substrate, and

baking microchannels, said liquid, and said catalyst leaving said catalyst in said microchannels coating said microchannels with said catalyst.

2. The method of producing a microreactor of claim 1 wherein said step of aligning a substrate over said microchannels in said silicon wafer comprises aligning a silicon wafer substrate over said microchannels in said silicon wafer.

3. The method of producing a microreactor of claim 1 wherein said step of aligning a substrate over said microchannels in said silicon wafer comprises aligning a glass substrate over said microchannels in said silicon wafer.

4. The method of producing a microreactor of claim 1 wherein said step of bonding said silicon wafer and said substrate comprises anodic bonding or fusion bonding.

5. The method of producing a microreactor of claim 1 wherein said step of bonding said silicon wafer and said substrate comprises anodic bonding.

6. The method of producing a microreactor of claim 1 wherein said step of bonding said silicon wafer and said substrate comprises fusion bonding.

7. The method of producing a microreactor of claim 1 wherein said microchannels comprise a multiplicity of individual microchannels with each michrochannel having an end, and wherein said step of applying a liquid containing a catalyst to said microchannels filling said microchannels with said liquid containing a catalyst comprises applying a liquid containing a catalyst to said end of said michrochannel.

8. The method of producing a microreactor of claim 1 wherein said microchannels comprise a multiplicity of individual microchannels with each michrochannel having an end, and wherein said step of applying a liquid containing a catalyst to said microchannels filling said microchannels with said liquid containing a catalyst comprises applying a liquid containing a catalyst to said end of said michrochannel and closing said end of said michrochannel whereby said liquid containing a catalyst is wetted onto said microchannel by surface tension providing uniform coating of said microchannel through capillary forces.

9. The method of producing a microreactor of claim 1 wherein said microchannels comprise a multiplicity of individual microchannels with each michrochannel having an inlet and an outlet, and wherein said step of applying a liquid containing a catalyst to said microchannels filling said microchannels with said liquid containing a catalyst comprises applying said liquid containing a catalyst to said inlet and allowing said liquid containing a catalyst to flow to said outlet.

10. The method of producing a microreactor of claim 1 wherein said microchannels comprise a multiplicity of individual microchannels with each michrochannel having an inlet and an outlet, and wherein said step of applying a liquid containing a catalyst to said microchannels filling said microchannels with said liquid containing a catalyst comprises applying a liquid containing an aerogel catalyst to said microchannels filling said microchannels with said liquid containing an aerogel catalyst.

11. The method of producing a microreactor of claim 1 wherein said microchannels comprise a multiplicity of individual microchannels with each michrochannel having an inlet and an outlet, and wherein said step of applying a liquid containing a catalyst to said microchannels filling said microchannels with said liquid containing a catalyst comprises applying a liquid containing an solgel catalyst to said microchannels filling said microchannels with said liquid containing a solgel catalyst.

12. The method of producing a microreactor of claim 1 wherein said microchannels comprise a multiplicity of individual microchannels with each michrochannel having an inlet and an outlet, and wherein said step of applying a liquid containing a catalyst to said microchannels filling said microchannels with said liquid containing a catalyst comprises applying a liquid containing a zeolite catalyst to said microchannels filling said microchannels with said liquid containing a zeolite catalyst.

13. The method of producing a microreactor of claim 1 wherein said microchannels comprise a multiplicity of individual microchannels with each michrochannel having an inlet and an outlet, and wherein said step of applying a liquid containing a catalyst to said microchannels filling said microchannels with said liquid containing a catalyst comprises applying a liquid containing an an aerogel of zirconia, or alumina, or ceria, or calcia or silica, and combinations of zirconia, or alumina, or ceria, or calcia or silica to said microchannels filling said microchannels with said liquid containing an aerogel of zirconia, or alumina, or ceria, or calcia or silica, and combinations of zirconia, or alumina, or ceria, or calcia or silica.

14. The method of producing a microreactor of claim 1 wherein said microchannels comprise a multiplicity of individual microchannels with each michrochannel having an inlet and an outlet, and wherein said step of applying a liquid containing a catalyst to said microchannels filling said microchannels with said liquid containing a catalyst comprises applying a liquid containing copper, or zinc, or zirconium, or nickel, or chromium, or cobalt, or cerium, or silicon, or silica, or titanium, or aluminum nitrates, acetates, chlorides, oxychlorides or other soluble salts, or oxides thereof to said microchannels filling said microchannels with said liquid containing coating said microchannels with copper, or zinc, or zirconium, or nickel, or chromium, or cobalt, or cerium, or silicon, or silica, or titanium, or aluminum nitrates, acetates, chlorides, oxychlorides or other soluble salts, or oxides thereof.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 31, 2016
From: THE REGENTS OF THE UNIVERSITY OF CALIFORNIA
To: LAWRENCE LIVERMORE NATIONAL SECURITY, LLC
Reel/Frame 038163/0540 →
CONFIRMATORY LICENSE Recorded Dec 10, 2015
From: LAWRENCE LIVERMORE NATIONAL SECURITY, LLC
To: U.S. DEPARTMENT OF ENERGY
Reel/Frame 037260/0546 →
Continuity (3)
Division 11119047 · Apr 28, 2005
Provisional Application 60566775 · Apr 29, 2004
Related Publication 20100221667A1 · Sep 2, 2010