IP Library Granted Patent US 9,732,443
Granted Patent B2
US 9,732,443 · App. 14/915,648 · Granted Aug 15, 2017

Polyester fiber

Inventors: Takeshi Kikutani (Tokyo, JP); Wataru Takarada (Kanagawa, JP); Noriyuki Suzuki (Settsu, JP); Tetsuya Minami (Settsu, JP); Takahiko Sugaya (Settsu, JP)
Assignees: TOKYO INSTITUTE OF TECHNOLOGY; KANEKA CORPORATION
D01F6/84B29C47/0014B29C47/8805C08G63/06D01F6/625B29K2067/00B29L2031/731C08G2230/00D10B2331/041D10B2401/063D10B2401/12D10B2401/20
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Quick Facts
Patent No.
US 9,732,443
App. No.
14/915,648
Granted
Aug 15, 2017
Kind
B2
Abstract

An object of the present invention is to improve spinnability, productivity, and tensile strength of a polyester fiber containing poly(3-hydroxybutyrate-co-3-hydroxyhexanoate). By spinning the polyester resin containing the poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) at a high spinning velocity, the spinnability, productivity, and tensile strength of the polyester fiber can be improved.

Claims (27)

1. A polyester fiber produced by spinning a polyester resin comprising poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) at a spinning velocity of from 1,500 to 7,000 m/min,

wherein the polyester fiber has a ratio I β /I α of not less than 0.02, where I α denotes a diffraction intensity from α-crystals, I β denotes a diffraction intensity from β-crystals, and an influence on I α and I β caused by an amorphous phase in the polyester fiber is removed when measuring I α and I β .

2. The polyester fiber according to claim 1 , wherein the poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) comprises 3-hydroxybutyrate as a monomer in an amount of from 99.5 to 88.5 mol %.

3. The polyester fiber according to claim 1 , wherein the spinning of the polyester resin comprises extruding the polyester resin from a spinning die at a resin temperature of from 145 to 190° C.

4. The polyester fiber according to claim 1 , wherein the poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) has a weight-average molecular weight of from 150,000 to 1,500,000.

5. The polyester fiber according to claim 1 , wherein the poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) has a weight-average molecular weight of from 200,000 to 1,000,000.

6. The polyester fiber according to claim 1 , wherein the poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) comprises 3-hydroxybutyrate as a monomer in an amount of from 99 to 93 mol %.

7. The polyester fiber according to claim 1 , wherein the polyester resin comprises not less than 70 wt % of the poly(3-hydroxybutyrate-co-3-hydroxyhexanoate).

8. The polyester fiber according to claim 1 , wherein the polyester resin further comprises at least one of a lubricant and a plasticizer.

9. A method for producing a polyester fiber, comprising:

spinning a polyester resin comprising poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) at a spinning velocity of from 1,500 to 7,000 m/min such that a polyester fiber is produced and that the polyester fiber has a ratio I β /I α of not less than 0.02, where I α denotes a diffraction intensity from α-crystals, I β denotes a diffraction intensity from β-crystals, and an influence on I α and I β caused by an amorphous phase in the polyester fiber is removed when measuring I α and I β .

10. The method according to claim 9 , wherein the spinning of the polyester resin comprises extruding the polyester resin from a spinning die at a resin temperature of from 145 to 190° C.

11. The method according to claim 9 , wherein the spinning of the polyester resin comprises extruding the polyester resin from a spinning die at a resin temperature of from 150 to 190° C.

12. The method according to claim 9 , wherein the spinning die has an opening having an area of from 0.15 mm 2 to 3.5 mm 2 .

13. The method according to claim 9 , wherein, in the spinning, the spinning velocity is from 2,000 to 7,000 m/min.

14. The method according to claim 9 , further comprising:

culturing a microorganism such that the poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) is accumulated in the microorganism.

15. The method according to claim 9 , wherein the poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) comprises 3-hydroxybutyrate as a monomer in an amount of from 99.5 to 88.5 mol %.

16. The method according to claim 9 , wherein the poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) has a weight-average molecular weight of from 150,000 to 1,500,000.

17. The method according to claim 9 , wherein the poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) comprises 3-hydroxybutyrate as a monomer in an amount of from 99 to 93 mol %.

18. The method according to claim 9 , wherein the polyester resin comprises not less than 70 wt % of the poly(3-hydroxybutyrate-co-3-hydroxyhexanoate).

19. The method according to claim 9 , wherein the polyester resin further comprises at least one of a lubricant and a plasticizer.

20. The method according to claim 9 , further comprising:

stretching the polyester fiber within 120 minutes after the spinning of the polyester resin is completed.

21. A polyester fiber produced by spinning a polyester resin comprising poly(3-hydroxybutyrate-co-3-hydroxyhexanoate),

wherein the polyester fiber has a ratio I β /I α of not less than 0.02, where I α denotes a diffraction intensity from α-crystals, I β denotes a diffraction intensity from β-crystals, and an influence on I α and I β caused by an amorphous phase in the polyester fiber is removed when measuring I α and I β .

22. The polyester fiber of claim 21 , wherein a spinning velocity is not less than 1,500 m/min.

Assignments (3)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 20, 2024
From: INSTITUTE OF SCIENCE TOKYO
To: KANEKA CORPORATION
Reel/Frame 069341/0214 →
CHANGE OF NAME Recorded Nov 20, 2024
From: TOKYO INSTITUTE OF TECHNOLOGY
To: INSTITUTE OF SCIENCE TOKYO
Reel/Frame 069403/0943 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 11, 2016
From: KIKUTANI, TAKESHI; TAKARADA, WATARU; SUZUKI, NORIYUKI; MINAMI, TETSUYA; SUGAYA, TAKAHIKO
To: TOKYO INSTITUTE OF TECHNOLOGY; KANEKA CORPORATION
Reel/Frame 039400/0127 →
Priority Claims (1)
JP 2013-181537 · Sep 2, 2013 · national
Continuity (1)
Related Publication 20160230313A1 · Aug 11, 2016