IP Library Granted Patent US 10,139,417
Granted Patent B2
US 10,139,417 · App. 14/376,154 · Granted Nov 27, 2018

Systems, apparatuses and methods for reading an amino acid sequence

Inventors: Stuart Lindsay (Phoenix, AZ); Peiming Zhang (Gilbert, AZ); Yanan Zhao (Tempe, AZ)
Assignee: ARIZONA BOARD OF REGENTS ON BEHALF OF ARIZONA STATE UNIVERSITY
G01N33/6821G01N33/48721
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Quick Facts
Patent No.
US 10,139,417
App. No.
14/376,154
Granted
Nov 27, 2018
Kind
B2
Abstract

Embodiments of the present disclosure relate to amino acid, modified amino acid, peptide and protein identification and sequencing, by means of, for example, electronic detection of individual amino acids or small peptides.

Claims (19)

1. An apparatus for sequencing a molecule comprising:

at least a first and a second electrode;

a dielectric layer of between about 1 nm and about 4 nm separating the first and second electrodes;

a membrane between about 10 to about 100 nm in thickness;

a channel containing an electrolyte solution, wherein the membrane spans and divides the channel to form a cis chamber and a trans chamber,

wherein the cis chamber and the trans chamber are in fluid communication with one another via a nanopore, and

a bead in the cis chamber and arranged within 150 μm of the nanopore, the bead including a molecule for sequencing and/or identifying bound thereto,

wherein:

the nanopore is formed on the same substrate as the pair of electrodes,

the nanopore is between about 1 nm and about 5 nm in diameter at the point where it passes through the electrodes, and

the electrodes include between about 1 nm to about 5 nm of silver, gold, palladium and/or platinum, and the electrodes are functionalized.

2. The apparatus according to claim 1 , wherein each chamber is filled with an electrolyte comprising at least one of KCl and NaClO3 in a concentration between about 1 mM to about 1M.

3. The apparatus according to claim 1 , wherein the bead includes enzymes attached thereto which are fixed in turn to the walls of the channel.

4. The apparatus according to claim 3 , wherein the enzymes comprise proteases selected from the group consisting of trypsin, chymotrypsin, pepsin, papain, elastase and combinations thereof.

5. The apparatus according to claim 3 , wherein the bead is functionalized with proteosomes to sequentially degrade proteins into their component amino acids.

6. The apparatus according to claim 3 , wherein the molecule comprises an isolated protein or peptide.

7. The apparatus according to claim 1 , further comprising one or more reference electrodes.

8. The apparatus according to claim 1 , wherein the bead is affixed to the wall of the channel.

9. The apparatus according to claim 1 , wherein the molecule is not a protease.

Assignments (2)
CONFIRMATORY LICENSE Recorded Feb 1, 2019
From: ARIZONA STATE UNIVERSITY, TEMPE CAMPUS
To: NATIONAL INSTITUTES OF HEALTH (NIH), U.S. DEPT. OF HEALTH AND HUMAN SERVICES (DHHS), U.S. GOVERNMENT
Reel/Frame 048228/0766 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 25, 2014
From: LINDSAY, STUART; ZHANG, PEIMING; ZHAO, YANA
To: ARIZONA BOARD OF REGENTS ON BEHALF OF ARIZONA STATE UNIVERSITY
Reel/Frame 034261/0787 →
Continuity (3)
Provisional Application 61593552 · Feb 1, 2012
Provisional Application 61647847 · May 16, 2012
Related Publication 20150010935A1 · Jan 8, 2015