IP Library Granted Patent US 10,559,449
Granted Patent B2
US 10,559,449 · App. 15/844,854 · Granted Feb 11, 2020

Stable support films for electron microscopy

Inventors: Robert M. Glaeser (Berkeley, CA); Bong-Gyoon Han (Castro Valley, CA)
Assignee: The Regents of the University of California
H01J37/20H01J37/261H01J2237/2007
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Quick Facts
Patent No.
US 10,559,449
App. No.
15/844,854
Granted
Feb 11, 2020
Kind
B2
Abstract

This disclosure provides systems, methods, and apparatus related to arrangements including electron microscopy grids. In one aspect an arrangement includes an electron microscopy grid. The electron microscopy grid comprises a first surface and a second surface, with the first surface having a holey carbon film disposed thereon. A plurality of lipid molecules are disposed in a hole in the holey carbon film. Each lipid molecule of the plurality of lipid molecules has a hydrophilic head and a hydrophobic tail. A biotin-binding protein is attached to the hydrophilic heads of the plurality of lipid molecules. The biotin-binding protein is crystalline.

Claims (34)

1. An arrangement comprising:

an electron microscopy grid, the electron microscopy grid comprising a first surface and a second surface, the first surface having a holey carbon film disposed thereon;

a plurality of lipid molecules disposed in a hole in the holey carbon film, the hole in the holey carbon film having a dimension of about 1 micron to 2 microns, each lipid molecule of the plurality of lipid molecules having a hydrophilic head and a hydrophobic tail;

a biotin-binding protein attached to hydrophilic heads of the plurality of lipid molecules, the biotin-binding protein being crystalline, a crystal of the biotin-binding protein spanning the hole in the holey carbon film; and

small molecules disposed on the biotin-binding protein, the small molecules operable to preserve a structure of the biotin-binding protein at room temperature.

2. The arrangement of claim 1 , wherein the small molecules form a layer, and wherein the layer is about 50 nanometers to 150 nanometers thick.

3. The arrangement of claim 1 , further comprising:

a layer of carbon disposed on hydrophobic tails of the plurality of lipid molecules.

4. The arrangement of claim 3 , wherein the layer of carbon has a thickness of 5 nanometers or less.

5. The arrangement of claim 1 , wherein the plurality of lipid molecules comprises a homogenous mixture of lipid molecules with biotinylated head groups.

6. The arrangement of claim 1 , wherein the plurality of lipid molecules comprises a heterogeneous mixture of lipid molecules, and wherein at least a part of the heterogeneous mixture comprises lipid molecules with biotinylated head groups.

7. The arrangement of claim 1 , wherein the biotin-binding protein comprises streptavidin.

8. The arrangement of claim 1 , wherein the small molecules are selected from a group consisting of trehalose, glucose, betaine, proline, and glycine.

9. The arrangement of claim 1 , wherein the holey carbon film is about 10 nanometers to 25 nanometers thick.

10. A method comprising:

(a) providing an electron microscopy grid, the electron microscopy grid comprising a first surface and a second surface, the first surface having a holey carbon film disposed thereon;

(b) providing a plurality of lipid molecules, each lipid molecule of the plurality of lipid molecules having a hydrophilic head and a hydrophobic tail;

(c) contacting the holey carbon film with hydrophobic tails of the plurality of lipid molecules to form a lipid monolayer disposed in a hole in the holey carbon film, the lipid monolayer comprising a portion of the plurality of lipid molecules;

(d) after operation (c), attaching a biotin-binding protein to hydrophilic heads of the lipid monolayer; and

(e) after operation (d), allowing a period of time to elapse to allow the biotin-binding protein to crystalize while being attached to the hydrophilic heads of the lipid monolayer disposed in the hole in the holey carbon film.

11. The method of claim 10 , further comprising:

depositing small molecules on the biotin-binding protein after operation (e).

12. The method of claim 10 , further comprising:

depositing a layer of carbon on the hydrophobic tails of the lipid monolayer.

13. The method of claim 10 , further comprising:

removing the biotin-binding protein that is not attached to the hydrophilic heads of the lipid monolayer after operation (d).

14. The method of claim 10 , wherein the period of time in operation (e) is about 1 minute to 20 minutes.

15. The method of claim 10 , wherein the plurality of lipid molecules comprises a homogenous mixture of lipid molecules with biotinylated head groups.

16. The method of claim 10 , wherein the plurality of lipid molecules comprises a heterogeneous mixture of lipid molecules, and wherein at least part of the heterogeneous mixture comprises lipid molecules with biotinylated head groups.

17. The method of claim 10 , wherein the biotin-binding protein comprises streptavidin.

18. The method of claim 11 , wherein the small molecules are selected a group consisting of trehalose, glucose, betaine, proline, and glycine.

19. The method of claim 10 , wherein the holey carbon film is about 10 nanometers to 25 nanometers thick, and wherein the hole in the holey carbon film has dimensions of about 1 micron to 2 microns.

20. The arrangement of claim 1 , wherein the hole in the holey carbon film has dimensions of about 2 microns.

21. The method of claim 11 , wherein the small molecules form a layer, and wherein the layer is about 50 nanometers to 150 nanometers thick.

Assignments (2)
CONFIRMATORY LICENSE Recorded Mar 28, 2018
From: UNIVERSITY OF CALIF-LAWRENC BERKELEY LAB
To: UNITED STATES DEPARTMENT OF ENERGY
Reel/Frame 045370/0126 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 12, 2018
From: GLAESER, ROBERT M.; HAN, BONG-GYOON
To: THE REGENTS OF THE UNIVERSITY OF CALIFORNIA
Reel/Frame 044606/0659 →
Continuity (3)
Continuation PCTUS2016038683 · Jun 22, 2016
Provisional Application 62184532 · Jun 25, 2015
Related Publication 20180108510A1 · Apr 19, 2018