IP Library Granted Patent US 11,248,125
Granted Patent B2
US 11,248,125 · App. 15/939,345 · Granted Feb 15, 2022

Coating system for aluminum-magnesium alloys

Inventors: Jason J. Benkoski (Catonsville, MD); Christopher M. Hoffman, Jr. (Odenton, MD); Rengaswamy Srinivasan (Ellicott City, MD); Keith S. Caruso (Catonsville, MD)
Assignee: The Johns Hopkins University
C09D5/002C09D1/02C09D1/04C09D5/004C09D5/084C09D5/086C09D7/60C09D7/61C09D7/63C09D7/65C09D183/04C09K3/18C08K2003/265
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Quick Facts
Patent No.
US 11,248,125
App. No.
15/939,345
Granted
Feb 15, 2022
Kind
B2
Abstract

A coating system may be configured to be applied to an aluminum-magnesium substrate of an object. The coating system may include a primer configured to reduce the corrosion rate of the aluminum-magnesium substrate and a topcoat configured to resist water and improve solar reflectance of the coating system. The primer may include a silicate and a first additive configured to increase corrosion resistance of the coating system The topcoat may include a siloxane and a second additive configured to reduce solar absorptance of the coating system.

Claims (20)

1. A coating system disposed on an aluminum-magnesium substrate of an object, the coating system comprising:

a primer in the form of an insoluble film and configured to reduce the corrosion rate of the aluminum-magnesium substrate, the primer comprising a silicate, and a plurality of first additives configured to increase corrosion resistance of the coating system, wherein the plurality of first additives includes cerium (III) phosphate in powder form, a dibasic ester, 3-glycidyloxypropyltriethoxysilane, and polyethyleneimine; wherein the polyethyleneimine and the silicate define a co-continuous polymer network, wherein the silicate is covalently coupled to the polyethyleneimine via the 3-glycidyloxypropyltriethoxysilane and wherein the silicate has a reduced tendency to crack upon drying by virtue of being incorporated into the co-continuous polymer network; and

a topcoat configured to resist water and improve solar reflectance of the coating system, the topcoat comprising a siloxane and a second additive configured to reduce solar absorptance of the coating system.

2. The coating system of claim 1 , wherein the silicate is potassium silicate.

3. The coating system of claim 1 , wherein the primer comprises 30% to 60% of the silicate by weight of the primer.

4. The coating system of claim 1 , wherein the siloxane is polydimethylsiloxane.

5. The coating system of claim 1 , wherein the topcoat comprises 30% to 60% of the siloxane by weight of the topcoat.

6. The coating system of claim 1 , wherein the primer further comprises any one of zinc oxide, or a silane.

7. The coating system of claim 1 , wherein the primer further comprises methyltrimethoxysilane or dimethyldimethoxysilane.

8. The coating system of claim 1 , wherein the second additive is calcium carbonate.

9. The coating system of claim 1 , wherein the primer comprises from 0.1% to 10% of the polyethyleneimine by weight of the primer.

10. The coating system of claim 1 , wherein the primer comprises from 0.1% to 5% of the 3-glycidyloxypropyltriethoxysilane by weight of the primer.

11. The coating system of claim 1 , wherein the primer comprises 0.1% to 2% of the cerium (III) phosphate by weight of the primer.

12. The coating system of claim 1 , wherein the primer has a ratio between 3-glycidyloxypropyltriethoxysilane and polyethyleneimine from 0.4 to 1.

13. A coating system configured to be applied to an aluminum-magnesium substrate of an object, the coating system comprising:

a primer configured to reduce the corrosion rate of the aluminum-magnesium substrate, the primer comprising (i) a silicate, (ii) cerium (III) phosphate in powder form, (iii) a dibasic ester, (iv) zinc oxide, (v) 3-glycidyloxypropyltriethoxysilane, (vi) methyltrimethoxysilane or dimethyldimethoxysilane, and (vii) polyethyleneimine; wherein the polyethyleneimine forms a co-continuous polymer network with the silicate via the 3-glycidoxypropyltrimethoxysilane that covalently couples the silicate to the polyethyleneimine, and wherein the silicate has a reduced tendency to crack upon drying by virtue of being incorporated into the co-continuous polymer network; and

a topcoat configured to resist water and improve solar reflectance of the coating system, the topcoat comprising a siloxane and a second additive configured to reduce solar absorptance of the coating system.

14. The coating system of claim 13 , wherein the primer further comprises glycerol and fumed silica.

15. The coating system of claim 14 , wherein the primer consists of (i) a silicate, (ii) cerium (III) phosphate in powder form, (iii) a dibasic ester, (iv) zinc oxide, (v) 3-glycidyloxypropyltriethoxysilane, (vi) methyltrimethoxysilane or dimethyldimethoxysilane, (vii) polyethyleneimine, (viii) glycerol, and (ix) fumed silica; wherein the primer has a ratio between 3-glycidoxypropyltrimethoxysilane and polyethyleneimine from 0.4 to 1.

16. The coating system of claim 15 , wherein the primer is disposed onto the aluminum-magnesium substrate and is provided in a dried state.

Assignments (3)
CONFIRMATORY LICENSE Recorded Jan 16, 2019
From: JOHNS HOPKINS UNIVERSITY
To: NAVY, SECRETARY OF THE UNITED STATES OF AMERICA
Reel/Frame 048119/0783 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Apr 20, 2018
From: BENKOSKI, JASON J.; SRINIVASAN, RENGASWAMY; CARUSO, KEITH S.
To: THE JOHNS HOPKINS UNIVERSITY
Reel/Frame 045597/0023 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 29, 2018
From: HOFFMAN, CHRISTOPHER M., JR.
To: THE JOHNS HOPKINS UNIVERSITY
Reel/Frame 045381/0132 →
Continuity (2)
Provisional Application 62513455 · Jun 1, 2017
Related Publication 20190031886A1 · Jan 31, 2019