IP Library Granted Patent US 10,381,656
Granted Patent B2
US 10,381,656 · App. 14/946,031 · Granted Aug 13, 2019

Nanocomposite electrode material for proton conducting fuel cell

Inventors: Alexander B. Papandrew (Knoxville, TN); Ramez A. Elgammal (Knoxville, TN)
Assignee: University of Tennessee Research Foundation
H01M4/926H01M4/8663H01M4/8673H01M4/92H01M2008/1095
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Quick Facts
Patent No.
US 10,381,656
App. No.
14/946,031
Granted
Aug 13, 2019
Kind
B2
Abstract

An electrode includes a proton conducting electrolyte phase, an electronic conducting phase, and a metal or metal alloy catalyst in contact with each of the phases. The electronic conducting phase is infiltrated with the proton conducting electrolyte phase such that the phases form a solid nanocomposite with bulk electronic conductivity.

Claims (24)

1. An electrode comprising:

a proton conducting electrolyte phase;

an electronic conducting phase having pores thereon and interior diameter regions therein both infiltrated with the proton conducting electrolyte phase such that the phases form a solid nanocomposite with bulk electronic conductivity; and

a metal or metal alloy catalyst in contact with each of the phases.

2. The electrode of claim 1 , wherein the proton conducting electrolyte phase is a phosphate.

3. The electrode of claim 1 , wherein the proton conducting electrolyte phase is a superprotonic solid acid.

4. The electrode of claim 1 , wherein the proton conducting electrolyte phase is a pyrophosphate.

5. The electrode of claim 1 , wherein the proton conducting electrolyte phase is an oxide.

6. The electrode of claim 1 , wherein the proton conducting electrolyte phase is a polymer.

7. The electrode of claim 1 , wherein the proton conducting electrolyte phase is organic.

8. The electrode of claim 1 , wherein the electronic conducting phase is chemically functionalized.

9. The electrode of claim 1 , wherein the electronic conducting phase is doped with heteroatoms.

10. The electrode of claim 6 , wherein the heteroatoms include boron, nitrogen or phosphorous.

11. The electrode of claim 1 , wherein the electronic conducting phase is carbon nanotubes.

12. The electrode of claim 1 , wherein the electronic conducting phase is mesoporous carbon.

13. The electrode of claim 1 , wherein the electronic conducting phase is single-walled or multi-walled carbon nanohorn.

14. The electrode of claim 1 , wherein the electronic conducting phase is porous carbon fibers.

15. The electrode of claim 14 , wherein the porous carbon fibers are doped with heteroatoms.

16. The electrode of claim 1 , wherein the metal or metal alloy catalyst includes platinum.

17. A proton conducting fuel cell comprising:

a separator membrane; and

an electrode in contact with the separator membrane, and including an electronic conducting phase having pores thereon and interior diameter regions therein, a proton conducting electrolyte phase infiltrated within the pores and interior diameter regions, and a metal or metal alloy catalyst in contact with the phases to form a solid nanocomposite with bulk electronic conductivity.

18. The proton conducting fuel cell of claim 17 , wherein the electrode is an anode.

19. The proton conducting fuel cell of claim 18 , wherein the catalyst includes palladium or ruthenium.

Assignments (2)
CONFIRMATORY LICENSE Recorded Feb 6, 2018
From: UNIVERSITY OF TENNESSEE SYSTEM
To: U.S. DEPARTMENT OF ENERGY
Reel/Frame 045261/0094 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 20, 2015
From: PAPANDREW, ALEXANDER B.; ELGAMMAL, RAMEZ A.
To: UNIVERSITY OF TENNESSEE RESEARCH FOUNDATION
Reel/Frame 037095/0947 →
Continuity (1)
Related Publication 20170149068A1 · May 25, 2017