BENZYL (METH)ACRYLATE MONOMERS SUITABLE FOR MICROSTRUCTURED OPTICAL FILMS
Presently described are optical films comprising a polymerized (e.g. microstructured) surface that comprises the reaction product of a polymerizable resin composition and polymerizable resin compositions that comprise nanoparticles; at least one first monomer comprising at least two (meth)acrylate groups; and at least one second (meth)acrylate monomer having the structure wherein at least one R1 comprises an aromatic substituent, t is an integer from 1 to 4, and R2 is hydrogen or methyl.
1 . An optical film comprising a polymerized microstructured surface that comprises the reaction product of a polymerizable resin composition comprising
nanoparticles;
at least one first monomer comprising at least two (meth)acrylate groups; and
at least one second (meth)acrylate monomer having the structure
wherein at least one R1 comprises an aromatic substituent,
t is an integer from 1 to 4, and
R2 is hydrogen or methyl.
2 . The optical film of claim 1 wherein t is 1.
3 . The optical film of claim 1 wherein R1 is selected from the group consisting
4 . The optical film of claim 1 wherein the monomer has a refractive index of at least 1.54.
5 . The optical film of claim 1 wherein the monomer has a viscosity of less than 100 cps at 25° C.
6 . The optical film of claim 1 wherein the first monomer comprises at least two aromatic rings.
7 . The optical film of claim 6 wherein the first monomer is a bisphenol, fluorene or biphenyl (meth)acrylate monomer.
8 . The optical film of claim 1 wherein the polymerizable resin comprises up to 15 wt-% of one or more first monomers comprising at least two (meth)acrylate groups.
9 . The optical film of claim 1 wherein the first monomer comprising at least two (meth)acrylate groups has a molecular weight of at least 350 g/mole.
10 . The optical film of claim 1 wherein the polymerizable resin composition is non-halogenated.
11 . The optical film of claim 1 wherein the nanoparticles have a refractive index of at least 1.60.
12 . The optical film of claim 11 wherein the nanoparticles comprise zirconia.
13 . The optical film of claim 11 wherein the polymerizable resin comprises at least 40 wt-% nanoparticles.
14 . The optical film of claim 1 wherein the optical film is a brightness enhancing film.
15 . The optical film of claim 14 wherein the brightness enhancing film has a single sheet relative gain of at least 1.75.
16 . An optical film comprising a polymerized surface that comprises the reaction product of a polymerizable resin composition comprising
nanoparticles;
at least one first monomer comprising at least two (meth)acrylate groups; and
at least one second (meth)acrylate monomer having the structure
wherein at least one R1 comprises an aromatic substituent,
t is an integer from 1 to 4, and
R2 is hydrogen or methyl.
17 . A polymerizable resin composition comprising
nanoparticles;
at least one first monomer comprising at least two (meth)acrylate groups; and
at least one second (meth)acrylate monomer having the structure
wherein at least one R1 comprises an aromatic substituent,
t is an integer from 1 to 4, and
R2 is hydrogen or methyl.