IP Library Granted Patent US 9,254,505
Granted Patent B2
US 9,254,505 · App. 13/690,582 · Granted Feb 9, 2016

Method for manufacturing nanowire meshes

Inventors: Steve T. Connor (Stanford, CA); Jung-Yong Lee (Menlo Park, CA); Yi Cui (Sunnyvale, CA); Peter Peumans (Leuven, BE)
Assignee: The Board of Trustees of the Leland Stanford Junior University
B05D5/12B05D7/20B82Y20/00B82Y30/00C23C18/16H01L31/022433H01L31/1884H01L51/441H01L51/442H01L51/444H01L51/445B82Y35/00H01L51/0037H01L51/0053H01L51/4246Y02E10/549
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Quick Facts
Patent No.
US 9,254,505
App. No.
13/690,582
Granted
Feb 9, 2016
Kind
B2
Abstract

A variety of methods, devices, systems and arrangements are implemented involving nanowire meshes. One such method is implemented to include synthesizing metal nanowires in a solution containing a structure-directing agent. The metal nanowires are deposited on a substrate to form a sheet of nanowires. The deposited metal nanowires are heated to a temperature less than about 200 degrees Celsius and for a period of time of about 10 minutes to 60 minutes, thereby removing the structure-directing agent and modifying the electrical conductivity and optical transmittance of the sheet of nanowires.

Claims (23)

1. A method comprising:

synthesizing nanowires containing silver in a solution containing a structure-directing agent;

forming a sheet of nanowires from the synthesizing nanowires; and

heating the sheet of nanowires at a temperature and for a time sufficient to remove the structure-directing agent and to produce a sheet conductivity level, for the sheet of nanowires, that is less than 25 ohms per square and a sheet transmittance, for the sheet of nanowires, of at least about 80% for all wavelengths between about 400 nanometers and 800 nanometers.

2. The method of claim 1 , wherein the step of heating includes heating the sheet of nanowires to a temperature of between 180-200 degrees (Celsius) for 18-22 minutes, and results in the sheet conductivity level being less than 15 ohms per square and sheet transmittance of at least 80% for all wavelengths between 400 nanometers and 800 nanometers.

3. The method of claim 1 , wherein the step of heating results in sheet transmittance of at least about 88% for all wavelengths between about 400 nanometers and 800 nanometers, further including applying a metallic coating to the nanowires.

4. The method of claim 1 , wherein the step of synthesizing nanowires includes creating predominantly silver nanowires having an average length of about 5 μm to 20 μm and an average diameter of less than about 100 nm.

5. The method of claim 1 , wherein the step of synthesizing nanowires includes creating predominantly silver nanowires having an average length of about 8 μm to 9 μm and an average diameter of less than of about 100 nm.

6. The method of claim 1 , further including a step of immersing the sheet of nanowires in a solution of gold salt (HAuCl4) to effect a replacement of at least some of the silver in the nanowire with gold.

7. The method of claim 6 , further including a step of heating the immersed sheet of nanowires at temperatures between 25 degrees and 100 degrees (Celsius) for 1 to 10 minutes.

8. The method of claim 6 , further including a step of selecting an immersion time as a function of a desired ratio of gold to silver.

9. The method of claim 6 , wherein processing parameters for the step of immersing is controlled to form a thin shell of gold on the sheet of nanowires.

10. The method of claim 1 , further including a step of depositing an organic photovoltaic cell onto the sheet of nanowires.

11. The method of claim 1 , further including a step of applying, to the heated and deposited silver nanowires, pressure of about 1.4(+/−0.6)×10e4 pounds per square inch for about 30 seconds.

12. The method of claim 1 , further including a step of applying uni-axial pressure to the sheet of heated nanowires to reduce surface roughness of the sheet of nanowires.

13. The method of claim 1 , wherein the sheet of nanowires exhibits resistance that is greater than 1 kΩ/sq prior to heating.

14. The method of claim 1 , wherein the sheet of nanowires exhibits resistance that is approximately 100 Ω/sq after the step of heating.

15. The method of claim 1 , further comprising:

providing a substrate; and wherein the step of heating results in a silver nanowire mesh located on the substrate and having a sheet conductivity level that is less than 25 ohms per square and a sheet transmittance of at least 80% for all wavelengths between about 400 nanometers and 800 nanometers.

16. The method of claim 15 , further including small molecular weight organic photovoltaic cells located on the silver nanowire mesh.

17. The method of claim 15 , wherein the silver nanowire mesh includes a poly(ethylenedioxythiophene) poly(styrenesulfonate) (PEDOT:PSS) layer.

18. The method of claim 17 , further including a bilayer solar cell located on the silver nanowire mesh.

19. The method of claim 18 , wherein the bilayer solar cell includes a layer structure of copper phthalocyanine (CuPc), perylenetetracarboxylix bisbenzimidazole (PTCBI) and of bathocuproine (BCP).

Assignments (2)
CONFIRMATORY LICENSE Recorded Jun 5, 2015
From: STANFORD UNIVERSITY
To: NATIONAL SCIENCE FOUNDATION
Reel/Frame 035841/0596 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 20, 2014
From: CONNOR, STEVE T.; LEE, JUNG-YONG; CUI, YI; PEUMANS, PETER
To: THE BOARD OF TRUSTEES OF THE LELAND STANFORD JUNIOR UNIVERSITY
Reel/Frame 032259/0405 →
Continuity (2)
Continuation 12351313 · Jan 9, 2009
Related Publication 20130098436A1 · Apr 25, 2013