IP Library Granted Patent US 10,279,318
Granted Patent B2
US 10,279,318 · App. 15/344,697 · Granted May 7, 2019

Robust carbon nanotube membranes and methods of making the same

Inventors: Seyed A. Dastgheib (Savoy, IL); Ali Ashraf (Beaverton, OR); SungWoo Nam (Savoy, IL)
Assignee: The Board of Trustees of the University of Illinois
B01D71/021B01D61/025B01D61/027B01D61/147B01D61/364B01D67/0039C02F1/441C02F1/442C02F1/444C02F2103/08
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Quick Facts
Patent No.
US 10,279,318
App. No.
15/344,697
Granted
May 7, 2019
Kind
B2
Abstract

Carbon nanotube membranes that are flexible, non-fragile, stable at high temperatures, superhydrophobic, have submicrometer openings, and are resistant to delamination and corrosive conditions are provided. The carbon nanotube membranes comprise carbon nanotubes grown on a microporous, metal substrate, e.g. silver, quartz fiber filter, and HAST. Methods of fabricating the carbon nanotubes are also provided.

Claims (9)

1. A carbon nanotube membrane comprising a substrate coated with carbon nanotubes, wherein the substrate has micrometer-sized openings and wherein the substrate is selected from silver, nickel sputtered silver, Hastelloy C22 (HAST) and quartz fiber filter.

2. The carbon nanotube membrane according to claim 1 , wherein the carbon nanotube membrane is resistant to thermal and oxidative weight loss up to about 500° C.

3. The carbon nanotube membrane according to claim 1 , wherein the carbon nanotube membrane is superhydrophobic.

4. The carbon nanotube membrane according to claim 1 , wherein the carbon nanotube membrane has pore openings of about 0.5 nm to about 500 nm.

5. The carbon nanotube membrane according to claim 1 , wherein the carbon nanotube membrane is flexible, non-fragile, and resistant to delamination and corrosive conditions, compared to a membrane with a stainless steel substrate.

6. A carbon nanotube membrane according to claim 1 , which is resistant to corrosion in acids or salt solutions, compared to a membrane with a stainless steel substrate.

7. A carbon nanotube membrane according to claim 6 wherein the acid is selected from hydrochloric acid, sulfuric acid, phosphoric acid, and nitric acid and wherein the salt solution is selected from a solution of sodium chloride or calcium chloride.

8. A carbon nanotube membrane according to claim 1 which is resistant to corrosion in water or humid conditions, compared to a membrane with a stainless steel substrate.

9. A carbon nanotube membrane according to claim 1 which is resistant to delamination and disintegration of the CNT structure, as determined in an adhesion performance test according to ASTM D3359 or as determined in a sonication performance test for 40 seconds at a frequency of 20 KHz and an input energy of 240 W/L using a Fisher Scientific F550 sonic dismembrator or equivalent instrument.

Assignments (2)
CONFIRMATORY LICENSE Recorded Jan 22, 2019
From: UNIVERSITY OF ILLINOIS AT URBANA-CHAMPAIGN
To: UNITED STATES DEPARTMENT OF ENERGY
Reel/Frame 048106/0958 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 23, 2017
From: DASTGHEIB, SEYED A.; ASHRAF, ALI; SALIH, HAFIZ; NAM, SUNGWOO
To: THE BOARD OF TRUSTEES OF THE UNIVERSITY OF ILLINOIS
Reel/Frame 041359/0836 →
Continuity (2)
Provisional Application 62266171 · Dec 11, 2015
Related Publication 20170165612A1 · Jun 15, 2017