IP Library Granted Patent US 12,306,154
Granted Patent B2
US 12,306,154 · App. 15/832,379 · Granted May 20, 2025

Meltable color changeable indicators with organic polymer cores and methods of making such meltable indicators and composites thereof

Inventors: Gregory L. Heacock (Maple Valley, WA); Andrew Mills (Holywood, GB)
Assignee: THERMOGRAPHIC MEASUREMENTS LIMITED
G01N31/223B29C48/04B32B27/00C08J3/02C08J3/126C08J3/226C08K5/17C08K9/10C08L23/04C08L23/06C08L23/12C08L25/06C08L33/12C08K5/0041C08K5/42C08K5/46C08L2666/70
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Quick Facts
Patent No.
US 12,306,154
App. No.
15/832,379
Granted
May 20, 2025
Kind
B2
Abstract

Color changeable indicator particles having a meltable, particulate organic core, and at least one color changeable indicator coated on the particulate organic core. Color changeable indicator particles can be incorporated into composite polymer materials while maintaining the efficacy and stability of the indicator. The indicators provide simple, reliable, and cost effective detection means for detecting ammonia and carbon dioxide, and may find use in applications such as food packaging and medical applications.

Claims (11)

1. A color changeable organic polymeric composite comprising:

bulk organic polymer;

organic polymer core particles; and

organic color changeable indicator dye that detects the presence of a chemical substance, wherein the organic color changeable indicator dye is coated on the organic polymer core particles to form organic indicator particles, wherein the organic indicator particles have an average particle size between 10 and 1000 microns, wherein the bulk organic polymer is extruded or melted with the organic indicator particles to produce the color changeable organic polymer composite, wherein the organic color changeable indicator dye is substantially homogeneously dispersed within and throughout the color changeable organic polymer composite, and wherein the color changeable organic polymer composite substantially lacks inorganic particulates, and wherein the color changeable organic polymeric composite is in the form of a film having a thickness of approximately 10 microns to approximately 250 microns.

2. The color changeable organic polymeric composite of claim 1 wherein the color changeable organic polymeric composite is substantially free of aggregation of the organic color changeable indicator dye.

3. The color changeable organic polymeric composite of claim 1 wherein the at least one bulk organic polymer and the at least one core organic polymer are selected from the group consisting of low density polyethylene (LDPE), polystyrene (PS), polymethylmethacrylate (PMMA), polypropylene (PP), polycaprolactone (PCL), and mixtures thereof.

4. The color changeable organic polymeric composite of claim 1 wherein the at least one organic color changeable indicator dye is a carbon dioxide-based indicator dye.

5. The color changeable organic polymeric composite of claim 1 wherein the at least one organic color changeable indicator dye is an ammonia-based indicator dye.

6. The color changeable organic polymeric composite of claim 1 wherein the at least one organic color changeable indicator dye is selected from the group consisting of: metacresol purple (MCP), thymol blue (TB), phenol red (PR), cresol red (CR), bromocresol green (BCG), bromophenol blue (BPB), chlorophenol red (CPR), methylene blue (MB), and mixtures thereof.

7. The color changeable organic polymeric composite of claim 1 wherein the at least one bulk organic polymer is LDPE and the organic color changeable indicator dye is selected from metacresol purple (MCP), thymol blue (TB) and phenol red (PR).

8. The color changeable organic polymeric composite of claim 1 wherein the color changeable organic polymeric composite is incorporated into or disposed on a ring.

Assignments (3)
SECURITY INTEREST Recorded Oct 15, 2024
From: THERMOGRAPHIC MEASUREMENTS LIMITED
To: BARINGS FINANCE LLC
Reel/Frame 068895/0356 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 10, 2023
From: SENSOR INTERNATIONAL, LLC
To: THERMOGRAPHIC MEASUREMENTS LIMITED
Reel/Frame 063590/0203 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 6, 2017
From: HEACOCK, GREGORY L; MILLS, ANDREW
To: SENSOR INTERNATIONAL, LLC
Reel/Frame 044313/0658 →
Continuity (1)
Related Publication 20190170714A1 · Jun 6, 2019
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