IP Library Granted Patent US 10,647,638
Granted Patent B2
US 10,647,638 · App. 15/779,615 · Granted May 12, 2020

Method for producing butadiene

Inventors: Sosuke Higuchi (Tokyo, JP); Nobuhiro Kimura (Tokyo, JP)
Assignee: JXTG Nippon Oil & Energy Corporation
C07C5/48B01J23/002B01J23/31B01J23/8876B01J37/04B01J37/088C07C11/167B01J2523/54B01J2523/68C07C2523/18C07C2523/28C07C2523/31C07C2523/745C07C2523/75C07C2523/887
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Quick Facts
Patent No.
US 10,647,638
App. No.
15/779,615
Granted
May 12, 2020
Kind
B2
Abstract

A method for producing butadiene comprises a step of obtaining a product gas containing butadiene, by feeding a raw-material gas containing straight-chain butene and an oxygen-containing gas containing molecular oxygen to a reactor and performing oxidative dehydrogenation reaction in the presence of a catalyst, wherein the catalyst comprises a composite oxide containing molybdenum and bismuth, and the concentration of hydrocarbons having 5 or more carbon atoms in the raw-material gas is 0.05 mol % to 7.0 mol %.

Claims (11)

1. A method for producing butadiene, comprising:

providing a raw material gas comprising straight-chain butene and an oxygen-containing gas comprising molecular oxygen,

adding hydrocarbons having 5 or more carbon atoms to the raw material gas or adjusting the amount of hydrocarbons having 5 or more carbon atoms in the raw material gas to obtain an amount of hydrocarbons having 5 or more carbons atoms in the raw material gas in the range of 0.2-7.0 mol %, and

performing oxidative dehydrogenation reaction of the raw material gas with the oxygen-containing gas in a reactor and in the presence of a catalyst to produce a product gas comprising butadiene,

wherein:

the catalyst comprises a composite oxide containing molybdenum and bismuth;

the concentration of isobutene in the raw material gas is 1.0 mol % or less;

the concentration of butadiene in the raw material gas is 1.0 mol % or less; and

the amount of hydrocarbons having 5 or more carbon atoms in the raw material gas allows dissolving by-products of the oxidative dehydrogenation reaction and prevents reactor blockage.

2. The method according to claim 1 , wherein the amount of hydrocarbons having 5 or more carbon atoms in the raw-material gas is in the range of 0.2-6.0 mol %.

3. The method according to claim 1 , wherein the concentration of the straight-chain butene in the raw-material gas is 60 mol % or more.

Assignments (2)
CHANGE OF NAME Recorded Oct 9, 2020
From: JXTG NIPPON OIL & ENERGY CORPORATION
To: ENEOS CORPORATION
Reel/Frame 054036/0001 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 29, 2018
From: HIGUCHI, SOSUKE; KIMURA, NOBUHIRO
To: JXTG NIPPON OIL & ENERGY CORPORATION
Reel/Frame 045920/0373 →
Priority Claims (1)
JP 2015-234994 · Dec 1, 2015 · national
Continuity (1)
Related Publication 20180346395A1 · Dec 6, 2018