IP Library Granted Patent US 10,946,361
Granted Patent B2
US 10,946,361 · App. 15/866,179 · Granted Mar 16, 2021

Compositions and methods for selectively sequestering metal ions

Inventors: Matthew D. Shoulders (Cambridge, MA); Stephen J. Lippard (Washington, DC); Elizabeth Marie Nolan (Cambridge, MA); Christopher E. R. Richardson (Boston, MA); Lisa S. Cunden (Somerville, MA)
Assignee: Massachusetts Institute of Technology
B01J20/3274C07K14/47C08L5/12B01D2257/60
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Quick Facts
Patent No.
US 10,946,361
App. No.
15/866,179
Granted
Mar 16, 2021
Kind
B2
Abstract

Compositions and methods for the selective sequestration of metal ions are generally described.

Claims (23)

1. A composition, comprising:

a plurality of S100 protein molecules; and

a support comprising a plurality of functional groups,

wherein the plurality of S100 protein molecules are covalently immobilized on the support via reactions between the plurality of functional groups and amine groups of the plurality of S100 protein molecules, such that the covalently immobilized S100 protein molecules have binding sites available for chelation of metal ions and are thus configured to selectively sequester metal ions.

2. The composition of claim 1 , wherein the plurality of S100 protein molecules is a plurality of S100A12 protein molecules.

3. The composition of claim 1 , wherein the support is a solid support.

4. The composition of claim 1 , wherein the support is agarose resin.

5. The composition of claim 4 , wherein the agarose resin is N-hydroxy-succinimide-modified agarose resin.

6. The composition of claim 1 , wherein the plurality of S100 protein molecules is covalently attached to the support through amide linkages.

7. The composition of claim 1 , wherein the functional groups are ester groups.

8. The composition of claim 1 , wherein selectively sequestering metal ions comprises:

exposing the composition to a sample comprising a plurality of a first type of metal ion and a plurality of a second type of metal ion;

wherein following the exposing step, greater than about 90% of the first type of metal ion in the sample are sequestered by the plurality of S100 protein molecules immobilized on the support, and;

less than about 5% of the second type of metal ion in the sample are sequestered by the plurality of S100 protein molecules immobilized on the support.

9. A composition, comprising:

a plurality of S100 protein molecules; and

a support comprising a plurality of functional groups,

wherein the plurality of S100 protein molecules are covalently immobilized on the support via reactions between the plurality of functional groups and amine groups of the plurality of S100 protein molecules,

whereby the covalently immobilized protein molecules have more binding sites available for chelation of metal ions than an essentially identical comparative protein immobilized on a comparative support via reactions between carboxy functional groups on the comparative protein and functional groups on the comparative support, such that the covalently immobilized protein molecules are thus better able to carry out their function as compared to the comparative protein immobilized on the comparative support,

wherein the function comprises:

exposing the composition to a sample comprising a plurality of a first type of metal ion and a plurality of a second type of metal ion,

wherein following the exposing step, greater than about 90% of the first type of metal ion in the sample are sequestered by the plurality of protein molecules immobilized on the support, and

less than about 5% of the second type of metal ion in the sample are sequestered by the plurality of protein molecules immobilized on the support.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 19, 2018
From: SHOULDERS, MATTHEW D.; LIPPARD, STEPHEN J.; NOLAN, ELIZABETH MARIE; RICHARDSON, CHRISTOPHER E.R.; CUNDEN, LISA S.
To: MASSACHUSETTS INSTITUTE OF TECHNOLOGY
Reel/Frame 047872/0480 →
CONFIRMATORY LICENSE Recorded Feb 27, 2018
From: MASSACHUSETTS INSTITUTE OF TECHNOLOGY
To: NATIONAL SCIENCE FOUNDATION
Reel/Frame 045450/0529 →
Continuity (1)
Related Publication 20190210005A1 · Jul 11, 2019