IP Library Granted Patent US 9,347,143
Granted Patent B2
US 9,347,143 · App. 14/118,891 · Granted May 24, 2016

Membrane template synthesis of microtube engines

Inventors: Joseph Wang (San Diego, CA); Wei Gao (La Jolla, CA); Sirilak Sattayasamitsathit (San Diego, CA)
Assignee: The Regents of the University of California
C25D1/02B82Y30/00F03H99/00
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Quick Facts
Patent No.
US 9,347,143
App. No.
14/118,891
Granted
May 24, 2016
Kind
B2
Abstract

Methods, structures, devices and systems are disclosed for fabrication of microtube engines using membrane template electrodeposition. Such nanomotors operate based on bubble-induced propulsion in biological fluids and salt-rich environments. In one aspect, fabricating microengines includes depositing a polymer layer on a membrane template, depositing a conductive metal layer on the polymer layer, and dissolving the membrane template to release the multilayer microtubes.

Claims (42)

1. A method of fabricating one or more microtubes, comprising:

depositing a first layer on a template that has one or more holes of a desired hole geometry to form a tube of the first layer in each hole;

depositing a second layer over the first layer inside each hole of the template to form a bilayer microtube formed of the first and second layers inside each hole; and

separating the template from each bilayer microtube;

wherein the first layer comprises a polymer material;

wherein the polymer material comprises one of polypyrrole (PPy) and poly(3,4-ethylenedioxythiophene) (PEDOT).

2. The method of claim 1 , wherein the second layer comprises a material that is reactive with a fuel or is a catalyst of a fuel.

3. The method of claim 2 , wherein the material that is reactive with a fuel or is a catalyst of a fuel comprises a conductive metal.

4. The method of claim 2 , wherein the material that is a catalyst of a fuel comprises platinum.

5. A method of fabricating one or more microtubes, comprising:

depositing a first layer on a template that has one or more holes of a desired hole geometry to form a tube of the first layer in each hole;

depositing a second layer over the first layer inside each hole of the template to form a bilayer microtube formed of the first and second layers inside each hole; and

separating the template from each bilayer microtube;

wherein the template comprises cyclopore polycarbonated membrane.

6. The method of claim 5 , wherein the cyclopore polycarbonated membrane comprises an asymmetrical, conically-shaped pore structure.

7. The method of claim 6 , wherein the asymmetrical conically-shaped pore structure comprises different cone angles.

8. A method of fabricating one or more microtubes, comprising:

depositing a first layer on a template that has one or more holes of a desired hole geometry to form a tube of the first layer in each hole;

depositing a second layer over the first layer inside each hole of the template to form a bilayer microtube formed of the first and second layers inside each hole; and

separating the template from each bilayer microtube;

wherein the microtube comprises a self-propulsion.

9. The method of claim 8 , wherein several hundreds of microtube body lengths per second speed is achieved.

10. The method of claim 1 , the microtube comprises a fuel based microtube.

11. The method of claim 10 , wherein the fuel based microtube uses a 0.2%-30% concentration hydrogen peroxide fuel.

12. The method of claim 8 , wherein the microtube is fabricated to different diameters and lengths.

13. The method of claim 1 , wherein the separating is performed by dissolving the template.

14. The method of claim 13 , wherein the intermediate second layer comprises a ferromagnetic material.

15. The method of claim 14 , wherein the ferromagnetic material comprises nickel, iron or cobalt.

16. The method of claim 13 , wherein the third layer comprises a material that is reactive with a fuel or a catalyst of a fuel.

17. The method of claim 16 , wherein the material that is reactive with a fuel or a catalyst of a fuel comprises a conductive material.

18. The method of claim 16 , wherein the material that is reactive with a fuel or a catalyst of a fuel a fuel comprises platinum.

19. The method of claim 13 , wherein the dissolving is performed using methylene chloride.

20. The method of claim 1 , wherein the depositing the second layer includes depositing the second layer by using a galvanostatic deposition.

21. A method of fabricating one or more microtubes, comprising:

depositing a first layer on a template that has one or more holes to form a tube of the first layer in each hole;

depositing an intermediate second layer over the first layer inside each hole;

depositing a third layer over the intermediate second layer inside each hold to form a trilayer microtube formed of the first, intermediate second, and third layers inside each hole; and

separating the template from each trilayer microtube;

wherein the polymer material comprises one of polypyrrole (PPy) and poly(3,4-ethylenedioxythiophene) (PEDOT).

22. The method of claim 21 , wherein the separating is performed by dissolving the template.

23. The method of claim 22 , wherein the dissolving is performed using methylene chloride.

24. The method of claim 21 , wherein the depositing the second layer includes depositing the second layer by using a galvanostatic deposition.

Assignments (2)
CONFIRMATORY LICENSE Recorded Jul 30, 2014
From: UNIVERSITY OF CALIFORNIA SAN DIEGO
To: NATIONAL SCIENCE FOUNDATION
Reel/Frame 033448/0579 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 18, 2014
From: WANG, JOSEPH; GAO, WEI; SATTAYASAMITSATHIT, SIRILAK
To: THE REGENTS OF THE UNIVERSITY OF CALIFORNIA
Reel/Frame 032235/0585 →
Continuity (2)
Provisional Application 61492782 · Jun 2, 2011
Related Publication 20140162870A1 · Jun 12, 2014