IP Library Granted Patent US 10,036,754
Granted Patent B2
US 10,036,754 · App. 15/605,616 · Granted Jul 31, 2018

Water soluble fluorescent or colored dyes and methods for their use

Inventors: Tracy Matray (Snohomish, WA); Hesham Sherif (Redmond, WA)
Assignees: Sony Corporation; Sony Corporation of America
G01N33/583C07F9/093C07F9/094C07F9/2408C09B1/00C09B69/00G01N21/29G01N33/52
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Quick Facts
Patent No.
US 10,036,754
App. No.
15/605,616
Granted
Jul 31, 2018
Kind
B2
Abstract

Compounds useful as fluorescent or colored dyes are disclosed. The compounds have the following structure (I): including stereoisomers, salts and tautomers thereof, wherein R 1a , R 1b , R 2a , R 2b , R 2c , R 2d , R 2e , R 2f , R 2g , R 2h , R 2i , R 2j , R 2k , R 2l , R 2m , R 2n , R 2o , R 2p , R 2q , R 2r and R 2s are as defined herein. Methods associated with preparation and use of such compounds are also provided.

Claims (35)

1. A method of staining a sample, the method comprising adding to the sample an analyte molecule in an amount sufficient to produce an optical response when said sample is illuminated at an appropriate wavelength,

wherein:

the analyte molecule has the following structure (I′):

or a salt thereof, wherein:

R 1a and R 1b are each independently hydroxyl or alkoxy; and

R 2a , R 2b , R 2c , R 2d , R 2e , R 2f , R 2g , R 2h , R 2i , R 2j , R 2k , R 2l , R 2m , R 2n , R 2o , R 2p , R 2q , R 2r , R 2s and R 2t are each independently H, halo or -L 1 -R 3 ;

R 3 is, at each occurrence, independently a nucleic acid, peptide, carbohydrate, lipid, enzyme, receptor, receptor ligand, antibody, glycoprotein, aptamer, antigen, prion, drug, vitamin or small molecule; and

L 1 is an optional linker moiety,

wherein at least one of R 2a , R 2b , R 2c , R 2d , R 2e , R 2f , R 2g , R 2h , R 2i , R 2j , R 2k , R 2l , R 2m , R 2n , R 2o , R 2p , R 2q , R 2r , R 2s or R 2t is -L 1 -R 3 .

2. The method of claim 1 , wherein said optical response is a fluorescent response.

3. The method of claim 1 , wherein said sample comprises cells.

4. The method of claim 3 further comprising observing said cells by flow cytometry.

5. The method of claim 4 , further comprising distinguishing the fluorescence response from that of a second fluorophore having detectably different optical properties.

6. A method for visually detecting an analyte molecule, the method comprising:

(a) providing the analyte molecule; and

(b) detecting the analyte molecule by its visible properties

wherein:

the analyte molecule has the following structure (I′):

or a salt thereof, wherein:

R 1a and R 1b are each independently hydroxyl or alkoxy; and

R 2a , R 2b , R 2c , R 2d , R 2e , R 2f , R 2g , R 2h , R 2i , R 2j , R 2k , R 2l , R 2m , R 2n , R 2o , R 2p , R 2q , R 2r , R 2s and R 2t are each independently H, halo or -L 1 -R 3 ;

R 3 is, at each occurrence, independently a nucleic acid, peptide, carbohydrate, lipid, enzyme, receptor, receptor ligand, antibody, glycoprotein, aptamer, antigen, prion, drug, vitamin or small molecule; and

L 1 is an optional linker moiety,

wherein at least one of R 2a , R 2b , R 2c , R 2d , R 2e , R 2f , R 2g , R 2h , R 2i , R 2j , R 2k , R 2l , R 2m , R 2n , R 2o , R 2p , R 2q , R 2r , R 2s or R 2t is -L 1 -R 3 .

7. A method for visually detecting a biomolecule, the method comprising:

(a) admixing a compound with one or more biomolecules; and

(b) detecting the compound by its visible properties

wherein:

the compound has the following structure (I):

or a salt, stereoisomer or tautomer thereof, wherein:

R 1a and R 1b are each independently hydroxyl or alkoxy; and

R 2a , R 2b , R 2c , R 2d , R 2e , R 2f , R 2g , R 2h , R 2i , R 2j , R 2k , R 2l , R 2m , R 2n , R 2o , R 2p , R 2q , R 2r , R 2s and R 2t are each independently H, halo or -L 1 -R 3 ;

R 3 is, at each occurrence, independently the biomolecule, an alkyl substituted with one or more of hydroxyl, protected hydroxyl, amino, alkylamino, alkoxy, polyalkyether, hydroxylalkoxy, aminoalkoxy, hydroxylpolyalkyether, aminopolyalkyether, phosphate, thiophosphate, phospho, thiophospho, phosphoalkylether, Ophosphoalkylether, thiophosphoalkylether, Othiophosphoalkylether, phosphoramidite or activated phosphorous; or R 3 is a microparticle; and

L 1 is an optional linker moiety.

8. The method of claim 2 , wherein said sample comprises cells.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 14, 2020
From: SONY CORPORATION OF AMERICA
To: SONY CORPORATION
Reel/Frame 054751/0070 →
Continuity (3)
Continuation 15112395
Provisional Application 61928147 · Jan 16, 2014
Related Publication 20180100861A1 · Apr 12, 2018
Cited By (15)
US 12,194,104 US 12,270,812 US 12,275,851 US 12,290,571 US 12,319,817 US 12,359,071 US 12,391,833 US 12,461,106 US 12,473,433 US 12,539,334 US 12,560,612 US 12,577,403 US 12,578,342 US 12,606,588 US 12,629,425