IP Library Granted Patent US 10,512,910
Granted Patent B2
US 10,512,910 · App. 15/707,908 · Granted Dec 24, 2019

Droplet-based analysis method

Inventors: Billy W. Colston, Jr. (San Ramon, CA); Benjamin J. Hindson (Livermore, CA); Kevin D. Ness (Pleasanton, CA); Donald A. Masquelier (Tracy, CA)
Assignee: Bio-Rad Laboratories, Inc.
B01L3/50273B01F3/0807B01F13/0062B01F13/1022B01L3/502B01L3/502784B01L3/52B01L9/527C12Q1/686B01F5/0085B01F5/0256B01F13/0071B01L3/502761B01L2200/025B01L2200/0636B01L2200/0647B01L2200/0673B01L2200/14B01L2200/16B01L2300/0609B01L2300/0681B01L2300/0816B01L2300/0829B01L2300/0861B01L2400/049G01N35/08
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Quick Facts
Patent No.
US 10,512,910
App. No.
15/707,908
Filed
Sep 18, 2017
Granted
Dec 24, 2019
Kind
B2
Art Unit
1797
USPC
436/89
Abstract

Droplet-based methods of analysis. In an exemplary method, a device having a port connected to a chamber may be selected. A sample-containing fluid may be placed into the port. A pressure differential may be created that drives the sample-containing fluid from the port to the chamber and separates the sample-containing fluid into droplets. A two-dimensional monolayer of the droplets may be formed in the chamber. At least a portion of the monolayer may be imaged.

Claims (31)

1. A method of analysis, the method comprising:

selecting a device having a port connected to a chamber;

placing a sample-containing fluid into the port;

creating a pressure differential that drives the sample-containing fluid from the port to the chamber and separates the sample-containing fluid into droplets;

forming a two-dimensional monolayer of the droplets in the chamber; and

imaging at least a portion of the monolayer.

2. The method of claim 1 , wherein the step of placing includes a step of placing the sample-containing fluid as a continuous phase into a well of the device.

3. The method of claim 1 , wherein the droplets are aqueous droplets that are separated from one another by an immiscible carrier liquid.

4. The method of claim 1 , wherein the step of forming includes a step of collecting the droplets in a chamber having a height corresponding to a diameter of the droplets.

5. The method of claim 1 , wherein the step of creating a pressure differential includes a step of applying positive gas pressure or negative gas pressure to a port of the device.

6. The method of claim 1 , further comprising a step of thermally cycling the monolayer to promote nucleic acid amplification in a subset of droplets of the monolayer.

7. The method of claim 1 , wherein the step of imaging includes a step of detecting fluorescence from the monolayer.

8. The method of claim 1 , wherein the step of imaging creates one or more images of droplets of the monolayer, wherein only a subset of the droplets contain an analyte, and wherein the one or more images indicate whether the analyte is present in individual droplets.

9. The method of claim 8 , further comprising a step of determining a number of droplets containing the analyte using the one or more images.

10. The method of claim 8 , wherein the analyte is a nucleic acid target, further comprising a step of amplifying the nucleic acid target within the monolayer.

11. The method of claim 10 , wherein the step of amplifying includes a step of thermally cycling the monolayer to promote nucleic acid amplification in droplets thereof.

12. The method of claim 10 , wherein the droplets contain an intercalating dye or a probe, wherein the probe includes an oligonucleotide labeled with a fluorophore, and wherein the step of imaging includes a step of detecting fluorescence from the intercalating dye or the fluorophore.

13. The method of claim 1 , wherein the chamber lies in a plane and defines an area of the plane, and wherein the step of forming includes a step of covering a majority of the area with droplets.

14. A method of analysis, the method comprising:

selecting a device having a chamber connected separately to a port and a vent;

placing an aqueous fluid into the port;

applying gas pressure to the device to drive the aqueous fluid from the port to the chamber and form partitions of the aqueous fluid, the partitions being separated from one another by a carrier liquid;

amplifying a nucleic acid target in only of a subset of the partitions while the partitions are arranged in a two-dimensional monolayer in the chamber;

imaging at least a portion of the monolayer to create one or more images; and

determining whether individual partitions of the monolayer contain the nucleic acid target using the one or more images.

15. The method of claim 14 , wherein the chamber has a top wall facing a bottom wall, and wherein the chamber has a height measured between the top and bottom walls corresponding to a diameter of the partitions.

16. The method of claim 14 , wherein the chamber lies in a plane and defines an area of the plane, and wherein the step of amplifying is performed while a majority of the area is covered with partitions.

17. The method of claim 14 , wherein the port includes a well, and wherein the step of placing an aqueous fluid includes a step of placing the aqueous fluid into the well.

18. The method of claim 14 , wherein the step of imaging includes a step of detecting fluorescence from the monolayer.

19. The method of claim 14 , wherein the step of amplifying includes a step of thermally cycling the monolayer.

20. The method of claim 14 , wherein the step of applying gas pressure includes a step of applying positive gas pressure or negative gas pressure to the device.

Assignments (3)
MERGER Recorded Oct 8, 2019
From: QUANTALIFE, INC.
To: BIO-RAD QL, INC.
Reel/Frame 050658/0872 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 8, 2019
From: BIO-RAD QL, INC.
To: BIO-RAD LABORATORIES, INC.
Reel/Frame 050658/0888 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 8, 2019
From: COLSTON, BILLY WAYNE, JR.; HINDSON, BENJAMIN JOSEPH; NESS, KEVIN DEAN; MASQUELIER, DONALD ARTHUR; MILANOVICH, FRED PAUL; MODLIN, DOUGLAS N.; RIOT, VINCENT; BURD, SAMUEL; MAKAREWICZ, ANTHONY JOSEPH, JR.; BELGRADER, PHILLIP; BRIGHT, ISAAC J.; LUCERO, MICHAEL Y.
To: QUANTALIFE, INC.
Reel/Frame 050672/0742 →
Continuity (92)
Continuation 15351354 · Nov 14, 2016
Continuation In Part 12954634 · Nov 25, 2010
Continuation In Part 13400030 · Feb 17, 2012
Continuation In Part 14020742 · Sep 6, 2013
Continuation In Part 14159410 · Jan 20, 2014
Continuation In Part 14201752 · Mar 7, 2014
Continuation In Part 14848311 · Sep 8, 2015
Continuation In Part 12586626 · Sep 23, 2009
Continuation In Part 12862542 · Aug 24, 2010
Continuation In Part 12890550 · Sep 24, 2010
Continuation In Part 13245575 · Sep 26, 2011
Continuation In Part 13945661 · Jul 18, 2013
Continuation In Part 12962507 · Dec 7, 2010
Continuation In Part 12962511 · Dec 7, 2010
Continuation In Part 12962502 · Dec 7, 2010
Continuation In Part 12963523 · Dec 8, 2010
Continuation In Part 13039233 · Mar 2, 2011
Continuation In Part 12976827 · Dec 22, 2010
Continuation In Part 13341669 · Dec 30, 2011
Continuation In Part 13341678 · Dec 30, 2011
Continuation In Part 13072673 · Mar 25, 2011
Continuation In Part 13341688 · Dec 30, 2011
Continuation In Part 13287120 · Nov 1, 2011
Continuation In Part 13424304 · Mar 19, 2012
Continuation In Part 13548062 · Jul 12, 2012
Continuation In Part PCTUS2012048198 · Jul 25, 2012
Continuation In Part 13562198 · Jul 30, 2012
Continuation In Part 13287095 · Nov 1, 2011
Continuation In Part 13863231 · Apr 15, 2013
Continuation In Part 12586626 · Sep 23, 2009
Continuation 12586626 · Sep 23, 2009
Continuation In Part 13251016 · Sep 30, 2011
Continuation In Part 13245575 · Sep 26, 2011
Continuation In Part 12976827 · Dec 22, 2010
Continuation 12586626 · Sep 23, 2009
Continuation 12588626 · Sep 23, 2009
Continuation 12588626 · Sep 23, 2009
Continuation 12586626 · Sep 23, 2009
Continuation PCTUS2011030101 · Mar 25, 2011
Continuation PCTUS2011030077 · Mar 25, 2011
Continuation In Part 12586626 · Sep 23, 2009
Continuation PCTUS2011030097 · Mar 25, 2011
Continuation In Part 12976827 · Dec 22, 2010
Division 13385277 · Feb 9, 2012
Provisional Application 61194043 · Sep 23, 2008
Provisional Application 61206978 · Feb 5, 2009
Provisional Application 61271538 · Jul 21, 2009
Provisional Application 61275731 · Sep 1, 2009
Provisional Application 61277200 · Sep 21, 2009
Provisional Application 61277203 · Sep 21, 2009
Provisional Application 61277204 · Sep 21, 2009
Provisional Application 61277216 · Sep 21, 2009
Provisional Application 61277249 · Sep 21, 2009
Provisional Application 61277270 · Sep 22, 2009
Provisional Application 61275860 · Sep 2, 2009
Provisional Application 61309837 · Mar 2, 2010
Provisional Application 61309845 · Mar 2, 2010
Provisional Application 61341218 · Mar 25, 2010
Provisional Application 61317635 · Mar 25, 2010
Provisional Application 61380981 · Sep 8, 2010
Provisional Application 61409106 · Nov 1, 2010
Provisional Application 61409473 · Nov 2, 2010
Provisional Application 61410769 · Nov 5, 2010
Provisional Application 61417241 · Nov 25, 2010
Provisional Application 61317681 · Mar 25, 2011
Provisional Application 61467347 · Mar 24, 2011
Provisional Application 61341065 · Mar 25, 2010
Provisional Application 61454373 · Mar 18, 2011
Provisional Application 61507082 · Jul 12, 2011
Provisional Application 61510013 · Jul 20, 2011
Provisional Application 61511445 · Jul 25, 2011
Provisional Application 61513474 · Jul 29, 2011
Provisional Application 61601514 · Feb 21, 2012
Provisional Application 61624199 · Apr 13, 2012
Provisional Application 61264591 · Nov 25, 2009
Provisional Application 61317684 · Mar 25, 2010
Provisional Application 61317639 · Mar 25, 2010
Provisional Application 61341065 · Mar 25, 2010
Provisional Application 61444674 · Feb 18, 2011
Provisional Application 61449580 · Mar 4, 2011
Provisional Application 61453537 · Mar 16, 2011
Provisional Application 61478777 · Apr 25, 2011
Provisional Application 61488667 · May 20, 2011
Provisional Application 61490040 · May 25, 2011
Provisional Application 61697982 · Sep 7, 2012
Provisional Application 61775415 · Mar 8, 2013
Provisional Application 61441209 · Feb 9, 2011
Provisional Application 61444539 · Feb 18, 2011
Provisional Application 61476115 · Apr 15, 2011
Provisional Application 61484197 · May 9, 2011
Provisional Application 61490055 · May 25, 2011
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