IP Library › Granted Patent US 9,862,607
Granted Patent B2
US 9,862,607 · App. 15/216,614 · Granted Jan 9, 2018

Fabrication and application of nanofiber ribbons and sheets and twisted and non-twisted nanofiber yarns

Inventors: Mei Zhang (Plano, TX); Shaoli Fang (Richardson, TX); Ray H. Baughman (Dallas, TX); Anvar A. Zakhidov (McKinney, TX); Kenneth Ross Atkinson (Victoria, AU); Ali E. Aliev (Dallas, TX); Sergey Li (Dallas, TX); Chris Williams (Dallas, TX)
Assignee: Board of Regents, The University of Texas System
C01B31/024B01L3/502707B29C47/0059B32B5/02B32B5/12B32B18/00B32B37/12B82Y10/00C01B31/0226C01B31/0253C01B31/0293C04B35/62231C04B35/62272C04B35/62281C04B35/62855C04B35/62892C04B35/62897C04B35/80C23C16/44C23C16/50D01F9/08D01F9/12D01F9/127D01F9/1273D01F9/1275D02G3/16D02G3/28D02G3/44D04H3/002D06B15/00D06M15/256D06M15/333G01L1/2287G02F1/133308H01B1/24H01B5/08H01G11/36H01L51/0048H01L51/444H01L51/5206H01M4/926H01M10/0565H05K9/0081B32B2262/106B32B2307/202B32B2310/00B32B2313/04B82Y30/00B82Y40/00C01B2202/06C01B2202/08C04B2235/422C04B2235/526C04B2235/5248C04B2235/5264C04B2235/616D10B2101/122G02F2001/133334G02F2001/1515H01L51/5234H01L51/5296H01M4/8605Y02E10/549Y02E60/13Y02P70/521Y10S977/742Y10S977/745Y10S977/746Y10S977/752Y10S977/843Y10S977/844Y10S977/847Y10S977/848Y10S977/932Y10S977/948Y10S977/961Y10T428/30
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Quick Facts
Patent No.
US 9,862,607
App. No.
15/216,614
Granted
Jan 9, 2018
Kind
B2
Abstract

Fabricating a nanofiber sheet, ribbon, or yarn by a continuous process that includes synthesizing a nanofiber forest in a forest growth region on a substrate, wherein the nanofiber forest comprises a parallel array of nanofibers, and further includes drawing said nanofibers from the nanofiber forest to form a primary assembly that is a sheet, ribbon or yarn. The substrate continuously moves from the furnace growth region into a region where the nanofibers in the forest are drawn.

Claims (27)

1. A process for continuously producing a nanofiber sheet, ribbon, or yarn, the process comprising:

(a) synthesizing a nanofiber forest in a furnace growth region on a substrate, wherein the nanofiber forest comprises a parallel array of nanofibers; and

(b) drawing said nanofibers from the nanofiber forest to form a primary assembly that is a sheet, ribbon or yarn, wherein the substrate continuously moves from the furnace growth region into a region where the nanofibers in the forest are drawn.

2. The process of claim 1 , wherein the drawing occurs without twisting when the primary assembly is a ribbon or a sheet and the drawing includes twisting when the primary assembly is a yarn.

3. The process of claim 1 , wherein the substrate is in motion with respect to the furnace growth region.

4. The process of claim 1 , wherein the substrate is flexible.

5. The process of claim 1 , wherein the substrate is a flexible belt or is attached to a moving belt.

6. The process of claim 1 , wherein the substrate on which the nanofiber forest is synthesized is a drum and the nanofibers are drawn from the drum.

7. The process of claim 1 further comprising depositing the primary assembly on a second substrate.

8. The process of claim 7 , wherein the step of depositing comprises wrapping the primary assembly on the second substrate.

9. The process of claim 1 , wherein the drawing of said nanofibers produces a nanofiber ribbon, and wherein the nanofiber ribbon is laminated to a second nanofiber ribbon to form a nanofiber sheet.

10. The process of claim 9 , wherein the step of laminating involves a laminating means selected from the group consisting of a chemical binding agent, an electron beam, a thermal treatment, an ion beam, radio frequency irradiation, microwave irradiation, and combinations thereof.

11. The process of claim 1 , wherein the nanofiber forest is synthesized by chemical vapor deposition.

12. The process of claim 1 , wherein said nanofiber forest is densified by imbibing a liquid comprising a volatile component and subsequently evaporating the volatile component of the liquid.

13. The process of claim 1 , wherein said nanofibers are selected from the group consisting of imogolite nanofibers; carbon nanotubes; doped carbon nanotubes; SiC nanofibers; MgB 2 nanofibers; carbon doped MgB 2 nanofibers; Bi nanofibers; nanofibers of binary group III-V elements; Si nanofibers; ZnO nanofibers; selenium nanofibers; nanofibers that are fluorinated; nanofibers that are compounds of Mo, S, and I; and combinations thereof.

14. The process of claim 1 , wherein the nanofibers comprise carbon nanotubes.

15. A process for continuously producing a nanofiber sheet, ribbon, or yarn, the process comprising:

(a) synthesizing a nanofiber forest in a furnace growth region on a substrate, wherein the nanofiber forest comprises a parallel array of nanofibers having a degree of inter-fiber connectivity;

(b) drawing said nanofibers from the nanofiber forest to form a primary assembly that is a sheet, ribbon or yarn, wherein the substrate continuously moves from the furnace growth region into a region where the nanofibers in the forest are drawn; and

(c) infiltrating the primary assembly with a liquid and subsequently evaporating the liquid from the primary assembly, wherein the infiltration and evaporation at least partially densifies the primary assembly.

16. The process of claim 15 , wherein said infiltration with the liquid comprises a method selected from the group consisting of vapor condensation, imbibing a liquid, exposure to a liquid aerosol, and combinations thereof.

17. The process of claim 15 , wherein the liquid comprises a substance selected from the group consisting of water, acetone, ethanol, methanol, isopropyl alcohol, toluene, chloroform, chlorobenzene and combinations thereof.

18. The process of claim 15 , wherein the substrate is flexible.

19. The process of claim 15 , wherein the substrate is a flexible belt or is attached to a moving belt.

20. The process of claim 15 , wherein the substrate is a drum.

21. The process of claim 15 , wherein the drawing occurs without twisting when the primary assembly is a ribbon or a sheet and the drawing includes twisting when the primary assembly is a yarn.

22. The process of claim 15 , wherein the nanofibers comprise carbon nanotubes.

Assignments (3)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 24, 2017
From: ZHANG, MEI; FANG, SHAOLI; BAUGHMAN, RAY H; ZAKHIDOV, ANVAR ABDULAHADOVIC; ALIEV, ALI E; LI, SERGEY; WILLIAMS, CHRIS
To: BOARD OF REGENTS, THE UNIVERSITY OF TEXAS SYSTEM
Reel/Frame 041372/0447 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 24, 2017
From: ATKINSON, KENNETH ROSS
To: COMMONWEALTH SCIENTIFIC AND INDUSTRIAL RESEARCH ORGANISATION
Reel/Frame 041372/0579 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 24, 2017
From: COMMONWEALTH SCIENTIFIC AND INDUSTRIAL RESEARCH ORGANISATION
To: BOARD OF REGENTS, THE UNIVERSITY OF TEXAS SYSTEM
Reel/Frame 041372/0685 →
Continuity (7)
Continuation 14952244 · Nov 25, 2015
Division 14332632 · Jul 16, 2014
Continuation 11718954
Provisional Application 60702444 · Jul 26, 2005
Provisional Application 60666351 · Mar 30, 2005
Provisional Application 60626314 · Nov 9, 2004
Related Publication 20170137290A1 · May 18, 2017