IP Library Granted Patent US 9,733,228
Granted Patent B2
US 9,733,228 · App. 14/426,879 · Granted Aug 15, 2017

Methods of analyzing crude oil

Inventors: Robert Graham Cooks (West Lafayette, IN); Fred Paul Mark Jjunju (West Lafayette, IN); Anyin Li (West Lafayette, IN); Iman S. Rogan (Thuwal, SA)
Assignee: Purdue Research Foundation
G01N33/2823G01N30/724G01N30/7266H01J49/0031H01J49/04H01J49/10H01J49/164
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Quick Facts
Patent No.
US 9,733,228
App. No.
14/426,879
Granted
Aug 15, 2017
Kind
B2
Abstract

The invention generally relates to methods of analyzing crude oil. In certain embodiments, methods of the invention involve obtaining a crude oil sample, and subjecting the crude oil sample to mass spectrometry analysis. In certain embodiments, the method is performed without any sample pre-purification steps.

Claims (11)

1. A method for analyzing a crude oil sample, the method comprising:

obtaining a crude oil sample comprising a non-naturally occurring substance within the crude oil sample;

introducing the crude oil sample to a porous paper substrate;

applying solvent and voltage to the crude oil sample on the substrate to generate ions of the non-naturally occurring substance directly and only from the crude oil sample, wherein the applying step is conducted without an external heat source; and

analyzing the ions using a mass spectrometer, wherein the method is performed without pre-purification of the crude oil sample.

2. The method according to claim 1 , wherein the mass spectrometer is selected from the group consisting of a bench-top mass spectrometer and a miniature mass spectrometer.

3. The method according to claim 1 , wherein the non-naturally occurring substance in the crude oil is a corrosion inhibitor.

4. The method according to claim 3 , wherein the corrosion inhibitor comprises at least one alkyl ammonium salt.

5. The method according to claim 4 , wherein the alkyl ammonium salt is selected from the group consisting of tetradodecylammonium bromide, benzylhexadecyldimethylammonium chloride, and a combination thereof.

6. The method according to claim 1 , wherein the mass spectrometer is coupled with a discontinuous atmospheric pressure interface.

7. The method according to claim 1 , wherein the solvent comprises a mixture of methanol and acetonitrile.

Assignments (2)
CONFIRMATORY LICENSE Recorded Apr 6, 2021
From: PURDUE UNIVERSITY
To: UNITED STATES DEPARTMENT OF ENERGY
Reel/Frame 055844/0533 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 15, 2015
From: COOKS, ROBERT GRAHAM; LI, ANYIN
To: PURDUE RESEARCH FOUNDATION
Reel/Frame 037295/0827 →
Continuity (2)
Provisional Application 61759097 · Jan 31, 2013
Related Publication 20150309001A1 · Oct 29, 2015