IP Library › Granted Patent US 9,364,824
Granted Patent B2
US 9,364,824 · App. 14/525,371 · Granted Jun 14, 2016

Electrospinning solution, polyvinyl alcohol nanofibers and ion-exchange membrane

Inventors: Hsin-Ying Chou (New Taipei, TW); Huan-Sheng Chien (New Taipei, TW); Haw-Jer Chang (New Taipei, TW); Ni Putu Dewi Nurmalasari (New Taipei, TW)
Assignee: TAIWAN TEXTILE RESEARCH INSTITUTE
B01J39/20B01D67/0004B01D69/02B01D71/38B01D71/82C08F116/06C08J5/22D01D5/00D01D5/003D01F1/10D01F6/14B01D2323/39D10B2321/06H01M2/1653Y10T428/298
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Quick Facts
Patent No.
US 9,364,824
App. No.
14/525,371
Granted
Jun 14, 2016
Kind
B2
Abstract

An ion-exchange membrane is provided, and the fibers of the ion-exchange membrane are obtained by electrospinning. The electrospinning solution contains 100 parts by weight of polyvinyl alcohol (PVA), 10-100 parts by weight of a modifier, 10-100 parts by weight of an ion exchanger, and 100-2,500 parts by weight of water. The modifier has a reactive group that can react with the hydroxyl groups of the PVA. The ion exchanger has a polar functional group that can form hydrogen bonds with the hydroxyl groups of the PVA, and has an anion group that can provide ion-exchange ability.

Claims (28)

1. An electrospinning solution, a composition of the electrospinning solution comprising:

100 parts by weight of polyvinyl alcohol (PVA);

10-100 parts by weight of a modifier having a reactive group that can react with hydroxyl groups of the PVA at a temperature of 100-200° C.;

10-100 parts by weight of an ion exchanger having a polar functional group and an anion group, wherein the polar functional group is —OH, —NH 2 , —COOH, —CHO, —F or any combinations thereof; and

100-2,500 parts by weight of water.

2. The electrospinning solution of claim 1 , wherein a weight average molecular weight of PVA is from about 15,000 to about 120,000.

3. The electrospinning solution of claim 1 , wherein the reactive group of the modifier comprises an isocyanate (—NCO) group, a carboxylate group (—COO − ), or a nitro group (—NO 2 − ).

4. The electrospinning solution of claim 1 , wherein the modifier is

and R 1 is

5. The electrospinning solution of claim 1 , wherein the anion group of the ion exchanger is —SO 3 , —COO − , or —NO 2 − .

6. The electrospinning solution of claim 1 , wherein the ion exchanger is 5-sodium sulfoisophthalate (5-SSIPA), sodium dimethyl 5-sulphonatoisophthalate (SIPM), dimethyl 5-sulfoisophthalate sodium salt hydrate (SIPE), trisodium 2-hydroxy-1,2,3-propanetricarboxylate (i.e. sodium citrate), dipotassium ethylenediamine tetraacetate, sodium tartrate, sodium alginate, or sodium nitrite.

7. Nanofibers of polyvinyl alcohol electrospun by an electrospinning solution, a composition of the electrospinning solution comprising:

100 parts by weight of polyvinyl alcohol (PVA);

10-100 parts by weight of a modifier having a reactive group that can react with hydroxyl groups of the PVA at a temperature of 100-200° C.;

10-100 parts by weight of an ion exchanger having a polar functional group and an anion group, wherein the polar functional group is —OH, —NH 2 , —COOH, —CHO, —F or any combinations thereof; and

100-2,500 parts by weight of water.

8. The nanofibers of claim 7 , wherein a weight average molecular weight of the PVA is from about 15,000 to about 120,000.

9. The nanofibers of claim 7 , wherein the reactive group of the modifier comprises an isocyanate (—NCO) group, a carboxylate group (—COO − ), or a nitro group (—NO 2 − ).

10. The nanofibers of claim 7 , wherein the anion group of the ion exchanger is —SO 3 , —COO − , or —NO 2 − .

11. The nanofibers of claim 7 , wherein a diameter of the nanofibers is from about 50 nm to about 300 nm.

12. An ion-exchange membrane comprising nanofibers of polyvinyl alcohol, wherein the nanofibers of polyvinyl alcohol are electrospun by an electrospinning solution, and a composition of the electrospinning solution comprising:

100 parts by weight of polyvinyl alcohol (PVA);

10-100 parts by weight of a modifier having a reactive group that can react with hydroxyl groups of the PVA at a temperature of 100-200° C.;

10-100 parts by weight of an ion exchanger having a polar functional group and an anion group, wherein the polar functional group is —OH, —NH 2 , —COOH, —CHO, —F or any combinations thereof; and

100-2,500 parts by weight of water.

13. The ion-exchange membrane of claim 12 , wherein a weight average molecular weight of the PVA is from about 15,000 to about 120,000.

14. The ion-exchange membrane of claim 12 , wherein the reactive group of the modifier comprises an isocyanate (—NCO) group, a carboxylate group (—COO − ), or a nitro group (—NO 2 − ).

15. The ion-exchange membrane of claim 12 , wherein the anion group of the ion exchanger is —SO 3 − , —COO − , or —NO 2 − .

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 28, 2014
From: CHOU, HSIN-YING; CHIEN, HUAN-SHENG; CHANG, HAW-JER; NURMALASARI, NI PUTU DEWI
To: TAIWAN TEXTILE RESEARCH INSTITUTE
Reel/Frame 034048/0124 →
Priority Claims (1)
TW 103116859 A · May 13, 2014 · national
Continuity (1)
Related Publication 20150328631A1 · Nov 19, 2015